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Compton suppression gamma-spectroscopy in the analysis of radium and lead isotopes in ocean sediments

  • Radium and Radon Measurement
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Abstract

Compton suppression gamma-spectroscopy provides an efficient method for measuring the concentration of226Ra,228Ra, and210Pb in ocean sediments. The background reduction realized from the suppressed mode of operation provides an “active shield” to allow for the low-level counting required for these measurements. We have used the method to study the possible accumulation of radium from produced waters in sediments from Gulf of Mexico sites of varied distances from drill platforms. In addition,210Pb levels were determined to evaluate the use of our spectrometer for this purpose. Baseline undisturbed concentrations have been obtained from the study of subsurface core material which predates drilling activities. Correlations of radium isotope concentrations with iron and barium provide information concerning the possible relationships between radium levels and drilling activity (excess barium) and natural variations in sediment texture (iron).

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References

  1. T.F. Kraemer, D.F. Reid, Isotope Geosci., 2 (1984) 153.

    CAS  Google Scholar 

  2. J. Kantele, P. Suominen, Nucl. Instr. Meth., 41 (1966) 41.

    Article  CAS  Google Scholar 

  3. R. L. Auble, D. B. Beery, G. Berzins, L. M. Beyer, R. C. Etherton., W. H. Kelly, Nucl. Instr., Meth., 51 (1967) 61.

    Article  CAS  Google Scholar 

  4. R. D. Cooper, G. L. Brownell, Nucl. Instr. Meth., 51 (1967) 72.

    Article  CAS  Google Scholar 

  5. W. Michaelis, H. Kupfer, Nucl. Instr. Meth., 56 (1967) 181.

    Article  CAS  Google Scholar 

  6. S. R. Lewis, N. H. Shafrir, Nucl. Instr. Meth., 93 (1971) 317.

    Article  CAS  Google Scholar 

  7. N. A. Wogman, Design and Environmental Applications of an Ultra-Low Background, High-Efficiency Intrinsic Ge Gamma-Ray Spectrometer, IAEA-SM-252/25, 1980.

  8. M. Petra, G. Swift, S. Landsberger, Nucl. Instr. Meth Phys. Res., A299 (1990) 85.

    Google Scholar 

  9. P. N. Boothe, B. J. Presley, Distribution and Behavior of Drilling Fluids and Cuttings around Gulf of Mexico Drilling Sites, final report to the American Petroleum Institute, Washington, DC.

  10. T.H. Trefry, B.J. Presley, Environ. Geol., 1 (1976) 282.

    Google Scholar 

  11. J. M. Brooks, C. P. Giammona, Mississippi-Alabama Marine Exosystem Study Annual Report: Year 2, report to the Minerals Management Service, New Orleans, LA.

  12. M. C. Kennicatt (Ed.), Gulf of Mexico Offshore Operations Monitoring Experiment, Phase I: Sublethal Responses to Contaminant Exposure, final report (OCS Study MMS 14-35-001-30582) to the Minerals Management Service, New Orleans, LA.

  13. E. S. Gladney, B. T. O'Malley, I. Roelandts, T. E. Gills, Standard Reference Materials: Compilation of Elemental Concentration Data for NBS Clinical, Biological, Geological, and Environmental Reference Materials, NBS Special Publication 260-111, U.S. Department of Commerce, November, 1987.

  14. Science Applications International Corporation, Analysis of Radioactivity in Produced Waters from Offshore Oil and Gas Platforms, final report submitted to U.S. Environmental Protection Agency (Contract 68-CO-0035), 1992.

  15. T. M. Randolph, R. C. Ayers, Jr., R. A. Shaul, A. D. Hart, W. T. Shebs, J. P. Ray, S. A. Savant-Malhiet R. V. Rivera, Produced Water,J. P. Ray andF. R. Englehardt (Eds), Plenum Press, New York, 1992, p. 267.

    Google Scholar 

  16. D. G. Moore, M. R. Scott, J. Geophys. Res., 91 (1986) 14317.

    CAS  Google Scholar 

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James, W.D., Boothe, P.N. & Presley, B.J. Compton suppression gamma-spectroscopy in the analysis of radium and lead isotopes in ocean sediments. J Radioanal Nucl Chem 236, 261–266 (1998). https://doi.org/10.1007/BF02386354

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  • DOI: https://doi.org/10.1007/BF02386354

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