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Bi(Li1/2Nb1/2)O3 addition inducing improved energy storage performance in lead-free BCZT ceramics

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Abstract

BCZT ceramics are considered to be a promising material due to the presence of its morphotropic phase boundary (MPB). However, most of the research on this material is focused on piezoelectric properties, and there is still a lack of research on energy storage properties. Here, a component represented as BiMeO3 [Me = (Li1/2Nb1/2)3+] with a similar structure as BCZT was introduced into ceramics to improve the energy storage properties. The phase composition changes, relaxation behavior, and energy storage properties of the samples were carefully investigated. The improved relative densities brought about by the introduction facilitate the increase in bulk resistance, thus increasing the break-down field strength. Due to the addition of BLN, the Curie temperature drops substantially below room temperature. Under the influence of phase composition and polar nano-regions (PNRs), BCZT ceramics exhibit slim hysteresis loops. In BCZT‒0.12BLN, the recoverable energy density can reach 2.06 J/cm3 and efficiency can stay in 80.5% at the same time. This proposed BCZT ceramic still has great research potential as an energy storage material.

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Data can be available from the corresponding author upon academic reasonable request.

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Acknowledgements

This work was supported by the Key Scientific Research Projects of Colleges and Universities in Henan Province (21A140014 and 21B140005) and the Young Backbone Teachers Training Plan of Colleges and Universities in Henan Province (2020GGJS060 and 2020GGJS062).

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Authors and Affiliations

  1. National Demonstration Center for Experimental Physics Education, School of Physics, Henan Normal University, and Henan Key Laboratory of Photovoltaic Materials, Xinxiang, 453007, People’s Republic of China

    Y. C. Hu, S. T. Dang, J. Q. Cao, W. L. Zhang, Y. J. Zai, P. S. Xu & X. W. Wang

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  1. Y. C. Hu
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Contributions

All authors have contributed to the study. Resources, funding acquisition, and project administration are provided by YH. Material preparation was performed by SD, WZ, YZ, and PX. Data collection and analysis were completed by SD and JC. The first draft of the manuscript was written by SD. Review and editing was completed by XW and YH. All authors commented on previous versions of the manuscript and read and approved the final manuscript.

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Correspondence to Y. C. Hu or X. W. Wang.

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Hu, Y.C., Dang, S.T., Cao, J.Q. et al. Bi(Li1/2Nb1/2)O3 addition inducing improved energy storage performance in lead-free BCZT ceramics. Appl. Phys. A 129, 602 (2023). https://doi.org/10.1007/s00339-023-06879-5

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