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Determination of uranium, antimony, indium, bromine and cobalt in atmospheric aerosols using epithermal neutron activation and a low-energy photon detector

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Abstract

Owing to the high ratio of resonance integral to thermal neutron activation cross-section of238U, a 5 min epithermal neutron irradiation under cadmium shielding, followed by measurement of the 74 keV photopeak of239U with a high resolution low-energy photon Ge(Li) detector, allows the fast determination of uranium in aerosols collected on a Whatman 41 cellulose filter. Uranium blanks of the cellulose filter paper require correction and limit the sensitivity. Simultaneously the concentrations of the elements cobalt, bromine, antimony and indium can be determined. In Belgium, the uranium concentrations of the aerosols were found to be constant and comparable to the uranium contents of rocks.

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References

  1. E. STEINNES, D. BRUNE, Talanta, 16 (1969) 1326.

    Article  CAS  Google Scholar 

  2. E. STEINNES, Radiochem. Radioanal. Letters, 16 (1973) 25.

    CAS  Google Scholar 

  3. H. MATSUDA, Y. TSUTSUI, S. NAKANO, S. UNEMOTO, Talanta, 19 (1972) 851.

    Article  CAS  Google Scholar 

  4. A. V. MURALI, P. P. PAREKH, M. SANKAR DAS, Anal. Chim. Acta, 50 (1970) 71.

    Article  CAS  Google Scholar 

  5. T. HASHIMOTO, Anal. Chim. Acta, 56 (1971) 347.

    Article  CAS  Google Scholar 

  6. T. NOZAKI, M. ICHIKAWA, T. SASUGA, M. INARIDA, J. Radioanal. Chem., 6 (1970) 33.

    Article  CAS  Google Scholar 

  7. J. W. ARDEN, N. H. GALE, Anal. Chem., 46 (1974) 687.

    Article  CAS  Google Scholar 

  8. C. TURKOWSKY, H. STÄRK, H. J. BORN, Radiochim. Acta, 8 (1967) 27.

    CAS  Google Scholar 

  9. G. A. WELFORD, R. BAIRD, Health Phys., 13 (1967) 1321.

    CAS  Google Scholar 

  10. M. WALD, G. WIEGAND, Radiochim. Acta, 19 (1973) 37.

    CAS  Google Scholar 

  11. P. PAKALNS, Anal. Chim. Acta, 69 (1974) 211.

    Article  CAS  Google Scholar 

  12. E. I. HAMILTON, Health Phys., 19 (1970) 511.

    Article  CAS  Google Scholar 

  13. P. MCEACHERN, W. G. MYERS, F. A. WHITE, Environ. Sci. Technol., 5 (1971) 700.

    Article  CAS  Google Scholar 

  14. R. VAN DER LINDEN, F. DE CORTE, J. HOSTE, J. Radioanal. Chem., 20 (1974) 695.

    Article  Google Scholar 

  15. R. VAN DER LINDEN, F. DE CORTE, P. VAN DEN WINKEL, J. HOSTE, J. Radioanal. Chem., 11 (1972) 133.

    Article  Google Scholar 

  16. E. STEINNES, Activation Analysis in Geochemistry and Cosmochemistry, Universitetsforlaget, Oslo, 1971, p. 113–128; plus references of this paper.

  17. W. H. ZOLLER, G. E. GORDON, Anal. Chem., 42 (1970) 257.

    Article  CAS  Google Scholar 

  18. N. E. HOLDEN, F. W. WALKER, Chart of the Nuclides, 11th ed., General Electric Co., April 1972.

  19. R. VAN DER LINDEN, F. DE CORTE, J. HOSTE, J. Radioanal. Chem., 23 (1974) 113.

    Article  Google Scholar 

  20. I. M. H. PAGDEN, G. J. PEARSON, J. M. BEWERS, J. Radioanal. Chem., 8 (1971) 127, 373.

    Article  CAS  Google Scholar 

  21. J. BLACHOT, R. DE TOURREIL, J. Radioanal. Chem., 11 (1972) 351.

    Article  CAS  Google Scholar 

  22. R. DAMS, R. HEINDRYCKX, Atmos. Environ., 7 (1973) 319.

    Article  CAS  Google Scholar 

  23. W. MAENHAUT, private communication.

  24. J. HERTOGEN, R. GIJBELS, Anal. Chim. Acta, 56 (1971) 61.

    Article  CAS  Google Scholar 

  25. R. DAMS, J. A. ROBBINS, K. A. RAHN, J. W. WINCHESTER, Anal. Chem., 42 (1970) 861.

    Article  CAS  Google Scholar 

  26. R. HEINDRYCKX, R. DAMS, Radiochem. Radioanal. Letters, 16 (1974) 209.

    CAS  Google Scholar 

  27. D. F. COVELL, Anal. Chem., 31 (1959) 1785.

    Article  CAS  Google Scholar 

  28. D. DE SOETE, R. GIJBELS, J. HOSTE, Neutron Activation Analysis, Wiley-Interscience, New York 1972, p. 482.

    Google Scholar 

  29. R. W. STOUGHTON, J. HALPERIN, Nucl. Sci. Eng., 15 (1963) 314.

    CAS  Google Scholar 

  30. F. ROSSITTO, M. TERRANI, S. TERRANI, Nucl. Instr. Methods, 103 (1972) 77.

    Article  CAS  Google Scholar 

  31. F. J. FLANAGAN, Geochim. Cosmochim. Acta, 37 (1973) 1189.

    Article  CAS  Google Scholar 

  32. J. W. MORGAN, K. S. HEIER, Earth Planet. Sci. Letters, 1 (1966) 158.

    Article  CAS  Google Scholar 

  33. A. O. BRUNFELT, E. STEINNES, Anal. Chim. Acta, 48 (1969) 13.

    Article  CAS  Google Scholar 

  34. J. HERTOGEN, private communication.

  35. Conf. on Chemical Analysis of Airborne Particulates. Intercomparison and Evaluation of Analytical Techniques, Ispra (Italy), July 1974.

  36. Study of National Air Pollution by Combustion, Progress Report, 1972, Inst. Nucl. Wet. (Univ. Gent); Lab. Toxicol. (Univ. Liege), 1973.

  37. M. Janssens, R. Dams, Anal. Chim. Acta, 70 (1974) 25.

    Article  CAS  Google Scholar 

  38. K. A. RAHN, M. DEMUYNCK, R. DAMS, J. DEGRAEVE, Proc. 3rd Intern. Clean Air Congress. Düsseldorf (Federal Republic of Germany), 1973, VDI-Verlag GmbH, Düsseldorf, C81.

    Google Scholar 

  39. B. MASON, Principles of Geochemistry, 3rd ed., Wiley, New York, 1966, p. 46.

    Google Scholar 

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Authors and Affiliations

  1. Institute of Nuclear Sciences, Rijksuniversiteit Gent, Proeftuinstraat 86, B-9000, Ghent, Belgium

    M. Janssens, B. Desmet (Technician of the I.I.K.W.), R. Dams & J. Hoste

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  1. M. Janssens
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  2. B. Desmet
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  3. R. Dams
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  4. J. Hoste
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Janssens, M., Desmet, B., Dams, R. et al. Determination of uranium, antimony, indium, bromine and cobalt in atmospheric aerosols using epithermal neutron activation and a low-energy photon detector. J. Radioanal. Chem. 26, 305–315 (1975). https://doi.org/10.1007/BF02524447

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  • DOI: https://doi.org/10.1007/BF02524447

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