This is a preview of subscription content, log in via an institution to check access.
Literature cited
N. R. Isenor, V. Merchant, R. S. Hallsworth, and M. C. Richardson, “CO2 laser induces dissociation of SiF4 molecules into electronically excited fragments,“ Can. J. Phys.,51, 1281–1290 (1973).
R. V. Ambartsumyan, V. S. Letokhov, E. A. Ryabov, and N. V. Chekalin, “Isoptopically selective chemical reaction of BCl3 molecules in a strong infrared laser field,” Pis'ma Zh. Ekps. Teor. Fiz.,20, 597–600 (1974).
R. V. Ambartsumiyan, Yu. A. Gorokhov, V. S. Letokhov, and G. N. Makarov, “Separation of sulfur isotopes with enrichment factor >103 with action of CO2 laser radiation on SF6 molecules,” Pis'ma Zh. Eksp. Teor. Fiz.,21, 375–378 (1975).
S. S. Alimpiev, N. V. Karlov, B. B. Krynetskii, and Yu. N. Petrov, Laser Isotope Separation [in Russian], VINITI, Moscow (1980), Pt. 1, pp. 86–134.
N. G. Basov, A. N. Oraevskii, and A. V. Pankratov, “Kinetics of laser-chemical reactions,” Kvantovaya Elektron.,3, 814–822 (1976).
V. N. Panfilov and Yu. N. Molin, “Infrared photochemistry,” Usp. Khim.,47, No. 6, 967–991 (1978).
V. N. Bagratashvili, V. S. Letokhov, A. A. Makarov, and E. A. Ryabov, Multiphoton Processes in Molecules in an Infrared Laser Field [in Russian], VINITI, Moscow (1980–1981).
V. S. Letokhov and A. A. Makarov, “Polyatomic molecules in a strong infrared field,” Usp. Fiz. Nauk,134, 45–91 (1981).
V. M. Akulin, S. S. Alimpiev, N. V. Karlov, et al., “Mechanism of collisionless dissociation of polyatomic molecules,” Tr. FIAN,114, 107–138 (1979).
B. I. Stepanov, Luminescence of Complex Molecules [in Russian], Izd. Akad. Nauk BSSR, Minsk (1955).
B. I. Stepanov and V. P. Gribkovskii, Introduction to the Theory of Luminescence [in Russian], Izd. Akad. Nauk BSSR, Minsk (1963).
N. A. Borisevich, Excited States of Complex Molecules in the Gas Phase [in Russian], Nauka i Tekhnika, Minsk (1967).
V. T. Galochkin and A. N. Oraevskii, “Characteristics of molecular absorption of intense IR radiation (Review),” Kvantovaya Elektron.,6, 885–901 (1979).
A. N. Oraevskii and V. A. Sawa, “Excitation of oscillations of molecules by a laser and by chemical reactions,” Kr. soobshch. po fizike, FIAN, No. 7, 50–55 (1970).
Z. Bialynicka-Birula, I. Bialynicki-Birula, J. H. Eberly, and B. W. Shore, “Coherent dynamics of N-level atoms and molecules. II. Analytic solutions,” Phys. Rev. A,16, 2048–2054 (1977).
G. K. Paramonov and V. A. Savva, “Excitation of multilevel systems by quasiresonant monochromatic radiation,” Preprint No. 223, Inst. Fiz. Akad. Nauk BSSR, Minsk (1980).
A. A. Makarov, “Coherent excitation of equidistant multilevel systems in a resonant monochromatic field,” Zh. Eksp. Teor. Fiz.,72, 1749–1761 (1977).
G. K. Paramonov and V. A. Savva, “Quasiresonant excitation of multilevel systems by monochromatic radiation,” Zh. Prikl. Spektrosk.,33, 56–63 (1980).
R. V. Ambartsumyan, Yu. A. Gorokhov, V. S. Letokhov, et al., “Explanation of selective dissociation of SF6 molecules in a strong IR laser field,” Pis'ma Zh. Eksp. Teor. Fiz.,23, 26–30 (1976).
M. V. Kuz'min, “Dynamics of multiphoton excitation of oscillations in molecules,” Kvantovaya Elektron.,5, 759–764 (1978).
M. V. Kuz'min and V. N. Sazonov, “Model of radiative dissociation of polyatomic molecules,” Kvantovaya Elektron.,6, 539–547 (1979).
V. M. Akulin, “Action of laser radiation on band-type multilevel systems,” Tr. FIAN,114, 60–89 (1979).
A. A. Makarov, V. T. Platonenko, and V. V. Tyakht, “Interaction of a quantum ‘levelband’ system with quasiresonant monochromatic field,” Zh. Eksp. Teor. Fiz.,75, 2075–2091 (1978).
I. I. Knyazev and V. V. Lobko, “Investigation of molecular absorption in a wide range of intensity of infrared laser radiation,” Zh. Eksp. Teor. Fiz.,77, 816–828 (1979).
G. K. Paramonov and V. A. Savva, “Formation of hot and cold ensembles with radiative excitation of particles with degenerate energy levels,” Zh. Prikl. Spektrosk.,36, 624–631 (1982).
G. K. Paramonov and V. A. Sawa, “Resonant laser excitation of equidistant system of doubly degenerate levels,” Dokl. Akad. Nauk BSSR,25, 24–27 (1981).
J. D. Stettler, C. M. Bowder, N. M. Witron, and J. H. Eberly, “Population trapping during laser induced molecular excitations and dissociation,” Phys. Lett. A,73, 171–174 (1979).
G. K. Paramonov and V. A. Savva, “Coherent excitation of quantum systems with degenerate energy levels,” Preprint No. 240, Inst. Fiz. Akad. Nauk BSSR, Minsk (1981).
V. P. Makarov and M. V. Federov, “Rotational spectrum of diatomic molecules in an intense electromagnetic radiation field,” Zh. Eksp. Teor. Fiz.,70, 1185–1196 (1976).
M. V. Fedorov, “Vibrational-rotational spectra and the process of excitation of a molecule in the field of an intense resonant wave,” Zh. Eksp. Teor. Fiz.,73, 134–145 (1977).
H. Beitmen and A. Erdelyi, Higher Transcendental Functions [Russian translation], Nauka, Moscow (1974), Vol. II, pp. 223–224.
R. V. Ambartzumian, V. S. Letokhov, G. N. Makarov, and A. A. Puretzkii, “Characteristics of multiphoton dissociation of OsO4. molecule by two-frequency tunable CO2 laser pulses,” Opt. Commun.,25, 69–73 (1978).
V. N. Bagratashvili, V. S. Dolzhikov, and V. S. Letokhov, “Kinetics of IR absorption spectra by SF6 molecules vibrationally excited by a powerful pulsed CO2 laser,” Zh. Eksp. Teor. Fiz.,76, 18–25 (1979).
Additional information
Written at the request of the editorial board in connection with the 60th anniversary of the formation of the USSR.
Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 38, No. 1, pp. 76–87, January, 1983.
Rights and permissions
About this article
Cite this article
Samson, A.M., Savva, V.A. & Paramonov, G.K. Role of coherence in multiquantum excitation of molecules by IR laser radiation. J Appl Spectrosc 38, 63–72 (1983). https://doi.org/10.1007/BF00659860
Received:
Issue Date:
DOI: https://doi.org/10.1007/BF00659860