Skip to main content
Log in

Chemical and physical processes of radionuclide migration at Yucca Mountain, Nevada

  • Published:
Journal of Radioanalytical and Nuclear Chemistry Aims and scope Submit manuscript

Abstract

The understanding and prediction of radionuclide migration within the geosphere of a high-level radioactive waste repository requires knowledge of chemical and physical processes. In this paper, we present an overview of the investigations being performed at Los Alamos National Laboratory for the site characterization activites of the Yucca Mountain Project. The areas of investigation include: the determination of solubility concentration limits and chemical speciation for fission products and actinides; the collection of sorption data and understanding of sorption mechanisms; and the transport mechanism of advection, diffusion, and dispersion.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. G. de Marsily, E. Ledoux, A. Barbreau, J. Margat, Science, 197 (1977) 519.

    Google Scholar 

  2. Code of Federal Regulations, Title 10, Part 60, 1987, p. 627.

  3. Code of Federal Regulations, Title 40, Part 191, 1986, p. 7.

  4. G. de Marsily, Radiochim. Acta, 44/45 (1988) 159.

    Google Scholar 

  5. J.F. Kerrisk, Los Alamos National Laboratory Report LA-10414-MS, 1985.

  6. A.E. Ogard, J.F. Kerrisk, Los Alamos National Laboratory Report LA-10188-MS, 1984.

  7. J.K. Johnston, R.R. Peters, P.F. Gnirk, Sandia National Laboratory Report SAND 83-0372, 1984.

  8. D.B. Tucker, E.M. Standifer, H. Nitsche, R.J. Silva, Lanthanide and Actinide Res., 2 (1988) 279.

    Google Scholar 

  9. D.E. Hobart, P.D. Palmer, T.W. Newton, Los Alamos National Laboratory Report LA-UR-89-968, 1986.

  10. D.E. Hobart, D.E. Morris, D.D. Palmer, T.W. Newton, Proc. Topical Meeting on Nuclear Waste Isolation in the Unsaturated Zone: FOCUS'89, 1989.

  11. T.J. Wolery, Lawrence Livermore National Laboratory Report UCRL-51, 1984.

  12. K.W. Thomas, Los Alamos National Laboratory Report LA-10960-MS, 1987.

  13. W.R. Daniels, K. Wolfsberg, R.S. Rundberg, A.E. Ogard, et al., Los Alamos National Laboratory Report LA-9328-MS, 1982.

  14. J.M.M. Morel P.M. Gschwend, Aquat. Surf. Chem., (1987) 405.

  15. H. Nitsche, E.M. Standifer, S.C. Lee, R.C. Gatti, D.B. Tucker, Lawrence Berkeley Laboratory Report LBL-27157, 1987.

  16. R.S. Rundberg, Los Alamos National Laboratory Report LA-11026-MS, 1987.

  17. G. Sposito, The Thermodynamics of Soil Solutions, Oxford Clarendon Press, New York, 1987.

    Google Scholar 

  18. R.S. Rundberg, Scientific Basis of Nuclear Waste Management VIII, 26, Nort-Holland, New York, 1984, p. 827.

    Google Scholar 

  19. A.L. Sanchez, J.W. Murray, T.H. Sibley, Geochim. Cosmochim. Acta, 49 (1985) 2297.

    Article  Google Scholar 

  20. T.K. Sherwood, R.L. Pigford, C.R. Wilke, Mass Transfer, McGraw-Hill, New York, 1975.

    Google Scholar 

  21. J. Bear, Hydraulics of Groundwater, McGraw-Hill, New York, 1979.

    Google Scholar 

  22. G. Matherson, G. de Marsily, Water Resources Res., 16 (1980) 901.

    Google Scholar 

  23. L.W. Gelher, A.L. Gutjahr, R.L. Naff, Water Resource Res., 15 (1979) 1387.

    Google Scholar 

  24. S.P. Neumann, C.L. Winter, C.M. Newman, Water Resource Res., 23 (1987) 453.

    Google Scholar 

  25. B.B. Mandelbrst, The Fractal Geometry of Nature, W.H. Freedman and Company, New York, 1977.

    Google Scholar 

  26. W.K. Hiester, T. Vermeulen, Chem. Eng. Prog., 48 (1952) 505.

    Google Scholar 

  27. E. Glueckauf, J.I. Coates, J. Chem. Soc., (1947) 1315.

  28. J.L. Thompson, J. Radioanal. Nucl. Chem., 130 (1989) 353.

    Google Scholar 

  29. J. Bear, Y. Bachmat, Int. Ass. Sci. Hydrol. Publ., 72 (1967).

  30. A. Dieulin, G. Matherson, G. de Marsily, The Science of the Total Environment, 21 (1981) 319.

    Article  Google Scholar 

  31. A.E. Ogard, J.L. Thompson, R.S. Rundberg, K. Wolfsberg, P.W. Kubik, D. Elmore, H.W. Bentley, Radiochim. Acta, 44/45 (1988) 213.

    Google Scholar 

  32. I. Neretnicks, J. Geophys. Res., 85 (1980) 4379.

    Google Scholar 

  33. P.H. Tang, E.O. Frind, E.A. Sudicky, Water Resource Res., 17 (1981) 555.

    Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Additional information

This work was supported by the Yucca Mountain Project Office as part of the Civilian Radioactive Waste Management Program. This project is managed by the U.S. Department of Energy, Nevada Operations Office.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Patera, E.S., Hobart, D.E., Meijer, A. et al. Chemical and physical processes of radionuclide migration at Yucca Mountain, Nevada. Journal of Radioanalytical and Nuclear Chemistry, Articles 142, 331–347 (1990). https://doi.org/10.1007/BF02039472

Download citation

  • Received:

  • Issue Date:

  • DOI: https://doi.org/10.1007/BF02039472

Keywords

Navigation