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Non-monotonic dependence of temperature of Au nanometer films dissociation into droplets on their thickness on Al2O3 surface

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Abstract

The process of melting with consequent disintegration into droplets of various thickness Au thin films has been studied. An unexpected character of the melting–disintegration temperature dependence on thin-film thickness has been found: a reduction of the process temperature has been observed with thickness in the range from 100 to 20 nm; however, the disintegration temperature starts to increase for Au film thicknesses lower than 20 nm. It is supposed that the observed non-monotonic behavior of the process temperature is caused by the influence of the substrate interaction with the film, resulting in an entropy change of the system.

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References

  1. M.L. Gimpl, A.D. McMaster, N. Fuschillo, J. Appl. Phys. 35, 3572 (1964)

    Article  ADS  Google Scholar 

  2. L. Bachmann, D.L. Sawyer, B.M. Siegel, J. Appl. Phys. 36, 304 (1965)

    Article  ADS  Google Scholar 

  3. A.E.B. Presland, G.L. Price, D.L. Trimm, Surf. Sci. 29, 435 (1972)

    Article  ADS  Google Scholar 

  4. C.M. Kennefick, R. Raj, Acta Metall. 37, 2947 (1989)

    Article  Google Scholar 

  5. E. Jiran, C.V. Thompson, J. Electron. Mater. 19, 1153 (1990)

    Article  ADS  Google Scholar 

  6. E. Jiran, C.V. Thompson, Thin Solid Films 208, 23 (1992)

    Article  ADS  Google Scholar 

  7. I. Beszeda, I.A. Szabo, E.G. Gontier-Moya, Appl. Phys. A 78, 1079 (2004)

    Article  ADS  Google Scholar 

  8. Y.F. Komnik, Fizika Metallicheskikh Plenok: Razmernie i Structurnie Effecti (Physics of Metallic Films: Size and Structural Effects) (Atomizdat, Moscow, 1979) (in Russian)

    Google Scholar 

  9. A.I. Gusev, A.A. Rempel, Nanocrystalline Materials (Fizmatlit/Cambridge International Science, Moscow/Cambridge, 2001/2004)

    Google Scholar 

  10. Y.E. Geguzin, Physics of Sintering (Nauka, Moscow, 1984) (in Russian)

    Google Scholar 

  11. U. Tartaglino, T. Zykova-Timan, F. Ercolessi, E. Tosatti, Phys. Rep. 411, 291 (2005)

    Article  ADS  Google Scholar 

  12. D.G. Gromov, S.A. Gavrilov, E.N. Redichev, Russ. J. Phys. Chem. 79, 1578 (2005)

    Google Scholar 

  13. D.G. Gromov, S.A. Gavrilov, E.N. Redichev, A.V. Klimovitskaya, R.M. Ammosov, Russ. J. Phys. Chem. 80, 1650 (2006)

    Article  Google Scholar 

  14. D.G. Gromov, S.A. Gavrilov, E.N. Redichev, R.M. Ammosov, Phys. Solid State 49, 178 (2007)

    Article  ADS  Google Scholar 

  15. S. Kodambaka, J.B. Hannon, R.M. Tromp, F.M. Ross, Nano Lett. 6, 1292 (2006)

    Article  ADS  Google Scholar 

  16. J. Albuschies, M. Baus, O. Winkler, B. Hadam, B. Spangenberg, H. Kurz, Microelectron. Eng. 83, 1530 (2006)

    Article  Google Scholar 

  17. S. Kodambaka, J. Tersoff, M.C. Reuter, K.B. Reuter, F.M. Ross, Microsc. Microanal. 13, 716 (2007)

    Article  Google Scholar 

  18. S.T. Boles, C.V. Thompson, E.A. Fitzgerald, J. Cryst. Growth 311, 1446 (2009)

    Article  ADS  Google Scholar 

  19. S.A. Dayeh, E.T. Yu, D. Wang, J. Phys. Chem. C 111, 13331 (2007)

    Article  Google Scholar 

  20. J.H. Kim, H.H. An, H.J. Woo, C.S. Yoon, Nanotechnology 19, 125604 (2008)

    Article  ADS  Google Scholar 

  21. D.G. Gromov, S.A. Gavrilov, Phys. Solid State 51, 2135 (2009)

    Article  ADS  Google Scholar 

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Correspondence to D. G. Gromov.

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Gromov, D.G., Gavrilov, S.A., Redichev, E.N. et al. Non-monotonic dependence of temperature of Au nanometer films dissociation into droplets on their thickness on Al2O3 surface. Appl. Phys. A 99, 67–71 (2010). https://doi.org/10.1007/s00339-009-5500-z

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  • DOI: https://doi.org/10.1007/s00339-009-5500-z

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