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A redetermination of the half-life of239Pu by specific activity measurements

  • Advances in Measurement and Data Handling
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Abstract

The half-life of239Pu has been determined by specific activity measurements on solutions prepared from the stoichiometric compounds Cs2 PuCl6, using plutonium 99.03% enriched in239Pu. The value obtained is 24,088 years, to which a realistic uncertainty of ±51 years is ascribed. This result is discussed in relationship to all previously reported values.

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References

  1. J. W. STOUT, W. N. JONES, Phys. Rev., 71 (1947) 582.

    Article  CAS  Google Scholar 

  2. G. C. HANNA, C. H. WESTCOTT, H. D. LEMMEL, B. R. LEONARD, J. S. ATORY, P. M. ATTREE, Atomic Energy Rev., 1 (1969) 3.

    Google Scholar 

  3. F. L. OETTING, Proc. IAEA Conf. on Thermodynamics of Nuclear Materials SM-98/37, 1967 p. 55.

  4. F. L. OETTING, RFP-1469, 1970.

  5. F. L. OETTING, J. Inorg. Nucl. Chem., 27 (1965) 2151.

    Article  CAS  Google Scholar 

  6. P. A. SELLARS, W. C. BENTLEY, M. H. STUDIER, ANL-5411, 1955.

  7. D. BROWN, S. N. DIXON, K. M. GLOVER, F. J. G. ROGERS, J. Inorg. Nucl. Chem., 30 (1968) 19.

    Article  CAS  Google Scholar 

  8. H. W. KIRBY, J. Inorg. Nucl. Chem., 18 (1961) 8.

    Article  CAS  Google Scholar 

  9. J. STOREY, AEE, Winfrith, Private Communication, 1974.

  10. A. LORENZ, INDC (NDS)-74/L+SP.

  11. Handbook of Chemistry and Physics 48th ed. 1967–68.

  12. C. E. PIETRI, A. W. WENZEL, Talanta, 18 (1971) 849.

    Article  CAS  Google Scholar 

  13. C. E. PIETRI, Anal. Chem., 34 (1962) 1604.

    Article  CAS  Google Scholar 

  14. F. J. MINER, R. P. DE GRAZIO, J. T. BYRNE, Anal. Chem. 35 (1963) 1113.

    Article  Google Scholar 

  15. K. M. GLOVER, R. HURST, AERE C/M 100, 1951.

  16. K. M. GLOVER, Proc. IAEA Conf. on Standardisation of Radionuclide SM-79/39, 1967, p. 463.

  17. M. LOUNSBURY, R. W. DURHAM, Proc. International Conference on Chemical Nuclear Data, 1971, p. 215.

  18. A. H. JAFFEY, Rev. Sci. Instr., 25 (1954) 349.

    Article  Google Scholar 

  19. E. R. COHEN, N. B. TAYLOR, J. Phys. Chem. Ref. Data, 2 (1973) 663.

    Article  CAS  Google Scholar 

  20. L. L. LUCAS, W. B. MANN, Int. J. App. Rad. Isotopes, 29 (1978) 523.

    Google Scholar 

  21. A. LORENZ, INDC (NDS) 96/N, 1978.

  22. American National Standards Institute N/15.22, 1975.

  23. A. H. WAPSTRA, N. B. GOVE, Nuclear Data Tables, A9 (1971) parts 4–5.

  24. D. BROWN, K. M. GLOVER, M. KING, G. PHILLIPS, F. J. G. ROGERS, R. A. P. WILTSHIRE, AERE R 9270, 1981.

  25. R. VANINBROUKX, J. BROTHAERTS, B. DENECKE, M. GALLET, G. GROSSE, F. HENDRICKX, A. LOOPMANS, W. ZEHNER, NEANDC (E) 172 (U) 1976, p. 25.

    Google Scholar 

  26. R. VANINBROUKX, B. DENECKE, M. GALLET, G. GROSSE, F. HENDRICKX, W. ZEHNER, NEANDC (E)-202 (U). Vol. 111-Euratom. 1978.

  27. A. H. JAFFREY, H. DIAMOND, W. C. BENTLEY, K. F. FLYN, D. J. ROKOP, A. M. ESSLING, J. WILLIAMS, Phys. Rev., C 16 (1977) 354.

    Article  Google Scholar 

  28. G. W. FARWELL, J. E. ROBERTS, A. C. WAHL, Phys. Rev., 94 (1954) 364.

    Article  Google Scholar 

  29. B. B. CUNNINGHAM, L. B. WERNER, J. Am. Chem. Soc., 71 (1949) 1521.

    Article  CAS  Google Scholar 

  30. E. F. WESTRUM, Jr., J. C. HINDMAN, R. GREENLEE, The Transuranium Elements 14B Paper 22.80.

  31. J. C. WALLMAN, UCRL-1255, 1951.

  32. T. L. MARKIN, J. Inorg. Nucl. Chem., 9 (1959) 320.

    Article  CAS  Google Scholar 

  33. Ya. P. DOKUCHAEV, I. S. OSIPOU, Soviet J. Atomic Energy 6 (1959) 41.

    Google Scholar 

  34. H. R. IHLE, M. KAROYANNIS, A. P. MURRENHOFF, JUL-347-PC, 1966.

  35. B. M. ALEKSANDROV et al., Bull. Acad. Sci. USSR Physics SER, 39 (1975) 20.

    Google Scholar 

  36. R. VANINBROUKX, CBNM/RN/11/75.

  37. R. VANINBROUKX, CBNM/RN/46/79.

  38. A. LORENZ, INDC (NDS)-108/N (1979).

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Brown, D., Glover, K.M., King, M. et al. A redetermination of the half-life of239Pu by specific activity measurements. J. Radioanal. Chem. 64, 181–193 (1981). https://doi.org/10.1007/BF02518350

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  • DOI: https://doi.org/10.1007/BF02518350

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