Abstract
The International Monitoring System includes a network of radionuclide detector stations and laboratories operated around the world monitoring for nuclear explosions. The United States Radionuclide Laboratory for radioxenon detection (USL16-NGL) was certified by the Preparatory Commission for the Comprehensive Nuclear-Test-Ban Treaty Organization in 2016. Since the certification of the laboratory, an additional set of four radioxenon detectors have been added to the laboratory. These supplementary radioxenon detectors allow for improved throughput for the laboratory and improving the ability to measure short lived radioxenon isotopes. In this paper, we describe the implementation of the additional radioxenon detectors and how they compare to current capabilities. Additionally, we detail implementation procedures to leverage the increased throughput.
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Auer, M., Axelsson, A., Blanchard, X., Bowyer, T. W., Brachet, G., Bulowski, I., Dubasov, Y., Elmgren, K., Fontaine, J. P., Harms, W., Hayes, J. C., Heimbigner, T. R., McIntyre, J. I., Panisko, M. E., Popov, Y., Ringbom, A., Sartorius, H., Schmid, S., Schulze, J., & Wernsperger, B. (2004). Intercomparison experiments of systems for the measurement of xenon radionuclides in the atmosphere. Applied Radiation and Isotopes, 60(6), 863–877. https://doi.org/10.1016/j.apradiso.2004.01.011
Bowyer, T. W., Abel, K. H., Hubbard, C. W., McKinnon, A. D., Panisko, M. E., Perkins, R. W., Reeder, P. L., Thompson, R. C., & Warner, R. A. (1998). Automated separation and measurement of radioxenon for the Comprehensive Test Ban Treaty. Journal of Radioanalytical and Nuclear Chemistry, 235(1–2), 77–82. https://doi.org/10.1007/bf02385941
Bowyer, T. W., Schlosser, C., Abel, K. H., Auer, M., Hayes, J. C., Heimbigner, T. R., McIntyre, J. I., Panisko, M. E., Reeder, P. L., Satorius, H., Schulze, J., & Weiss, W. (2002). Detection and analysis of xenon isotopes for the comprehensive nuclear-test-ban treaty international monitoring system. Journal of Environmental Radioactivity, 59(2), 139–151. https://doi.org/10.1016/S0265-931X(01)00042-X
Cagniant, A., Topin, S., Le Petit, G., Gross, P., Delaune, O., Philippe, T., & Douysset, G. (2018). SPALAX NG: A breakthrough in radioxenon field measurement. Applied Radiation and Isotopes, 134, 461–465. https://doi.org/10.1016/j.apradiso.2017.06.042
Cooper, M. W., Auer, M., Bowyer, T. W., Casey, L. A., Elmgren, K., Ely, J. H., Foxe, M. P., Gheddou, A., Gohla, H., Hayes, J. C., Johnson, C. M., Kalinowski, M., Klingberg, F. J., Liu, B., Mayer, M. F., McIntyre, J. I., Plenteda, R., Popov, V., & Zahringer, M. (2019). Radioxenon net count calculations revisited. Journal of Radioanalytical and Nuclear Chemistry, 321(2), 369–382. https://doi.org/10.1007/s10967-019-06565-y
Cooper, M. W., Ely, J. H., Haas, D. A., Hayes, J. C., McIntyre, J. I., Lidey, L. S., & Schrom, B. T. (2013). Absolute efficiency calibration of a beta–gamma detector. IEEE Transactions on Nuclear Science, 60(2), 676–680. https://doi.org/10.1109/TNS.2013.2243165
Currie, L. A. (1968). Limits for qualitative detection and quantitative determination. Application to radiochemistry. Analytical Chemistry, 40(3), 586–593. https://doi.org/10.1021/ac60259a007
Foltz Biegalski, K. M., & Biegalski, S. R. (2001). Determining detection limits and minimum detectable concentrations for noble gas detectors utilizing beta–gamma coincidence systems. Journal of Radioanalytical and Nuclear Chemistry, 248(3), 673–682. https://doi.org/10.1023/A:1010684410475
