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Enhanced energy storage performance of KNN-BLZS dielectric ceramic

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Abstract

Exploring high-performance energy storage dielectric ceramics for pulse power applications is paramount concern for a multitude of researchers. In this work, a (1 – x)K0.5Na0.5NbO3-xBi0.5La0.5(Zn0.5Sn0.5)O3 ((1–x)KNN-xBLZS) lead-free relaxor ceramic was successfully synthesized by a conventional solid-reaction method. X-ray diffraction and Raman spectra confirm the perovskite structure of the ceramics. With the addition of BLZS, the crystal growth is suppressed, the ceramic resistivity increases, and the relaxation properties of ceramics are enhanced. By optimizing the composition to x = 0.12, we achieved a significant ΔP of 12.8 μC/cm2, a Pmax of 14.6 μC/cm2, and a Pr of 1.8 μC/cm2. The resulting Wrec reached 0.84 J/cm3, accompanied by an outstanding efficiency (η) of 76%, superior frequency reliability, and robust thermal stability. Owing to these exceptional properties, the 0.88 KNN-0.12 BLZS ceramic demonstrates great potential for pulse power applications.

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Acknowledgements

This work was supported by the Guizhou Provincial Science and Technology Foundation (ZK [2022] General 112), and the National Natural Science Foundation of China (No. 42267009). We also thank Prof. Wu at Sichuan University for the valuable suggestions.

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Authors and Affiliations

  1. College of Materials and Metallurgy, Guizhou University, Guizhou, 550025, China

    Jizhong Deng, Yuesong Li, Ya Yang, Ronglian Li & Yuanyu Wang

  2. Geol Team 105, Guizhou Bur Geol & Mineral Explorat & Dev, Guizhou, 550018, China

    Ping Zhao

Authors
  1. Jizhong Deng
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  2. Yuesong Li
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  3. Ya Yang
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  4. Ronglian Li
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  5. Ping Zhao
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  6. Yuanyu Wang
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Contributions

All authors contributed to the study conception and design. Material preparation, data collection and analysis were performed by JZD, YSL, YY, RLL and PZ. The first draft of the manuscript was written by JZD and YSL and all authors commented on previous versions of the manuscript. All authors read and approved the final manuscript.

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Correspondence to Yuanyu Wang.

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Deng, J., Li, Y., Yang, Y. et al. Enhanced energy storage performance of KNN-BLZS dielectric ceramic. Appl. Phys. A 129, 508 (2023). https://doi.org/10.1007/s00339-023-06795-8

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