Abstract
A nonlinear stochastic Liouville equation postulated phenomenologically and used recently for the description of the interplay of damping and nonlinearity is shown to arise in a natural manner as an approximate consequence of a set of Langevin equations introduced for the analysis of the Brownian motion of a nonlinear quantum dimer. The validity of the phenomenological equation is discussed in the light of the approximate derivation. A more physical transport equation for the system density matrix is obtained and shown, on the one hand to reduce to the phenomenological equation in an appropriate high temperature limit, and on the other to predict novel behavior. The new nonlinear stochastic Liouville equation we present is capable of unifying the description of the nonlinear transport of quasiparticles in several different parameter regimes and we suggest that it should be regarded and used in the same role in the study of the physics of nonlinear transport phenomena that the linear stochastic Liouville equation does in fields such as (linear) exciton dynamics in molecular crystals and aggregates.
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Kenkre, V.M., Grigolini, P. A new nonlinear stochastic Liouville equation. Z. Physik B - Condensed Matter 90, 247–253 (1993). https://doi.org/10.1007/BF02198161
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DOI: https://doi.org/10.1007/BF02198161