Abstract
The spin dynamics of the muonium (Mu) atom diffusing quantum mechanically in solid nitrogen (s-14N2) has been studied using the technique of Mu spin relaxation. A strong relationship between longitudinal (T −11 ) and transverse (T −12 ) relaxation rates (familiar in NMR) has been experimentally demonstrated for the first time for muonium relaxation. At low temperatures the results are inconsistent with diffusion models using a single correlation timeτ c; this is taken as evidence for the intrinsic inhomogeneity of the problem. The temperature dependence of theaverage Mu hop rate τ −1c gives clear evidence that Mu quantum diffusion ins-N2 is governed by the two-phonon interaction.
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References
Yu. Kagan and N.V. Prokof'ev, “Quantum Tunneling Diffusion in Solids”, inModern Problems in Condensed Matter Science, eds. A.J. Leggett and Yu.M. Kagan (North-Holland, 1992).
P.C.E. Stamp and Chao Zhang,Phys. Rev. Lett. 66, 1902 (1991).
R. Kadono,Hyp. Int. 64, 615 (1990).
V. Storchaket al., Phys. Lett. A32, 77 (1992).
V. Storchaket al., to be published.
V. Storchaket al., Hyp. Int., to be published.
Yu. Kagan and N.V. Prokof'ev,Phys. Lett. A150, 320 (1990).
Yu. Kagan and N.V. Prokof'ev,Phys. Lett. A159, 289 (1991).
R.F. Kieflet al., Phys. Rev. Lett. 62, 792 (1989).
M. Celio,Helv. Phys. Acta. 60, 600 (1987); H.K. Yen, M. Sc. thesis, University of British Columbia, 1988 (unpublished).
C.P. Slichter,Principles of Magnetic Resonance (Springer-Verlag, 1980).
V. Storchaket al., Chem. Phys. Lett. 200, 546 (1992).
B.F. Kirillovet al., Hyperfine Int.65, 819 (1990).
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Storchak, V., Brewer, J.H., Hardy, W.N. et al. Inhomogeneous muonium diffusion in solid nitrogen. Hyperfine Interact 85, 103–108 (1994). https://doi.org/10.1007/BF02069409
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DOI: https://doi.org/10.1007/BF02069409