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Ultrafast dynamics of surface plasmon polaritons in plasmonic metamaterials

Applied Physics B volume 84, pages 183–189 (2006)Cite this article

Abstract

Using near-field scanning optical microscopy and ultrafast laser spectroscopy, we study the linear optical properties of subwavelength nanoslit and nanohole arrays in metal films, which are prototype structures for novel plasmonic metamaterials. Near-field microscopy provides direct evidence for surface plasmon polariton (SPP) excitation and allows for spatial imaging of the corresponding SPP modes. By employing spectral interferometry with ultrashort 11-fs light pulses, we directly reconstruct the temporal structure of the electric field of these pulses as they are transmitted through the metallic nanostructures. The analysis of these data allows for a quantitative extraction of the plasmonic band structure and the radiative damping of the corresponding SPP modes. Clear evidence for plasmonic band gap formation is given. Our results reveal that the coherent coupling between different SPP modes can result in a pronounced suppression of radiative SPP damping, increasing the SPP lifetime from 30 fs to more than 200 fs. These findings are relevant for optimizing and manipulating the optical properties of novel nano-plasmonic devices.

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References

  1. W.L. Barnes, A. Dereux, T.W. Ebbesen, Nature 424, 824 (2003)

    Article  ADS  Google Scholar 

  2. S.A. Maier, P.G. Kik, J.A. Atwater, S. Meltzer, E. Habel, B.E. Koel, A.A.G. Requicha, Nature Mater. 2, 229 (2003)

    Article  ADS  Google Scholar 

  3. H.J. Lezec, A. Degion, E. Deveaux, R.A. Linke, L. Martin-Moreno, F.J. Garcia-Vidal, T.W. Ebbesen, Science 297, 820 (2002)

    Article  ADS  Google Scholar 

  4. T.W. Ebbesen, H.J. Lezec, H.F. Ghaemi, T. Thio, P.A. Wolff, Nature 391, 667 (1998)

    Article  ADS  Google Scholar 

  5. J.B. Pendry, Phys. Rev. Lett. 85, 3966 (2000)

    Article  ADS  Google Scholar 

  6. D.S. Kim, S.C. Hohng, V. Malyarchuk, Y.C. Yoon, Y.H. Ahn, K.J. Yee, J.W. Park, J. Kim, Q.H. Park, C. Lienau, Phys. Rev. Lett. 91, 143901 (2003)

    Article  ADS  Google Scholar 

  7. A. Dogariu, T. Thio, L.J. Wang, T.W. Ebbesen, H.J. Lezec, Opt. Lett. 26, 450 (2001)

    Article  ADS  Google Scholar 

  8. A. Dogariu, A. Nahata, R. Linke, L. Wang, R. Trebino, Appl. Phys. B 74, 69 (2002)

    Article  ADS  Google Scholar 

  9. S.C. Hohng, Y.C. Yoon, D.S. Kim, V. Malyarchuk, R. Müller, C. Lienau, J.W. Park, K.H. Yoo, J. Kim, H.Y. Ryu, Q.H. Park, Appl. Phys. Lett. 81, 3239 (2002)

    Article  ADS  Google Scholar 

  10. C. Ropers, D.J. Park, G. Stibenz, G. Steinmeyer, J. Kim, D.S. Kim, C. Lienau, Phys. Rev. Lett. 94, 113901 (2005)

    Article  ADS  Google Scholar 

  11. R.H. Dicke, Phys. Rev. 93, 99 (1954)

    Article  ADS  Google Scholar 

  12. C. Iaconis, I.A. Walmsley, Opt. Lett. 23, 792 (1998)

    Article  ADS  Google Scholar 

  13. G. Stibenz, G. Steinmeyer, Opt. Express 12, 6319 (2004)

    Article  ADS  Google Scholar 

  14. J.-C. Diels, W. Rudolph, Ultrashort Laser Pulse Phenomena (Academic Press, San Diego, CA, 1996)

  15. F. Reynaud, F. Salin, A. Berthelemy, Opt. Lett. 14, 275 (1989)

    Article  ADS  Google Scholar 

  16. L. Lepetit, G. Cheriaux, M. Joffre, J. Opt. Soc. Am. B 12, 2467 (1995)

    Article  ADS  Google Scholar 

  17. H.F. Ghaemi, T. Thio, D.E. Grupp, T.W. Ebbesen, H.J. Lezec, Phys. Rev. B 58, 6779 (1998)

    Article  ADS  Google Scholar 

  18. A. Porto, F.J. Garcia-Valid, J.B. Pendry, Phys. Rev. Lett. 83, 2845 (1999)

    Article  ADS  Google Scholar 

  19. L. Salomon, F. Grillot, A.V. Zayats, F. de Fornel, Phys. Rev. Lett. 86, 1110 (2001)

    Article  ADS  Google Scholar 

  20. L. Martin-Moreno, F.J. Garcia-Vidal, H.J. Lezec, K.M. Pellerin, T. Thio, J.B. Pendry, T.W. Ebbesen, Phys. Rev. Lett. 86, 1114 (2001)

