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Nonlinear spectroscopy in an intense Markov field

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Radiophysics and Quantum Electronics Aims and scope

Conclusion

To sum up, it is first necessary to note that the stochastic nature of the fundamental wave field is manifested in the spectral line broadening of the susceptibility, whose width is formulated as a sum of spectral widths due to thermal relaxation and noise: 1/T2 + 1/τ0, in agreement with experiment [41], where the broadening of the spectral dependence of the third harmonic intensity was fixed.

Although the transformation coefficient in a phase-modulated field is always smaller than for monochromatic pumping, for wide-band excitation the saturation intensity increases:\(\tilde J_s = J_s /\sqrt {q_2 } \), which removes the saturation boundary toward higher intensities.

In an amplitude-modulated pumping field the transformation coefficient into harmonics exceeds that calculated for monochromatic excitation, and increases with the parameter q1. This is confirmed by the results of [57, 120, 152], showing that the effectiveness of nonlinear processes in a noisy field is higher than for regular pumping.

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Zaporozhskii Industrial Institute. Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Radiofizika, Vol. 26, No. 6, pp. 698–740, June, 1983.

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Oseledchik, Y.S., Burshtein, A.I. Nonlinear spectroscopy in an intense Markov field. Radiophys Quantum Electron 26, 514–549 (1983). https://doi.org/10.1007/BF01033699

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