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Toward single attosecond pulses using harmonic emission from solid-density plasmas


We report on investigations of high-order harmonic generation from solid surfaces in the coherent wake emission regime with relativistically intense few-cycle (8 fs) laser pulses. Significant spectral broadening compared to previous experiments with many-cycle pulses and the appearance of substructures on the harmonics are observed that strongly fluctuate from shot-to-shot. Measurements in which the linear polarization was rotated or ellipticity of the laser pulse was varied exhibit a strong dependence of the harmonic emission on the polarization state of the incident pulse. We show that the observed spectral features are ultimately connected to the sub-cycle electron dynamics in the laser-solid interaction and thus proof of the few-cycle nature of the observed harmonic emission. Using a simple model we have investigated the factors that play an important role in the shape of the emitted spectrum.

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  1. 1.

    Y. Nomura, R. Hörlein, P. Tzallas, B. Dromey, S. Rykovanov, Z. Major, J. Osterhoff, S. Karsch, L. Veisz, M. Zepf, D. Charalambidis, F. Krausz, G.D. Tsakiris, Nat. Phys. 5, 124 (2009)

    Article  Google Scholar 

  2. 2.

    R. Hörlein, Y. Nomura, P. Tzallas, S. Rykovanov, B. Dromey, J. Osterhoff, Z. Major, S. Karsch, L. Veisz, M. Zepf, D. Charalambidis, F. Krausz, G.D. Tsakiris, New J. Phys. 12, 043020 (2010)

    Article  Google Scholar 

  3. 3.

    R. Lichters, J. Meyer-ter Vehn, A. Pukhov, Phys. Plasmas 3, 3425 (1996)

    Article  ADS  Google Scholar 

  4. 4.

    T. Baeva, S. Gordienko, A. Pukhov, Phys. Rev. E 74, 046404 (2006)

    Article  ADS  Google Scholar 

  5. 5.

    Y.M. Mikhailova, V.T. Platonenko, S.G. Rykovanov, JETP Lett. 81, 571 (2005)

    Article  ADS  Google Scholar 

  6. 6.

    G.D. Tsakiris, K. Eidmann, J. Meyer-ter Vehn, F. Krausz, New J. Phys. 8, 19 (2006)

    Article  ADS  Google Scholar 

  7. 7.

    N.M. Naumova, C.P. Hauri, J.A. Nees, I.V. Sokolov, R. Lopez-Martens, G.A. Mourou, New J. Phys. 10, 025022 (2008)

    Article  ADS  Google Scholar 

  8. 8.

    U. Teubner, P. Gibbon, Rev. Mod. Phys. 81, 445 (2009)

    Article  ADS  Google Scholar 

  9. 9.

    F. Quéré, C. Thaury, P. Monot, S. Dobosz, P. Martin, J.-P. Geindre, P. Audebert, Phys. Rev. Lett. 96, 125004 (2006)

    Article  ADS  Google Scholar 

  10. 10.

    B. Dromey, M. Zepf, A. Gopal, K. Lancaster, M.S. Wei, K. Krushelnick, M. Tatarakis, N. Vakakis, S. Moustaizis, R. Kodama, M. Tampo, C. Stoeckl, R. Clarke, H. Habara, D. Neely, S. Karsch, P. Norreys, Nat. Phys. 2, 456 (2006)

    Article  Google Scholar 

  11. 11.

    B. Dromey, S. Kar, C. Bellei, D.C. Carroll, R.J. Clarke, J.S. Green, S. Kneip, K. Markey, S.R. Nagel, P.T. Simpson, L. Willingale, P. McKenna, D. Neely, Z. Najmudin, K. Krushelnick, P.A. Norreys, M. Zepf, Phys. Rev. Lett. 99, 085001 (2007)

    Article  ADS  Google Scholar 

  12. 12.

    A. Tarasevitch, K. Lobov, C. Wuensche, D. von der Linde, Phys. Rev. Lett. 98, 103902 (2007)

    Article  ADS  Google Scholar 

  13. 13.

    F. Quéré, C. Thaury, J.-P. Geindre, G. Bonnaud, P. Monot, P. Martin, Phys. Rev. Lett. 100, 095004 (2008)

    Article  ADS  Google Scholar 

  14. 14.

    C. Thaury, H. George, F. Quéré, R. Loch, J.-P. Geindre, P. Monot, P. Martin, Nat. Phys. 4, 631 (2008)

    Article  Google Scholar 

  15. 15.

    B. Dromey, D. Adams, R. Hörlein, Y. Nomura, S.G. Rykovanov, D.C. Caroll, P.S. Foster, S. Kar, K. Markey, P. McKenna, D. Neely, M. Geissler, G.D. Tsakiris, M. Zepf, Nat. Phys. 5, 146 (2009)

    Article  Google Scholar 

  16. 16.

    M. Hentschel, R. Kienberger, C. Spielmann, G.A. Reider, N. Milosevic, T. Brabec, P. Corkum, U. Heinzmann, M. Drescher, F. Krausz, Nature 414, 509 (2001)

    Article  ADS  Google Scholar 

  17. 17.

