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Synthesis of Ag/Co nanoparticles by dual pulsed laser ablation for synergistic photothermal study

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Abstract

Magneto-plasmonic nanoparticles have gained increasing interest, especially for the synergistic response study of hyperthermia applications. However, some challenges, including the synthesis process, dose optimization of laser, and magnetic field strength besides its frequency, need significant attention. Herein, we prepared magneto-plasmonic Ag/Co nanomaterials for photothermal performance evaluation using dual-beam of the Q-switched Nd:YAG 1064 nm pulsed laser ablation in distilled water, which can avoid any additive, contaminations, complicated route, and multiple purifications processes as they may occur in chemical synthesis processes. Properties, morphologies, and compositions of synthesized nanomaterials were studied, and results suggested that the main constituents of NPs were Ag/Co. The detailed theoretical calculation of the photothermal performance of nanofluid is described, along with an experimental study of nanofluid and the water as a reference medium using NIR 808 nm laser. The overall results suggest that the higher temperatures for Ag/Co nanofluid compared with water alone were recorded as 16.5 °C, 20.9 °C, 24.7 °C, 24.5 °C, 27.7 °C, and 30.2 °C during 808 nm laser irradiation operating at different corresponding powers, respectively. The possible reason for the higher temperature profiles and the rapid temperature rise of nanofluid than water alone is the localized surface plasmon effects of nanoparticles. These results evidence that silver and cobalt nanomaterials composite structures could significantly increase hyperthermia based on an effective and simple synthesis approach.

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Acknowledgements

Imran Ali and Yunxiang Pan contributed equally to this work. This work was financially supported by the Fundamental Research Funds for the Central Universities (No.30919011253, No.30918011335), National Natural Science Foundation of China (No.61975080, No.61805120), Natural Science Foundation of Jiangsu Province (BK20181296), Large Equipment Open Fund from Nanjing University of Science and Technology. Yasir Jamil is thankful to the Higher Education Commission of Pakistan for financial support under project No NRPU-6409.

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Authors and Affiliations

  1. School of Science, Nanjing University of Science and Technology, Nanjing, 210094, China

    Imran Ali, Yunxiang Pan, Jinning Hu & Zhonghua Shen

  2. Key Laboratory of Optoelectronic Technology of Jiangsu Province, Center for Quantum Transport and Thermal Energy Science, School of Physics and Technology, Nanjing Normal University, Nanjing, 210023, China

    Yawen Lin & Zhixing Gan

  3. Laser Spectroscopy Lab, Department of Physics, University of Agriculture, Faisalabad, Pakistan

    Yasir Jamil

  4. Institute of Optoelectronics Nanomaterials, MIIT Key Laboratory of Advanced Display Materials and Devices, College of Materials Science and Engineering, Nanjing University of Science and Technology, Nanjing, 210094, China

    Jun Chen

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Ali, I., Pan, Y., Lin, Y. et al. Synthesis of Ag/Co nanoparticles by dual pulsed laser ablation for synergistic photothermal study. Appl. Phys. A 127, 632 (2021). https://doi.org/10.1007/s00339-021-04706-3

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