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Enhancing magnetic properties of Ni3Si/Fe3O4@PVDF composites via lamellar Ni3Si template fabrication under pulsed magnetic fields

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Abstract

This study introduces a novel Ni3Si/Fe3O4@polyvinylidene fluoride (PVDF) composite, which is fabricated using a lamellar Ni3Si template under pulsed magnetic fields. The results reveal that increasing the content of Fe3O4 nanoparticles (NPs) enhances the densification of Fe3O4@PVDF slurries within the Ni3Si template. Interestingly, the ferromagnetic behavior of the Ni3Si/Fe3O4@PVDF composites shows an opposite trend to that of the Fe3O4@PVDF slurry as the magnetic flux density peak (MP) increases. Specifically, the maximum magnetization (Mmax) values achieved are 2.99 × 10–2, 2.79 × 10–2, 2.36 × 10–2, and 2.02 × 10–2 emu/g at MP values of 0, 4.5, 5.7, and 8.9 T, respectively. The influence of magnetic fields becomes more pronounced with higher Fe3O4 NPs content. However, when the Fe3O4 NPs content reaches 9.1% and the MP is 8.9 T, the uncertainty regarding the actual content of Fe3O4 NPs filled into the Ni3Si template poses challenges for the regulation of magnetic properties. Therefore, a lower Fe3O4 NPs content is more advantageous for controlling the magnetic properties of Ni3Si/Fe3O4@PVDF composites.

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Acknowledgements

Authors acknowledge the financial support from the Natural Science Foundation of Henan Province (No. 232300421321) and Natural Science Basic Research Program of Shaanxi (No. 2021JZ-10).

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Authors and Affiliations

  1. School of Mechanical and Power Engineering, Zhengzhou University, Science Road 100, Zhengzhou, 450001, China

    Kai Cui, Yuan Cao, Yichuan Yang & Genghuan Song

  2. School of Mechanical Engineering, Northwestern Polytechnical University, Youyi West Road 127, Xi’an, 710072, China

    Zhilong Zhao

  3. School of Management Engineering, Zhengzhou University of Aeronautics, Wenyuan West Road 15, Zhengzhou, 450046, China

    Hongli Lin

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  1. Kai Cui
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Contributions

KC: conceptualization, methodology, supervision, writing-original draft preparation. YC, YY and GS: visualization, investigation, validation. ZZ: writing—review and editing, funding acquisition, HL: writing—review and editing, supervision.

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Correspondence to Kai Cui.

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Cui, K., Cao, Y., Yang, Y. et al. Enhancing magnetic properties of Ni3Si/Fe3O4@PVDF composites via lamellar Ni3Si template fabrication under pulsed magnetic fields. Appl. Phys. A 129, 729 (2023). https://doi.org/10.1007/s00339-023-07018-w

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