Abstract
The distribution and inventory of artificial radionuclides,239,240Pu and137Cs were determined in the East China and the Yellow Seas in 1987. Almost all of239,240Pu and 50 to 80% of137Cs in the continental shelf area are retained in the sediment column.239,240Pu sediment inventory in the sea area is larger than the fallout input and tends to increase southwardly. This excess239,240Pu and the lateral distribution are attributable to the supply of239,240Pu by the Yangtze River discharge. On the contrary,137Cs sediment inventory shows a decrease to the south, and the fact can be accounted for by the southward dispersion of fine silt particles discharged from the Yellow River. Total137Cs inventory is smaller than the estimated fallout input, and the fact seems to indicate dispersion of137Cs out of the shelf region. Vertical profiles of239,240Pu and137Cs contents in sediments differ from that of natural210Pb, implying the effect of varied accumulation rates of the artificial radionuclides over the sediment particle mixing by benthic organisms. Apparent maximum sediment particle mixing coefficient (D B ) calculated from the excess210Pb profiles in stations located between the inner and outer shelves ranged from 1.4 to 8.3 cm2y−1. ThisD B value is higher than that in the Okinawa Trough (1.0 cm2y−1), but lower than previously estimatedD B value (≈26 cm2y−1) in the outer shelf mud.
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Beardsley, R. C., R. Limeburner, H. Yu and G. A. Cannon (1985): Discharge of the Changjiang (Yangtze River) into the East China Sea.Cont. Shelf Res.,4, 57–76.
Biscaye, T. G., R. F. Anderson and B. L. Deck (1988): Fluxes of particles and constituents to the eastern United States continental slope and rise: SEEP-I.Cont. Shelf Res.,8, 855–904.
Bradley, P. E., B. E. Economides, M. S. Baxter and D. J. Ellett (1988): Sellafield radiocesium as a tracer of water movement in the Scottish coastal zone. p. 281–293. InRadionuclides; A Tool for Oceanography, ed. by J. C. Guary, P. Guegueniat and R. J. Pentreath, Elsevier Sci. Pub. LTD, London.
Buesseler, K. O., H. D. Livingston and E. R. Sholkovitz (1985):239,240Pu and excess210Pb inventories along the shelf and slope of the northeast U.S.A.Earth Planet. Sci. Lett.,76, 10–22.
Calmet, D., J. M. Fernandez, P. Maunier and Y. Baron (1988): Spatal and temporal variations in the levels of cesium in the northwestern Mediterranean sea water (1985–1986). p. 217–226. InRadionuclides: A Tool for Oceanography, ed. by J. C. Guary, P. Guegueniat and R. J. Pentreath, Elsevier Sci. Pub. LTD, London.
Carpenter, R., T. M. Beasley, D. Zahnle and L. K. Somayajulu (1987): Cycling of fallout (Pu,241Am,137Cs) and natural (U, Th,210Pb) radionuclides in Washington continental slope sediments.Geochim. Cosmochim. Acta,51, 1897–1921.
Cochran, J. K. (1985): Particle mixing rates in sediments of the eastern equatorial Pacific: Evidence from210Pb,239,240Pu and137Cs distributions at MANOP sites.Geochim. Cosmochim. Acta,49, 1195–1210.
DeMaster, D. J., B. A. McKee, C. A. Nittouer, J.-c. Quian and G.-d. Cheng (1985): Rates of sediment accumulation and particle reworking based on radiochemical measurements from continental shelf deposits in the East China Sea.Cont. Shelf Res.,4, 143–158.
Desai, M. V. M., N. N. Dey, V. V. Kulkarni and K. C. Pillai (1989): Distribution of137Cs in various size fractions of bottom sediments of Bombay Harbour Bay.Indian J. Mar. Sci.,18, 198–200.
Donoghue, J. E., O. P. Bricker and C. R. Olsen (1989): Particle-borne radionuclides as tracer for sediment in the Susquehanna River and Chesapeake Bay.Estuarine Coast. Shelf Sci.,29, 341–360.
Hamada, S. and T. Mitsusio (1987): Submarine geological classification of bottom sediments in the East China Sea and the Yellow Sea.Bull. Seikai Fish. Res. Lab.,64, 25–34 (in Japanese).
Hayes, D. W. and W. M. Sackett (1987): Plutonium and cesium radionuclides in sediment of the Savanna River estuary.Estuarine Coast. Shelf Sci.,25, 169–174.
