Comb-assisted spectroscopy of CO2 absorption profiles in the near- and mid-infrared regions


A method of performing comb-assisted spectroscopy in the 2- and 4-μm wavelength regions is deeply discussed and applied to the spectroscopic characterization of absorption lines of a CO2 gas sample. The method relies on the use of a sum-frequency-generation scheme to relate the frequency of the probing laser to a frequency comb provided by an Er:fiber femtosecond oscillator. Controlled scans of the comb repetition frequency allow highly accurate and reproducible acquisition of the absorption spectra, which are used for subsequent retrieval of the underlying spectroscopic parameters.

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  1. 1.

    F. Chevalier, F.-M. Bréon, P.J. Rayner, J. Geophys. Res. 112, 1–11 (2007)

    Google Scholar 

  2. 2.

    D. Crisp, R.M. Atlas, F.-M. Breon, L.R. Brown, J.P. Burrows, P. Ciais, B.J. Connor, S.C. Doney, I.Y. Fung, D.J. Jacob, C.E. Miller, D. O’Brien, S. Pawson, J.T. Randerson, P. Rayner, R.J. Salawitch, S.P. Sander, B. Sen, G.L. Stephens, P.P. Tans, G.C. Toon, P.O. Wennberg, S.C. Wofsy, Y.L. Yung, Z. Kuang, B. Chudasama, G. Sprague, B. Weiss, R. Pollock, D. Kenyon, S. Schroll, Adv. Space Res. 34, 700 (2004)

    ADS  Article  Google Scholar 

  3. 3.

    H. Boesch, D. Baker, B. Connor, D. Crisp, C. Miller, Remote Sens. Environ. 3, 270 (2011)

    Google Scholar 

  4. 4.

    D.A. Long, K. Bielska, D. Lisak, D.K. Havey, M. Okumura, C.E. Miller, J.T. Hodges, J. Chem. Phys. 135, 064308 (2011)

    Article  Google Scholar 

  5. 5.

    A. Castrillo, E. Fasci, G. Galzerano, G. Casa, P. Laporta, L. Gianfrani, Opt. Express 18, 21851 (2010)

    ADS  Article  Google Scholar 

  6. 6.

    A. Castrillo, G. Gagliardi, G. Casa, L. Gianfrani, Phys. Rev. A 67, 062503 (2003)

    ADS  Article  Google Scholar 

  7. 7.

    Th. Udem, R. Holzwarth, T.W. Hänsch, Nature 416, 233 (2002)

    ADS  Article  Google Scholar 

  8. 8.

    D.J. Jones, S.A. Diddams, J.K. Ranka, A. Stentz, R.S. Windeler, J.L. Hall, S.T. Cundiff, Science 288, 635 (2000)

    ADS  Article  Google Scholar 

  9. 9.

    P. Balling, M. Fischer, P. Kubina, R. Holzwarth, Opt. Express 13, 9196 (2005)

    ADS  Article  Google Scholar 

  10. 10.

    J. Jiang, A. Onae, H. Matsumoto, F.-L. Hong, Opt. Express 13, 1958 (2005)

    ADS  Article  Google Scholar 

  11. 11.

    S. Borri, S. Bartalini, I. Galli, P. Cancio, G. Giusfredi, D. Mazzotti, A. Castrillo, L. Gianfrani, P. De Natale, Opt. Express 16, 11637 (2008)

    ADS  Article  Google Scholar 

  12. 12.

    F.-L. Hong, A. Onae, J.J.R. Guo, H. Inaba, K. Minoshima, T.R. Schibli, H. Matsumoto, K. Nakagawa, Opt. Lett. 28, 2324 (2003)

    ADS  Article  Google Scholar 

  13. 13.

    G. Galzerano, A. Gambetta, E. Fasci, A. Castrillo, M. Marangoni, P. Laporta, L. Gianfrani, Appl. Phys. B 102, 725 (2011)

    ADS  Article  Google Scholar 

  14. 14.

    V. Ahtee, M. Merimaa, K. Nyholm, Opt. Lett. 34, 2619 (2009)

    ADS  Article  Google Scholar 

  15. 15.