    Article  ADS  Google Scholar 

  21. Q. Cao, P. Lalanne, Phys. Rev. Lett. 88, 075403 (2002)

    Google Scholar 

  22. K.G. Lee, Q-Han Park, Phys. Rev. Lett. 95, 103902 (2005)

    Article  ADS  Google Scholar 

  23. H. Räther, Surface Plasmons (Springer, Berlin, 1988)

    Google Scholar 

  24. T. Thio, H.F. Ghaemi, H.J. Lezec, P.A. Wolff, T.W. Ebbesen, J. Opt. Soc. Am. B 16, 1743 (1999)

    Article  ADS  Google Scholar 

  25. A. Taflove, S.C. Hagness, Computational Electrodynamics. The Finite-Difference Time-Domain Method (Artech House, Boston, 2000)

    MATH  Google Scholar 

  26. R. Müller, V. Malyarchuk, C. Lienau, Phys. Rev. B 68, 205415 (2003)

    Article  ADS  Google Scholar 

  27. R. Müller, C. Ropers, C. Lienau, Opt. Express 12, 5067 (2004)

    Article  ADS  Google Scholar 

  28. H. Bethe, Phys. Rev. 66, 163 (1944)

    Article  ADS  MathSciNet  Google Scholar 

  29. C.W. Bouwkamp, Philips Res. Rep. 5, 321 (1950)

    Google Scholar 

  30. A. Bouhelier, M. Beversluis, A. Hartschuh, L. Novotny, Phys. Rev. Lett. 90, 013903 (2003)

    Article  ADS  Google Scholar 

  31. S. Linden, N. Rau, U. Neuberth, A. Naber, M. Wegener, S. Pereira, K. Busch, A. Christ, J. Kuhl, Phys. Rev. B 71, 245119 (2005)

    Article  ADS  Google Scholar 

  32. M.V. Berry, S. Klein, J. Mod. Opt. 43, 2139 (1996)

    Article  ADS  Google Scholar 

  33. J.-C. Diels, E.V. Stryland, G. Benedict, Opt. Commun. 25, 93 (1978)

    Article  ADS  Google Scholar 

  34. B. Lamprecht, J.R. Krenn, A. Leitner, F.R. Aussenegg, Phys. Rev. Lett. 83, 4421 (1999)

    Article  ADS  Google Scholar 

  35. J.H. Chung, A.M. Weiner, IEEE J. Sel. Top. Quantum Electron. 7, 656 (2001)

    Article  ADS  Google Scholar 

  36. G. Stibenz, G. Steinmeyer, Opt. Express 13, 2617 (2005)

    Article  ADS  Google Scholar 

  37. M. Sarrazin, J.-P. Vigneron, J.-M. Vigoureux, Phys. Rev. B 67, 085415 (2003)

    Article  ADS  Google Scholar 

  38. C. Genet, M.P. van Exter, J.P. Woerdman, Opt. Commun. 225, 331 (2003)

    Article  ADS  Google Scholar 

  39. S.G. Tikhodeev, A.L. Yablonskii, E.A. Muljarov, N.A. Gippius, T. Ishihara, Phys. Rev. B 66, 045102 (2002)

    Article  ADS  Google Scholar 

  40. S.G. Johnson, M. Ibanescu, M.A. Skorobogatiy, O. Weisberg, J.D. Joannopoulos, Y. Fink, Phys. Rev. E 65, 066611 (2002)

    Article  ADS  MathSciNet  Google Scholar 

  41. R.G. DeVoe, R.G. Brewer, Phys. Rev. Lett. 76, 2049 (1996)

    Article  ADS  Google Scholar 

  42. U. Akram, Z. Ficek, S. Swain, Phys. Rev. A 62, 013413 (2000)

    Article  ADS  Google Scholar 

  43. J.W. Lee, M.A. Seo, D.S. Kim, S.C. Jeoung, C. Lienau, J.H. Kang, Q.H. Park, Appl. Phys. Lett. 88, 071114 (2006)

    Article  ADS  Google Scholar 

  44. F. Yang, J.R. Sambles, Phys. Rev. Lett. 83, 2845 (1999)

    Article  Google Scholar 

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Authors and Affiliations

  1. Max-Born-Institut für Nichtlineare Optik und Kurzzeitspektroskopie, Max-Born-Strasse 2A, 12489, Berlin, Germany

    C. Ropers, G. Stibenz, G. Steinmeyer, R. Müller & C. Lienau

  2. School of Physics, Seoul National University, Seoul, 151-742, Korea

    D.J. Park, K.G. Lee, J.E. Kihm & D.S. Kim

  3. Korea Research Institute of Standards and Science, Yusung, Taejon, 305-600, Korea

    J. Kim

  4. Department of Physics, Korea University, Seoul, 136-701, Korea

    Q.H. Park

Authors
  1. C. Ropers
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  2. G. Stibenz
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  3. G. Steinmeyer
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  4. R. Müller
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  5. D.J. Park
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  6. K.G. Lee
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  7. J.E. Kihm
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  8. J. Kim
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  9. Q.H. Park
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  10. D.S. Kim
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  11. C. Lienau
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Correspondence to C. Lienau.

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PACS

42.70.Qs; 07.79.Fc; 42.25.-p

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Ropers, C., Stibenz, G., Steinmeyer, G. et al. Ultrafast dynamics of surface plasmon polaritons in plasmonic metamaterials. Appl. Phys. B 84, 183–189 (2006). https://doi.org/10.1007/s00340-006-2191-4

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  • DOI: https://doi.org/10.1007/s00340-006-2191-4