Abstract
Time-resolved optical studies using spectral interferometry and reflectance measurements of ultrafast laser excitation of quartz have been performed and combined with subsequent atomic force microscopy imaging of the laser-formed holes. A comprehensive investigation of these transient properties of the dielectric has been analysed in view of a single theoretical model describing the laser–material interaction in a multirate equation model including light propagation. Simulations demonstrate that self-trapped excitons in quartz significantly change the optical properties immediately after excitation.
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Acknowledgments
This work was supported by The Danish Council for Independent Research | Natural Sciences (FNU) and Laserlab Europe (Transnational Acces).
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Haahr-Lillevang, L., Wædegaard, K., Sandkamm, D.B. et al. Short-pulse laser excitation of quartz: experiments and modelling of transient optical properties and ablation. Appl. Phys. A 120, 1221–1227 (2015). https://doi.org/10.1007/s00339-015-9307-9
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DOI: https://doi.org/10.1007/s00339-015-9307-9