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Stimulated emission of mixed molecular crystals and its use for investigation of relaxation processes

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Literature cited

  1. T. J. Aartsma and D. A. Wiersma, “Photon-echo spectroscopy of organic mixed crystals,” Phys. Rev. Lett.,36, No. 23, 1360–1362 (1976).

    Google Scholar 

  2. T. J. Aartsma and D. A. Wiersma, “Coherent optical phenomena in organic mixed crystals,” Opt. Commun.,18, No. 2, 201–202 (1976).

    Google Scholar 

  3. D. E. Cooper, R. W. Olson, R. D. Wilting, et al., “Picosecond time scale optical coherence experiments in mixed molecular crystals: pentacene in naphthalene,” Chem. Phys. Lett.,67, No. 1, 41–47 (1979).

    Google Scholar 

  4. W. H. Hesselink and D. A. Wiersma, “Picosecond dephasing and relaxation on molecular vibrational states in condensed phase,” Chem. Phys. Lett.,65, No. 2, 300–303 (1979).

    Google Scholar 

  5. R. H. Dicke, “Coherence in spontaneous processes,” Phys. Rev.,93, 99–120 (1954).

    Google Scholar 

  6. J. C. MacGillivray and M. S. Zeld, “Superradiance in atoms and molecules, ” in: Use of Lasers in Atomic, Molecular, and Nuclear Physics. Proceedings of First All-Union School, Vilnius, 1978, Moscow (1979), pp. 117–130.

  7. A. S. Davydov, Theory of Molecular Excitons [in Russian], Nauka, Moscow (1968).

    Google Scholar 

  8. A. I. Kitaigorodskii, Organic Crystal Chemistry [in Russian], Akad. Nauk SSSR, Moscow (1955).

    Google Scholar 

  9. Yu. V. Naboikin and L. A. Ogurtsova, “Stimulated emission of mixed molecular crystals at low temperatures,” Zh. Prikl. Spektrosk.,31, No. 2, 189–204 (1979).

    Google Scholar 

  10. Yu. V. Naboikin, L. A. Ogurtsova, A. P. Podgornyi, et al., “Light generation by mixed molecular crystals at 4.2°K,” Kvantovaya Élektron.,5, No. 4, 795–803 (1978).

    Google Scholar 

  11. N. A. Aleksandrovskaya, V. K. Dobrokhotova, Yu. V. Naboikin, et al., “Features of luminescence of mixed molecular crystals in relation to structure of impurity center,” Ukr. Fiz. Zh.,22, No. 4, 575–784 (1977).

    Google Scholar 

  12. V. K. Dobrokhotova, V. S. Gorobchenko, Yu. V. Naboikin, et al., “Features of stimulated emission of mixed molecular crystals,” Opt. Spektrosk.,38, No. 3, 579–582 (1975).

    Google Scholar 

  13. Yu. V. Naboikin, L. A. Ogurtsova, A. P. Podgornyi, et al., “Determination of relaxation times of ground-state vibrational levels of mixed molecular crystals,” J. Lumines.,17, 367–374 (1978).

    Google Scholar 

  14. Yu. V. Naboikin, L. A. Ogurtsova, A. P. Podgornyi, et al., “Effect of lifetime of groundstate vibrational levels on development of stimulated emission of molecular crystals,” Zh. Prikl. Spektrosk.,25, No. 1, 59–62 (1976).

    Google Scholar 

  15. Yu. V. Naboikin, L. A. Ogurtsova, A. P. Podgornyi, et al., “Determination of relaxation time of ground-state vibrational levels of molecular crystals,“Zh. Prikl. Spektrosk.,27, No. 4, 675–680 (1977).

    Google Scholar 

  16. Yu. V. Naboikin, “Organic crystals at low temperatures — new materials for quantum electronics,” in: All-Union Conference on Organic Luminophors (Kharkov, September 15–17, 1976). Abstracts of Papers [in Russian], Kharkov (1977), pp. 37–38.

  17. A. Bree and V. V. B. Vilkos, “A study of some singlet and triplet electronic states of pyrene,“ Spectrochim. Acta,27a, No. 11, 2333–2354 (1971).

    Google Scholar 

  18. P. V. Zinov'ev, Yu. V. Naboikin, L. A. Ogurtsova, et al., “Use of polarization characteristics of luminescence of pyrene in diphenyl crystals to obtain stimulated emission on 0-0 transition frequency,” Ukr. Fiz. Zh.,24, No. 1, 122–124 (1979).

    Google Scholar 

  19. P. V. Zinov'ev, Yu. V. Naboikin, and N. B. Silaeva, “Stimulated emission on 0-0 transition of pyrene in diphenyl crystals at 4.2°K,” Pis'ma Zh. Tekh. Fiz.,5, No. 2, 80–82.