Horibe, Y., K. Taira, T. Terashima, H. Tsubota, S. Imawaki, K. Kodama and H. Igarashi (1977): Development and recovery of moored arrays of instruments, large volume sampler, autoanalyzer. p. 184–208. InEnvironmental Marine Science, ed. by Y. Horibe, Univ. Tokyo Press, Tokyo (in Japanese).
Kelly, M., S. Mudge, J. Hamilton-Taylor and K. Bradshaw (1988): The behaviour of dissolved plutonium in the Esk estuary, U.K. p. 321–330. InRadionuclides; A Tool for Oceanography, ed. by J. C. Guary, P. Guegueniat and R. J. Pentreath, Elsevier Sci. Pub. LTD, London.
Kershaw, P. J., P. A. Gurbutt, A. K. Young and D. J. Allington (1988): Scavenging and bioturbation in the Irish Sea from measurements of234Th/238U and210Pb/226Ra disequilibria. p. 131–142. InRadionuclides; A Tool for Oceanography, ed. by J. C. Guary, P. Guegueniat and R. J. Pentreath, Elsevier Sci. Pub. LTD, London.
Koide, M., E. D. Goldberg and V. F. Hodge (1980):241Pu and241Am in sediment from coastal basins off California and Mexico.Earth Planet. Sci. Lett.,48, 250–256.
Livingston, H. D., V. T. Bowen and S. L. Kupferman (1982): Radionuclides from Windscale discharge II. Their dispersion in Scottish and Norwegian coastal circulation.J. Mar. Res.,40, 1227–1258.
McKee, B. A., D. J. DeMaster and C. A. Nittrouer (1984): The use of234Th/238U disequilibrium to examine the fate of particle-reactive species on the Yangtze continental shelf.Earth Planet. Sci. Lett.,68, 431–442.
McLean, R. I. and J. K. Summers (1990): Evaluation of transport and storage of Co-60, Cs-134, Cs-137 and Zn-65 by river sediments in the lower Susquehannah River.Environ. Poll.,63, 137–153.
Milliman, J. D., R. C. Beardsley, Z.-s. Yang and R. Limeburner (1985): Modern Huanghe-derived muds on the outer shelf of the East China Sea: Identification and potential transport mechanisms.Cont. Shelf Res.,4, 175–188.
Nagaya, Y. and K. Nakamura (1975): Transport and accumulation of radiocobalt in the marine sediment of Urazoko Bay. p. 313–329. InImpacts of Nuclear Release into the Aquatic Environment, IAEA, Vienna.
Nagaya, Y. and K. Nakamura (1981): Artificial radionuclides in the western Northwest Pacific (I);90Sr and137Cs in the deep waters.J. Oceanogr. Soc. Japan,37, 135–144.
Nagaya, Y. and K. Nakamura (1984):239,240Pu,137Cs and90Sr in the central North Pacific.J. Oceanogr. Soc. Japan,40, 416–424.
Nagaya, Y. and K. Nakamura (1986):239,240Pu and137Cs concentrations in some marine biota, mostly from the sea around Japan.Nippon Suisan Gakkaishi,53, 873–879.
Nagaya, Y. and K. Nakamura (1987): Artificial Radionuclides in the western Northwest Pacific(II):137Cs and239,240Pu inventories in water and sediment columns observed from 1980 to 1986.J. Oceanogr. Soc. Japan,43, 345–355.
Nakamura, K. and Y. Nagaya (1985): Accumulation of Cs-137 and Pu-239, 240 in sediments of the coastal sea and the North Pacific. p. 171–180. InMarine and Coastal Geochemistry, ed. by A. C. Sigleo and A. Hattori, Lewis Pub. INC, Chelsea.
Nakamura, K. and Y. Nagaya (1990): Distribution of137Cs and239,240Pu in the sediment of the Seto Inland Sea.J. Radioanal. Nucl. Chem., Articles,138, 153–164.
Narita, H., K. Harada and S. Tsunogai (1990): Lateral transport of sediment particles in the Okinawa Trough determined by natural radionuclides.Geochem. J.,24, 207–216.
Nozaki, Y., J. K. Cochran, K. K. Turekian and G. Keller (1977): Radiocarbon and lead-210 distribution in submersible-taken deep-sea cores from Project FAMOUS.Earth Planet. Sci. Lett.,34, 167–173.