    C.P. McRaven, M.J. Cich, G.V. Lopez, T.J. Sears, D. Hurtmans, A.W. Mantz, J. Mol. Spectrosc. 266, 43 (2011)

    ADS  Article  Google Scholar 

  16. 16.

    M.J. Cich, C.P. McRaven, G.V. Lopez, T.J. Sears, D. Hurtmans, A.W. Mantz, Appl. Phys. B 1, 1–12 (2011)

    Google Scholar 

  17. 17.

    K.M.T. Yamada, A. Onae, F.-L. Hong, H. Inaba, H. Matsumoto, Y. Nakajima, F. Ito, T. Shimizu, J. Mol. Spectrosc. 249, 95 (2008)

    ADS  Article  Google Scholar 

  18. 18.

    P. Malara, P. Maddaloni, G. Gagliardi, P. De Natale, Opt. Express 16, 8242 (2008)

    ADS  Article  Google Scholar 

  19. 19.

    M. Vainio, M. Merimaa, L. Halonen, Opt. Lett. 36, 4122 (2011)

    ADS  Article  Google Scholar 

  20. 20.

    S. Bartalini, P. Cancio, G. Giusfredi, D. Mazzotti, P. De Natale, S. Borri, I. Galli, T. Leveque, L. Gianfrani, Opt. Lett. 32, 988 (2007)

    ADS  Article  Google Scholar 

  21. 21.

    M. Zimmermann, C. Gohle, R. Holzwarth, Th. Udem, Th.W. Hansch, Opt. Lett. 29, 310 (2004)

    ADS  Article  Google Scholar 

  22. 22.

    S.M. Foreman, A. Marian, J. Ye, E.A. Petrukhin, M.A. Gubin, O.D. Mücke, F.N.C. Wong, E.P. Ippen, F.X. Kärtner, Opt. Lett. 30, 570 (2005)

    ADS  Article  Google Scholar 

  23. 23.

    A. Amy-Klein, A. Goncharov, M. Guinet, Opt. Lett. 30, 3320 (2005)

    ADS  Article  Google Scholar 

  24. 24.

    N. Coluccelli, A. Gambetta, D. Gatti, M. Marangoni, A. Di Lieto, M. Tonelli, G. Galzerano, P. Laporta, Opt. Lett. 36, 2299 (2011)

    Article  Google Scholar 

  25. 25.

    R.W. Boyd, Nonlinear Optics, 2nd edn. (Academic Press, San Diego, 2003)

    Google Scholar 

  26. 26.

    D. Gatti, A. Gambetta, A. Castrillo, G. Galzerano, P. Laporta, L. Gianfrani, M. Marangoni, Opt. Express 19, 17520 (2011)

    ADS  Article  Google Scholar 

  27. 27.

    N. Newbury, W. Swann, J. Opt. Soc. Am. B 24, 1756 (2007)

    ADS  Article  Google Scholar 

  28. 28.

    C. Erny, K. Moutzouris, J. Biegert, D. Kuhlke, F. Adler, A. Leitenstorfer, U. Keller, Opt. Lett. 32, 1138 (2007)

    ADS  Article  Google Scholar 

  29. 29.

    A. Gambetta, R. Ramponi, M. Marangoni, Opt. Lett. 33, 2671 (2008)

    ADS  Article  Google Scholar 

  30. 30.

    L. Tombez, J. Di Francesco, S. Schilt, G. Di Domenico, J. Faist, P. Thomann, D. Hofstetter, Opt. Lett. 36, 3109 (2011)

    ADS  Article  Google Scholar 

  31. 31.

    A. Gambetta, D. Gatti, A. Castrillo, G. Galzerano, P. Laporta, L. Gianfrani, M. Marangoni, Appl. Phys. Lett. 99, 251107 (2011)

    Article  Google Scholar 

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The authors acknowledge support by the EU FP7 FET project CROSS TRAP (Contract No. ICT-244068).

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Correspondence to M. Marangoni.

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Gambetta, A., Gatti, D., Castrillo, A. et al. Comb-assisted spectroscopy of CO2 absorption profiles in the near- and mid-infrared regions. Appl. Phys. B 109, 385–390 (2012).

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  • Quantum Cascade Laser
  • Frequency Comb
  • Phase Lock
  • Slave Laser
  • Master Laser