Abstract
The problem of the self-trapping of the Frenkel exciton interacting with phonons is considered in the adiabatic approximation. The self-trapping is assumed to take place at a single site. The exciton scattering by phonons at this site and the nearest neighbouring sites is taken into account. Analytical expressions for the adiabatic surface of self-trapping excitons, in particular, for the barrier height separating almost free and self-trapped states, are found. The condition for the applicability of the model to the describing of the self-trapping barrier is determined. The adiabatic surface is shown to have several minima separated by a barrier, i.e. the coexistence of several types of self-trapped excitons is possible.
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Dedicated to Professor Miroslav Trlifaj on the occasion of his sixtieth birthday.
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Hizhnyakov, V.V., Sherman, A.V. Adiabatic surface of self-trapping excitons. Czech J Phys 32, 58–68 (1982). https://doi.org/10.1007/BF01597546
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DOI: https://doi.org/10.1007/BF01597546