Abstract
Multi-layer metals films are widely used in modern engineering applications such as gold-coated metal mirrors used in high power laser systems. A transient heat flux model is derived to analyze multi-layer metal films under laser heating. The two separate system composed of electrons and the lattice is considered to take into account the electron–lattice interaction. The present model predicted the effects of underlying chromium’s thermal properties on temperature rise of the top gold layer. The effects of two adjacent and different metals with different electron–lattice coupling factors are analyzed for the heating mechanism of different lattices. The derived transient model combined with the two different conservation equations for the lattice and electrons are applied for the ultra short-pulse laser heating of a multi-layer film composed of gold and chromium.
Similar content being viewed by others
Abbreviations
- C :
-
Heat capacity (J m−3 K−1)
- G :
-
Electron lattice coupling factor (W m−3 K−1)
- J :
-
Laser pulse intensity (J m−3)
- k B :
-
Boltzmann constant (J K−1)
- L :
-
Film thickness (m)
- Q :
-
Heat flux (W m−2)
- R :
-
Surface reflectivity
- S :
-
Source term (W m−3)
- t :
-
Time (s)
- t p :
-
Laser pulse duration (s)
- T :
-
Temperature (K)
- x :
-
Spatial coordinate (m)
- δ :
-
Radiation penetration depth (m)
- κ :
-
Thermal conductivity (W m−1 K−1)
- τ :
-
Electron relaxation time (s)
- E:
-
Electron
- L:
-
Lattice
References
Qiu TQ, Tien CL (1992) Short-pulse laser heating of metals. Int J Heat Mass Transfer 35:719–726
Qiu TQ, Tien CL (1994) Femtosecond laser heating of multi layer metals. I. Analysis. Int J Heat Mass Transfer 37(17):2789–2797
Majumdar A (1998) Microscale energy transport in solids. In: Tien CL, Majundar A, Gerner FM (eds) Microscale energy transport. Taylor & Francis, Washington, DC, pp 3–93
Yilbas BS (2002) Short-pulse laser heating of gold–chromium layers: thermo-elasto-plastic analysis. J Phys D Appl Phys 35:1210–1217
Musikant S (1985) Optical materials: an introduction to selection and application. Marcel-Dekker, New York
Joseph EE, Presiozi L (1989) Heat waves. Rev Mod Phys 61:41–73
Maurer MJ (1969) Relaxation model for heat conduction in metals. J Appl Phys 40(13):5123–5130
Kaganov MI, Lifshitz IM, Tanatarov LV (1957) Relaxation between electrons and the crystalline lattice. Sov Phys JETP 4:173–178
Anisimov SI, Kapeliovich BL, Perel’man TL (1974) Electron emission from metal surfaces exposed to ultra short laser pulses. Sov Phys JETP 39:375–377
Qiu TQ, Tien CL (1993) Heat transfer mechanisms during short-pulse laser heating of metals. ASME J Heat Transfer 115:835–842
Ziman JM (1965) Principles of the theory of solids. Cambridge University Press, Cambridge
Yilbas BS (2001) Material response to thermal loading due to short pulse laser heating. Int J Heat Mass Transfer 44:3787–3798
Yilbas BS (2002) Laser short-pulse heating of gold–copper two-layer assembly: thermo-elasto-plastic analysis. Jpn J Appl Phys 41:5226–5234
Wilson AH (1954) The theory of metals, 2nd edn. Cambridge University Press, New York
Ziman JM (1960) Electrons and phonons: the theory of transport phenomena in solids. Clarendon Press, Oxford
Majumdar A (1993) Microscale heat conduction in dielectric thin films. ASME J Heat Transfer 115:7–16
Goodson KE (1996) Thermal conduction in nonhomogeneous CVD diamond layers in electronic microstructures. ASME J Heat Transfer 118:279–286
Fujimoto JG, Liu JM, Ippen EP (1984) Femtosecond laser interaction with metallic tungsten and nonequilibrium electron and lattice temperatures. Phys Rev Lett 53:1840–1847
Elsayed-Ali HE, Norris TB, Pessot MA, Mourou GA (1987) Time resolved observation of electron–phonon relaxation in copper. Phys Rev Lett 58:1212–1215
Brorson SD, Fujimoto JG, Ippen EP (1987) Femtosecond electronic heat transfer dynamics in thin gold film. Phys Rev Lett 59:1062–1065
Allen PB (1987) Theory of thermal relaxation of electrons in metals. Phys Rev Lett 59:1460–1463
Elsayed-Ali HE, Jushasz T (1993) Femtosecond time-resolved thermomodulation of thin gold films with different crystal structures. Phys Rev B 47:13599–13610
Eesley GL (1986) Observation of nonequilibrium electron and lattice temperatures in copper by picosecond laser pulses. Phys Rev B 33:2144–2151
Scouler WJ (1967) Temperature modulated reflectance of gold from 2 to 10 eV. Phys Rev Lett 18:445–448
Chapman S, Cowling TG (1953) The mathematical theory of non-uniform gases. Cambridge University Press, Cambridge
Acknowledgments
The authors would like to acknowledge Deniz Seker, M.S. for his contribution on computer applications.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Karakas, A., Tunc, M. & Camdali, Ü. Thermal analysis of thin multi-layer metal films during femtosecond laser heating. Heat Mass Transfer 46, 1287–1293 (2010). https://doi.org/10.1007/s00231-010-0653-z
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s00231-010-0653-z