Skip to main content
Log in

Temporal pulsewidth and the wavelength dependences of the product ions obtained by laser ablation of solid C60

  • Published:
Applied Physics A Aims and scope Submit manuscript

Abstract

By ablating solid C60 with a laser pulse, we observe various processes such as the prompt- and the delayed-ionization of C60, the fragmentation into molecular ions and the formation of cluster ions. We found these processes show distinct dependences on the temporal pulse width, the power and the wavelength of the ablation laser. From the observations, we could confirm efficient coupling of laser energy to C60 through the molecular absorption even with a laser pulse width less than the electron-phonon coupling time of the C60 molecule.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. R.J. Levis, M.J. DeWitt, J. Phys. Chem. A 103, 6493 (1999)

    Article  Google Scholar 

  2. I.V. Hertel, T. Laarmann, C.P. Schulz, Adv. At. Mol. Opt. Phys. 50, 219 (2005)

    Google Scholar 

  3. P. Wurz, K.R. Lykke, Chem. Phys. 184, 335 (1994)

    Article  ADS  Google Scholar 

  4. M. Tchaplyguine, K. Hoffmann, O. Duhr, H. Hohmann, G. Korn, H. Rottke, M. Wittmann, I.V. Hertel, E.E.B. Campbell, J. Chem. Phys. 112, 2781 (2000)

    Article  ADS  Google Scholar 

  5. M. Kurata-Nishimura, F. Tokanai, Y. Matsuo, T. Kobayashi, J. Kawai, H. Kumagai, K. Midorikawa, I. Tanihata, Y. Hayashizaki, Appl. Surf. Sci. 197–198, 715 (2002)

    Article  Google Scholar 

  6. T. Kobayashi, T. Kato, Y. Matsuo, M. Kurata-Nishimura, J. Kawai, Y. Hayashizaki, J. Chem. Phys. 126, 061101 (2007)

    Article  ADS  Google Scholar 

  7. T. Kobayashi, T. Kato, Y. Matsuo, M. Kurata-Nishimura, J. Kawai, Y. Hayashizaki, J. Chem. Phys. 127, 111101 (2007)

    Article  ADS  Google Scholar 

  8. K. Hansen, K. Hoffmann, E.E.B. Campbell, J. Chem. Phys. 119, 2513 (2003)

    Article  ADS  Google Scholar 

  9. G. von Helden, M.-T. Hsu, N. Gotts, M.T. Bowers, J. Phys. Chem. 97, 8182 (1993)

    Article  Google Scholar 

  10. J.R. Heath, R.F. Curl, R.E. Smalley, J. Chem. Phys. 87, 4236 (1987)

    Article  ADS  Google Scholar 

  11. A. Skumanich, Chem. Phys. Lett. 182, 486 (1991)

    Article  ADS  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to T. Kobayashi.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Kobayashi, T., Kato, T., Matsuo, Y. et al. Temporal pulsewidth and the wavelength dependences of the product ions obtained by laser ablation of solid C60 . Appl. Phys. A 92, 777–780 (2008). https://doi.org/10.1007/s00339-008-4564-5

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s00339-008-4564-5

PACS

Navigation