Nozaki, Y., V. Kasemuspaya and H. Tsubota (1989): Mean residence time of the shelf water in the East China and Yellow Seas determined by228Ra/226Ra measurements.Geophys. Res. Lett.,16, 1297–1300.
Nozaki, Y., H. Tsubota and V. Kasemsupaya (1991): Residence time of surface water and particule reactive210Pb and210Po in the East China and Yellow Seas.Geochim. Cosmochim. Acta,55, 1265–1272.
Olsen, C. R., M. Thein, I. L. Larsen, P. D. Lowry, P. J. Mulholland, N. H. Cutshall, J. T. Byrd and H. L. Windom (1989): Plutonium, lead-210 and carbon isotopes in the Savanna estuary: Riverborne versus marine sources.Environ. Sci. Tech.,23, 1475–1481.
Rhoads, D. C., D. F. Boesch, Z. Tang, F.-S. Xu, L.-C. Huang and K. J. Nilsen (1985): Macrobenthos and sedimentary facies on the Changjuan delta platform and adjacent continental shelf, East China Sea.Cont. Shelf Res.,4, 189–213.
Shen, G. T., E. R. Sholkovitz and D. R. Mann (1983): The coagulation of dissolved239,240Pu in estuaries as determined from a mixing experiment.Earth Planet. Sci. Lett.,64, 437–444.
Shi, Y.-l., W. Yang and M.-e. Ren (1985): Hydrological characteristics of the Changjiang and its relation to sediment transport to the sea.Cont. Shelf Res.,4, 5–15.
Sholkovitz, E. R. and D. R. Mann (1987):239,240Pu in estuarine and shelf waters of the north-eastern United States.Estuarine Coast. Shelf Sci.,25, 413–434.
Silverberg, N., H. V. Nguyen, G. Delibrias, M. Koide, B. Sundby, Y. Yokoyama and R. Chesselet (1986): Radionuclide profiles, sedimentation rates and bioturbation in modern sediments of the Laurentian Trough, Gulf of St. Lawrence.Oceanol. Acta,9, 285–290.
Simpson, H. J. and S. C. Williams (1975): Plutonium and cesium radionuclides in the Hudson River estuary. COO-2529-1, 44 pp.
Sternberg, R. W., L. H. Larsen and Y. T. Miao (1985): Tidally driven sediment transport on the East China Sea continental shelf.Cont. Shelf Res.,4, 105–129.
Taylor, J. Hamilton, M. Kelly, S. Mudge and K. Bradshaw (1987): Rapid remobilization of plutonium from estuarine sediments.J. Environ. Radioact.,5, 409–423.
United Nations Scientific Committee on the Effects of Atomic Radiation (1982): Exposure resulting from nuclear explosions. p. 211–248. InIonizing Radiation: Sources and Biological Effects, 1982 Report, United Nations, New York.
Woodhead, D. S. (1988): Mixing process in near-shore marine sediments as inferred from the bioturbation of radionuclides discharged into the northeast Irish Sea from BNFL, Sellafield. p. 331–340. InRadionuclides: A Tool for Oceanography, ed. by J. C. Guary, P. Guegueniat and R. J. Pentreath, Elsevier Sci. Publ. LTD, London.
Wright, L. D., W. J. Wiseman, B. D. Bornhold, D. B. Prior, J. N. Suhayda, G. H. Keller, Z.-s. Yang and Y. B. Fan (1988): Marine dispersal and deposition of Yellow River silts by gravity driven underflows.Nature,332, 629–632.
Wright, L. D., W. J. Wiswman, Jr., Z.-S. Yang, B. D. Bornhold, G. H. Keller, D. B. Prior and J. N. Suhayda (1990): Processes of marine dispersal and deposition of suspended silt off the modern mouth of the Huanghe (Yellow River).Cont. Shelf Res.,10, 1–40.
Yang, H.-s., Y. Nozaki, H. Sakai, Y. Nagaya and K. Nakamura (1986): Natural and man-made radionuclide distributions in northwest Pacific deep-sea sediments: rates of sedimentation, bioturbation and226Ra migration.Geochem. J.,20, 29–40.
Ying, W. and D. G. Aubrey (1987): The characteristics of the China coastline.Cont. Shelf Res.,7, 329–349.
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Nagaya, Y., Nakamura, K. 239,240Pu and137Cs in the East China and the Yellow Seas. J Oceanogr 48, 23–35 (1992). https://doi.org/10.1007/BF02234030
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DOI: https://doi.org/10.1007/BF02234030