Abstract
Concentrations, congener profiles, gas-particle partitioning and size distributions of polybrominated diphenyl ethers (PBDEs) in the atmosphere of Taizhou were studied to evaluate the impact of e-waste recycling on the environment. Total concentration of 13 PBDEs near the e-waste dismantling area was 506 pg m−3 in summer and 1,662 pg m−3 in winter, about 7 times higher than that of the reference urban site, but much lower than that of Guiyu, another major e-waste dismantling area in China. This should be attributable to the centralized management measures taken in recent years in Taizhou. BDE-209 was the major congener and mainly in coarse particles.
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Alaee M, Arias P, Sjodin A, Bergman A (2003) An overview of commercially used brominated flame retardants, their applications, their use patterns in different countries/regions and possible modes of release. Environ Int 29:683–689. doi:10.1016/S0160-4120(03)00121-1
Cahill TM, Groskova D, Charles MJ, Sanborn JR, Denison MS, Baker L (2007) Atmospheric concentrations of polybrominated diphenyl ethers at near-source sites. Environ Sci Technol 41:6370–6377. doi:10.1021/es070844j
Cetin B, Odabasi M (2007) Air-water exchange and dry deposition of polybrominated diphenyl ethers at a coastal site in Izmir Bay, Turkey. Environ Sci Technol 41:785–791. doi:10.1021/es061368k
Chen LG, Mai BX, Bi XH, Chen SJ, Wang XM, Ran Y, Luo XJ, Sheng GY, Fu JM, Zeng EY (2006) Concentration levels, compositional profiles, and gas-particle partitioning of polybrominated diphenyl ethers in the atmosphere of an urban city in South China. Environ Sci Technol 40:1190–1196. doi:10.1021/es052123v
Chen DH, Bi XH, Zhao JP, Chen LG, Tan JH, Mai BX, Sheng GY, Fu JM, Wong MH (2009) Pollution characterization and diurnal variation of PBDEs in the atmosphere of an E-waste dismantling region. Environ Pollut 157:1051–1057. doi:10.1016/j.envpol.2008.06.005
de Wit CA (2002) An overview of brominated flame retardants in the environment. Chemosphere 46:583–624. doi:10.1016/S0045-6535(01)00225-9
Deng WJ, Zheng JS, Bi XH, Fu JM, Wong MH (2007) Distribution of PBDEs in air particles from an electronic waste recycling site compared with Guangzhou and Hong Kong, South China. Environ Int 33:1063–1069. doi:10.1016/j.envint.2007.06.007
Goss KU, Schwarzenbach RP (1998) Gas/solid and gas/liquid partitioning of organic compounds: Critical evaluation of the interpretation of equilibrium constants. Environ Sci Technol 32:2025–2032. doi:10.1021/es9710518
Hayakawa K, Takatsuki H, Watanabe I, Sakai S (2004) Polybrominated diphenyl ethers (PBDEs), polybrominated dibenzo-p-dioxins/dibenzofurans (PBDD/Fs) and monobromo-polychlorinated dibenzo-p-dioxins/dibenzofurans (MoBPXDD/Fs) in the atmosphere and bulk deposition in Kyoto, Japan. Chemosphere 57:343–356. doi:10.1016/j.chemosphere.2004.06.038
Hoh E, Hites RA (2005) Brominated flame retardants in the atmosphere of the east-central United States. Environ Sci Technol 39:7794–7802. doi:10.1021/es050718k
Li YM, Jiang GB, Wang YW, Wang P, Zhang QH (2008) Concentrations, profiles and gas-particle partitioning of PCDD/Fs, PCBs and PBDEs in the ambient air of an E-waste dismantling area, southeast China. Chin Sci Bull 53:521–528. doi:10.1007/s11434-008-0125-8
Meng XZ, Zeng EY, Yu LP, Guo Y, Mai BX (2007) Assessment of human exposure to polybrominated diphenyl ethers in China via fish consumption and inhalation. Environ Sci Technol 41:4882–4887. doi:10.1021/es0701560
Pankow JF (1994) An absorption model of gas/particle partitioning of organic compounds in the atmosphere. Atmos Environ 28:185–188. doi:10.1016/1352-2310(94)90093-0
Park RJ, Jacob DJ, Chin M, Martin RV (2003) Sources of carbonaceous aerosols over the United States and implications for natural visibility. J Geophys Res-Atmos 108:4355. doi:10.1029/2002jd003190
Tittlemier SA, Halldorson T, Stern GA, Tomy GT (2002) Vapor pressures, aqueous solubilities, and Henry’s law constants of some brominated flame retardants. Environ Toxicol Chem 21:1804–1810. doi:10.1897/1551-5028(2002)021<1804:VPASAH>2.0.CO;2
UNEP (2005) E-waste, the hidden side of IT equipment’s manufacturing and use. Chapter 5-early warning on emerging environmental threats. Available via http://www.grid.unep.ch/product/publication/EABs.php
Wen S, Yang FX, Gong Y, Zhang XL, Hui Y, Li JG, Liu AL, Wu YN, Lu WQ, Xu Y (2008) Elevated levels of urinary 8-hydroxy-2&-deoxyguanosine in male electrical and electronic equipment dismantling workers exposed to high concentrations of polychlorinated dibenzo-p-dioxins and dibenzofurans, polybrominated diphenyl ethers, and polychlorinated biphenyls. Environ Sci Technol 42:4202–4207. doi:10.1021/es800044m
Wilford BH, Thomas GO, Jones KC, Davison B, Hurst DK (2008) Decabromodiphenyl ether (deca-BDE) commercial mixture components, and other PBDEs, in airborne particles at a UK site. Environ Int 34:412–419. doi:10.1016/j.envint.2007.09.007
Yang ZZ, Zhao XR, Zhao Q, Qin ZF, Qin XF, Xu XB, Jin ZX, Xu CX (2008) Polybrominated diphenyl ethers in leaves and soil from typical electronic waste polluted area in South China. Bull Environ Contam Toxicol 80:340–344. doi:10.1007/s00128-008-9385-x
Acknowledgments
This study is financially supported by the Natural Science Foundation of China (Grant No: 40775084) and Shanghai Leading Academic Disciplines (S030109) for which the authors are grateful. We are also grateful to Mr. Wang Deqing for his assistance in GC-MS analysis.
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Han, W., Feng, J., Gu, Z. et al. Polybrominated Diphenyl Ethers in the Atmosphere of Taizhou, a Major E-Waste Dismantling Area in China. Bull Environ Contam Toxicol 83, 783–788 (2009). https://doi.org/10.1007/s00128-009-9855-9
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DOI: https://doi.org/10.1007/s00128-009-9855-9