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High pressure of solid noble gases in metals

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Abstract

The fact that noble gas ions implanted in metals with concentrations of a few percent precipitate at room temperature as solid bubbles under high pressure with a structure epitaxial with the host matrix (fcc or hcp) has been investigated recently. A brief survey of the results measured by transmission electron microscopy, glancing angle X-ray diffraction, energy-loss spectroscopy and positron annihilation is given. The main part of this paper deals with a study on83Kr+ implanted in Al using Mössbauer spectroscopy. The results are as follows: the precipitates grow from 1.5 nm after implantation to 3.7 nm after 700 K annealing. The recoilless fractions can be fitted very well to a Debye model. On annealing. the characteristic Mössbauer temperature gradually decreases from 89 K to 64 K, the value for solid Kr at 1 bar. At the same time a decrease in the isomer shift is observed. Even after annealing at 700 K our experiments do not show melting in the temperature range 0–230 K.

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Authors and Affiliations

  1. Shanghai Institute of Nuclear Research, Academia Sinica, P.O. Box 8204, 201849, Shanghai, China

    G. L. Zhang

  2. Laboratorium voor Algemene Natuurkunde and Materials Science Center, Westersingel 34, 9718 CM, Groningen, the Netherlands

    L. Niesen

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  1. G. L. Zhang
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  2. L. Niesen
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Zhang, G.L., Niesen, L. High pressure of solid noble gases in metals. Hyperfine Interact 53, 253–272 (1990). https://doi.org/10.1007/BF02101051

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