    F. Krausz, M. Ivanov, Rev. Mod. Phys. 81, 163 (2009)

    Article  ADS  Google Scholar 

  18. 18.

    P. Tzallas, E. Skantzakis, E.P. Benis, G.D. Tsakiris, D. Charalambidis, Nat. Phys. 3, 846 (2007)

    Article  Google Scholar 

  19. 19.

    T. Baeva, S. Gordienko, A. Pukhov, Phys. Rev. E 74, 065401 (2006)

    Article  ADS  Google Scholar 

  20. 20.

    S. Rykovanov, M. Geissler, J. Meyer-ter Vehn, G.D. Tsakiris, New J. Phys. 10, 025025 (2008)

    Article  ADS  Google Scholar 

  21. 21.

    A. Baltuska, M. Uiberacker, E. Goulielmakis, R. Kienberger, V.S. Yakovlev, T. Udem, T.W. Hänsch, F. Krausz, IEEE J. Sel. Top. Quantum Electron. 9, 972 (2003)

    Article  Google Scholar 

  22. 22.

    F. Tavella, Y. Nomura, L. Veisz, V. Pervak, A. Marcinkevicius, F. Krausz, Opt. Lett. 32, 2227 (2007)

    Article  ADS  Google Scholar 

  23. 23.

    D. Herrmann, L. Veisz, R. Tautz, F. Tavella, K. Schmid, V. Pervak, F. Krausz, Opt. Lett. 34, 2459 (2009)

    Article  ADS  Google Scholar 

  24. 24.

    C. Thaury, F. Quéré, J.-P. Geindre, A. Levy, T. Ceccotti, P. Monot, M. Bougeard, F. Réau, P. d’Oliveira, P. Audebert, R. Marjoribanks, P. Martin, Nat. Phys. 3, 424 (2007)

    Article  Google Scholar 

  25. 25.

    P. Gibbon, Phys. Rev. Lett. 76, 50 (1996)

    Article  ADS  Google Scholar 

  26. 26.

    K. Gál, S. Varró, Opt. Commun. 198, 419 (2001)

    Article  ADS  Google Scholar 

  27. 27.

    L.A. Gizzi, D. Giulietti, A. Giulietti, P. Audebert, S. Bastiani, J.P. Geindre, A. Mysyrowicz, Phys. Rev. Lett. 76, 2278 (1996)

    Article  ADS  Google Scholar 

  28. 28.

    E. Rácz, I.B. Földes, G. Kocsis, G. Veres, K. Eidmann, S. Szatmári, Appl. Phys. B, Lasers Opt. 82, 13 (2006)

    Article  ADS  Google Scholar 

  29. 29.

    P.A. Norreys, M. Zepf, S. Moustaizis, A.P. Fews, J. Zhang, P. Lee, M. Bakarezos, C.N. Danson, A. Dyson, P. Gibbon, P. Loukakos, D. Neely, F.N. Walsh, J.S. Wark, A.E. Dangor, Phys. Rev. Lett. 76, 1832 (1996)

    Article  ADS  Google Scholar 

  30. 30.

    G. Veres, J.S. Bakos, I.B. Földes, K. Gál, Z. Juhász, G. Kocsis, S. Szatmári, Europhys. Lett. 48, 390 (1999)

    Article  ADS  Google Scholar 

  31. 31.

    R.A. Ganeev, A. Ishizawa, T. Kanai, T. Ozaki, H. Kuroda, Opt. Commun. 227, 175 (2003)

    Article  ADS  Google Scholar 

  32. 32.

    P.B. Corkum, Phys. Rev. Lett. 71, 1994 (1993)

    Article  ADS  Google Scholar 

  33. 33.

    F. Brunel, Phys. Rev. Lett. 59, 52 (1987)

    Article  ADS  Google Scholar 

  34. 34.

    Z.-M. Sheng, K. Mima, J. Zhang, H. Sanuki, Phys. Rev. Lett. 94, 095003 (2005)

    Article  ADS  Google Scholar 

  35. 35.

    F. Brandl, B. Hidding, J. Osterholz, D. Hemmers, A. Karmakar, A. Pukhov, G. Pretzler, Phys. Rev. Lett. 102, 195001 (2009)

    Article  ADS  Google Scholar 

  36. 36.

    M. Cerchez, R. Jung, J. Osterholz, T. Toncian, O. Willi, Phys. Rev. Lett. 100, 245001 (2008)

    Article  ADS  Google Scholar 

  37. 37.

    B. Dromey, S.G. Rykovanov, D. Adams, R. Hörlein, Y. Nomura, D.C. Caroll, P.S. Foster, S. Kar, K. Markey, P. McKenna, D. Neely, M. Geissler, G.D. Tsakiris, M. Zepf, Phys. Rev. Lett. 102, 225002 (2009)

    Article  ADS  Google Scholar 

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Correspondence to P. Heissler.

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Heissler, P., Hörlein, R., Stafe, M. et al. Toward single attosecond pulses using harmonic emission from solid-density plasmas. Appl. Phys. B 101, 511–521 (2010).

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  • Laser Pulse
  • Harmonic Spectrum
  • Attosecond Pulse
  • Harmonic Emission
  • Driving Pulse