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Enhanced stimulated Raman scattering by intermolecular Fermi resonance

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Abstract

We demonstrate the stimulated Raman scattering (SRS) of a binary solution of toluene and m-xylene at different volume concentrations in liquid-core optical fiber (LCOF). The results show that SRS of three vibration modes of 1002 cm−1,2920 cm−1 and 3058 cm−1 bands are simultaneously generated at some volume concentrations. The 2920 cm−1 band and the 3058 cm−1 band are generated at one time, the SRS thresholds of the first-order Stokes of the 2920 cm−1 and 3058 cm−1 bands are lower compared with the second-order Stokes threshold of the 1002 cm−1 band and the main peak of the 2920 cm−1 and 3058 cm−1 bands changes from the 2920 cm−1 band to the 3058 cm−1 band as the volume concentrations are changed. We assume that these phenomena are attributed to the intermolecular Fermi resonance. Raman scattering cross section (RSCS) theory is used to explain this assumption.

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Acknowledgements

The authors thank the National Natural Science Foundation of China (NSFC) (Nos. 11104106 and 10974067), the Science and Technology Planning Project of Jilin Province (Nos. 20101508, 201101037 and 201115033) and the China Postdoctoral Science Foundation (No. 20100481062) for financial support of this research.

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Authors and Affiliations

  1. State Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, 130012, China

    W. Fang & C. Sun

  2. College of Physics, Jilin University, Changchun, 130012, China

    W. Fang, Z. Li, G. Qu & Z. Men

  3. School of Science, Changchun University of Science and Technology, Changchun, 130022, China

    A. Cao

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  1. W. Fang
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  2. Z. Li
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  3. G. Qu
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Correspondence to Z. Men or C. Sun.

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Fang, W., Li, Z., Qu, G. et al. Enhanced stimulated Raman scattering by intermolecular Fermi resonance. Appl. Phys. B 107, 145–149 (2012). https://doi.org/10.1007/s00340-012-4894-z

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