Abstract
Multiple bending can have detrimental effect on the performance of the microwave absorber as it may cause fractures and fatigues in the materials it is composed off. Consistency in absorption performance requires performance revertibility along with flexibility. Hydrogels with semi-liquid behavior are found to exhibit reversibility. Herein, meta-structure-based revertible absorbers have been proposed using PVA–borate cross-linked hydrogel popularly known as slime embedded in silicone rubber. Resonators are shaped into cuboidal and hexagonal–prism structures. Dual resonating structure technique has been employed to achieve a wide – 10 dB absorption bandwidth almost covering the entire X-band. The hydrogel with dielectric properties close to water assists in more than 90% absorption over the whole operating band. Simulation shows that the structures are bendable up to a bending radius of 10 mm without compromising on the absorption bandwidth. The self-healing property of slime further aids revertibility of the developed MSAs. Performance restoration is observed after 24 h of continuous application of deformation force for maximum bending. The absorption mechanism in the MSAs are discussed by vector field distribution. Polarization insensitive absorption is found over \(\pm 90^\circ\).
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References
H. Wang, J. Lu, H. Huang, S. Fang, M. Zubair, Z. Peng, A highly elastic, room-temperature repairable and recyclable conductive hydrogel for stretchable electronics. J. Colloid Interface Sci. 588, 295–304 (2021)
B. Ying, X. Liu, Skin-like hydrogel devices for wearable sensing, soft robotics and beyond. Iscience 24(11), 103174 (2021)
T. Qin, W. Liao, L. Yu, J. Zhu, M. Wu, Q. Peng, L. Han, H. Zeng, Recent progress in conductive self-healing hydrogels for flexible sensors. J. Polym. Sci. 60(18), 2607–2634 (2022)
K. Chen, K. Liang, H. Liu, R. Liu, Y. Liu, S. Zeng, Y. Tian, Skin-inspired ultra-tough supramolecular multifunctional hydrogel electronic skin for human–machine interaction. Nano Micro Lett 15(1), 102 (2023)
H. Zhang, A. Kalra, A. Lowe, Y. Yu, G. Anand, A hydrogel-based electronic skin for touch detection using electrical impedance tomography. Sensors 23(3), 1571 (2023)
E.M. Ahmed, Hydrogel: preparation, characterization, and applications: a review. J. Adv. Res. 6(2), 105–121 (2015)
M. Bahram, N. Mohseni, M. Moghtader, An introduction to hydrogels and some recent applications, in Emerging Concepts in Analysis and Applications of Hydrogels, ed. by S.B. Majee (IntechOpen, 2016). https://doi.org/10.5772/61692
Y. Guo, J. Bae, Z. Fang, P. Li, F. Zhao, G. Yu, Hydrogels and hydrogel-derived materials for energy and water sustainability. Chem. Rev. 120(15), 7642–7707 (2020)
D.J. Gogoi, N.S. Bhattacharyya, Embedded dielectric water “atom” array for broadband microwave absorber based on Mie resonance. J. Appl. Phys. 122(17), 175106 (2017)
Y. Huang, X. Yuan, M. Chen, W.-L. Song, J. Chen, Q. Fan, L. Tang, D. Fang, Ultrathin flexible carbon fiber reinforced hierarchical metastructure for broadband microwave absorption with nano lossy composite and multiscale optimization. ACS Appl. Mater. Interfaces 10(51), 44731–44740 (2018)
Y. Duan, Q. Liang, Z. Yang, Z. Li, H. Yin, Y. Cao, D. Li, A wide-angle broadband electromagnetic absorbing metastructure using 3D printing technology. Mater. Des. 208, 109900 (2021)
M. Abdullahi, M. Ali, Additively manufactured metastructure design for broadband radar absorption. Beni-Suef Univ. J. Basic Appl. Sci. 10(1), 1–12 (2021)
S. Saikia, N.S. Bhattacharyya, Slime based meta-structure absorber for X-band applications, in 2022 URSI Regional Conference on Radio Science (USRI-RCRS) (IEEE, New York City, 2022), pp. 1–4
D. Li, W. Pan, T. Wang, X. Wang, R. Gong, 3D printed lightweight metastructure with microwave absorption and mechanical resistance. Mater. Des. 225, 111506 (2023)
A. Valipour, M.H. Kargozarfard, M. Rakhshi, A. Yaghootian, H.M. Sedighi, Metamaterials and their applications: an overview. Proc. Inst. Mech. Eng. Part L: J. Mater.: Des. Appl. 236(11), 2171–2210 (2022)
S. Saikia, N.S. Bhattacharyya, An X-band meta-structure absorber based on gelated deep eutectic solvent. J. Appl. Phys. 131(22), 224901 (2022)
S. Saikia, N.S. Bhattacharyya, Polarization independent meta-structure absorber using array of embedded gelated deep eutectic solvent for X-band applications, in 2022 IEEE Microwaves, Antennas, and Propagation Conference (MAPCON) (IEEE, New York City, 2022), pp. 1689–1693
D.J. Gogoi, N.S. Bhattacharyya, Metasurface absorber based on water meta “molecule” for X-band microwave absorption. J. Appl. Phys. 124(7), 075106 (2018)
M. Amin, M. Akbar, S. Amin, Hydrophobicity of silicone rubber used for outdoor insulation (an overview). Rev. Adv. Mater. Sci. 16(1–2), 10–26 (2007)
L. Feng, S. Li, S. Feng, Preparation and characterization of silicone rubber with high modulus via tension spring-type crosslinking. RSC Adv. 7(22), 13130–13137 (2017)
N.I. Landy, S. Sajuyigbe, J.J. Mock, D.R. Smith, W.J. Padilla, Perfect metamaterial absorber. Phys. Rev. Lett. 100(20), 207402 (2008)
E.J. Rothwell, J.L. Frasch, S.M. Ellison, P. Chahal, R.O. Ouedraogo, Analysis of the Nicolson–Ross–Weir method for characterizing the electromagnetic properties of engineered materials. Prog. Electromagn. Res. 157, 31–47 (2016)
D. Zhou, X. Huang, Z. Du, Analysis and design of multilayered broadband radar absorbing metamaterial using the 3-D printing technology-based method. IEEE Antennas Wirel. Propag. Lett. 16, 133–136 (2016)
W.-L. Song, Z. Zhou, L.-C. Wang, X.-D. Cheng, M. Chen, R. He, H. Chen, Y. Yang, D. Fang, Constructing repairable meta-structures of ultra-broad-band electromagnetic absorption from three-dimensional printed patterned shells. ACS Appl. Mater. Interfaces 9(49), 43179–43187 (2017)
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All authors contributed to the study. Design and fabrication are performed by SS and HS. Data analysis is done by SS and supervised by Dr. NSB. The manuscript is drafted by SS and HS. Dr. NSB provided critical revision of the manuscript. All authors read and approved the final manuscript.
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Saikia, S., Saikia, H. & Bhattacharyya, N.S. Revertible wideband hydrogel-based meta-structure absorber. Appl. Phys. A 130, 189 (2024). https://doi.org/10.1007/s00339-024-07339-4
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DOI: https://doi.org/10.1007/s00339-024-07339-4