Foxe, M., Cooper, M., Haas, D., Hayes, J., Lowrey, J., & Prinke, A. (2019). Study of Shadowing in Beta–Gamma Coincidence Plots for Radioxenon (Issue PNNL-28404)
Foxe, M., Bowyer, T., Cameron, I., Cooper, M., Hayes, J., Haas, D., Lidey, L., Mayer, M., Mendez, J., & Slack, J. (2020a). Design and operation of the U.S. Radionuclide Noble Gas Laboratory for the CTBTO. Pure and Applied Geophysics. https://doi.org/10.1007/s00024-020-02591-0
Foxe, M., Bowyer, T., Carr, R., Orrell, J., & VanDevender, B. (2020b). Antineutrino detectors remain impractical for nuclear explosion monitoring. Pure and Applied Geophysics. https://doi.org/10.1007/s00024-020-02464-6
Gohla, H., Auer, M., Cassette, P., Hague, R. K., Lechermann, M., & Nadalut, B. (2016). Radioxenon standards used in laboratory inter-comparisons. Applied Radiation and Isotopes, 109, 24–29. https://doi.org/10.1016/j.apradiso.2015.11.044
Haas, D. A., Eslinger, P. W., Bowyer, T. W., Cameron, I. M., Hayes, J. C., Lowrey, J. D., & Miley, H. S. (2017). Improved performance comparisons of radioxenon systems for low level releases in nuclear explosion monitoring. Journal of Environmental Radioactivity, 178–179, 127–135. https://doi.org/10.1016/j.jenvrad.2017.08.005
Reeder, P. L., Bowyer, T. W., & Perkins, R. W. (1998). Beta–gamma counting system for Xe fission products. Journal of Radioanalytical and Nuclear Chemistry, 235(1–2), 89–94. https://doi.org/10.1007/BF02385943
Ringbom, A., Larson, T., Axelsson, A., Elmgren, K., & Johansson, C. (2003). SAUNA—A system for automatic sampling, processing, and analysis of radioactive xenon. Nuclear Instruments and Methods in Physics Research, Section a: Accelerators, Spectrometers, Detectors and Associated Equipment, 508(3), 542–553. https://doi.org/10.1016/S0168-9002(03)01657-7
Watrous, M. G., Delmore, J. E., Hague, R. K., Houghton, T. P., Jenson, D. D., & Mann, N. R. (2015). Radioxenon spiked air. Journal of Environmental Radioactivity, 150, 126–131. https://doi.org/10.1016/j.jenvrad.2015.08.005
Zhou, C., Zhou, G., Feng, S., Zhao, X., Huang, D., Tian, Z., Yu, X., & Cheng, Z. (2019). Radon removal trap design and coefficient testing for the development of an effective radioxenon sampling, separation and measurement system. Journal of Environmental Radioactivity, 199–200, 39–44. https://doi.org/10.1016/j.jenvrad.2019.01.003
Acknowledgements
The authors acknowledge the support of the Defense Threat Reduction Agency (DTRA) Nuclear Arms Control Technology (NACT) Program, U.S. Department of Defense, for funding this work. Any subjective views or opinions expressed in the paper do not necessarily represent the views of the U.S. Department of Energy, U.S. Department of Defense or the United States Government. Approved for public release; distribution is unlimited. PNNL-SA-169579.
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This study was funded by Defense Threat Reduction Agency.
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Foxe, M., Bowyer, T., Cameron, I. et al. Implementation of Additional Beta–Gamma Detectors for Improved Radioxenon Laboratory Throughput. Pure Appl. Geophys. 180, 1469–1478 (2023). https://doi.org/10.1007/s00024-022-03106-9
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DOI: https://doi.org/10.1007/s00024-022-03106-9