  20. V. A. Kovarskii, E. A. Popov, and I. A. Chaikovskii, “Radiative and nonradiative transitions of electrons in local centers involving hot phonons,” Phys. Status Solidi B,67, 427–433 (1975).

    Google Scholar 

  21. V. A. Kovarskii, “Multiquantum transitions in local centers of crystals in a strong electromagnetic field,” Izv. Akad. Nauk SSSR, Ser. Fiz.,40, 1879–1885 (1976).

    Google Scholar 

  22. A. V. Akimov, S. A. Basun, A. A. Kaplyanskii, et al., “Effect of heat pulses on fluorescence of organic impurity molecules in crystalline n-paraffin matrices,” Fiz. Tverd. Tela,20, No. 1, 220–227 (1978).

    Google Scholar 

  23. A. V. Belousov, V. A. Kovarskii, and É. P. Sinyavskii, “Properties of light absorption by a quantum system interacting with nonequilibrium phonons,” Fiz. Tverd. Tela,20, 205–210 (1978).

    Google Scholar 

  24. I. B. Levinson, “Distribution of hot phonons generated by laser emission,” Zh. Éksp. Teor. Fiz.,65., No. 1 (7), 331–341 (1973).

    Google Scholar 

  25. V. I. Emel'yanov, “Spatial and temporal oscillations of stimulated Raman scattering in saturated optical phonon generation,” Fiz. Tverd. Tela,20, No. 2, 439–443 (1978).

    Google Scholar 

  26. M. J. Colles and J. A. Giordmaine, “Generation and detection of large-k-vector phonons,” Phys. Rev. Lett.,27, No. 10, 670–674 (1971).

    Google Scholar 

  27. V. L. Broude, I. A. Vidmont, V. V. Korshunov, et al., “Propagation of nonequilibrium phonons in anthracene crystals at low temperatures,” Pis'ma Zh. Éksp. Teor. Fiz.,25, No. 6, 285–288 (1977).

    Google Scholar 

  28. V. L. Broude, I. A. Vidmont, D. V. Kazakovtsev, et al., “Excitation and propagation of phonons in anthracene crystals,” Zh. Éksp. Teor. Fiz.,74, No. 1, 314–327 (1978).

    Google Scholar 

  29. V. S. Bagachev, L. V. Keldysh, N. N. Sibel'din, et al., “Entrainment of excitons and electron-hole drops by phonon wind,” Zh. Éksp. Teor. Fiz.,70, No. 2, 702–716 (1976).

    Google Scholar 

  30. E. D. Vol, Yu. V. Naboikin, L. A. Ogurtsova, et al., “Features of stimulated emission of ββ-dinaphthylethylene in naphthalene at 4.2°K,” Izv. Akad. Nauk SSSR, Ser. Fiz.,39, No. 9, 1908–1912 (1975).

    Google Scholar 

  31. E. D. Vol, Yu. V. Naboikin, L. A. Ogurtsova, et al., “Possible effect of phonons on stimulated emission of mixed molecular crystals,” Kvantovaya Élektron.,3, No. 6, 1313–1319 (1976).

    Google Scholar 

  32. É. L. Bokhenkov, I. Natkanets, and É. R. Sheka, “Determination of density of phonon states in naphthalene crystals from inelastic incoherent neutron scattering,” Zh. Éksp. Teor. Fiz.,70, No. 3, 1027–1043 (1976).

    Google Scholar 

  33. Q. S. Pawley, “A model for the lattice dynamics of naphthalene and anthracene,” Phys. Status Solidi,20, 347–360 (1967).

    Google Scholar 

  34. Yu. V. Naboikin, L. A. Ogurtsova, and A. P. Podgornyi, “Role of nonequilibrium phonons in development of stimulated emission of mixed molecular crystals,” Fiz. Tverd. Tela,22, No. 2, 447–452 (1979).

    Google Scholar 

  35. V. A. Goloyadov, V. S. Gorobchenko, S. V. Lopina, et al., “Excitation of nonequilibrium phonons in a mixed molecular crystal by ultrashort light pulses,” Ukr. Fiz. Zh.,24, No. 1, 124–125 (1979).

    Google Scholar 

  36. M. A. Krivoglaz, “Theory of inelastic neutron scattering by imperfect crystals,” Zh. Éksp. Teor. Fiz.,40, No. 2, 567–584 (1961).

    Google Scholar 

  37. B. P. Nevzorov, Questions of Molecular Spectroscopy [in Russian], Nauka, Novosibirsk (1974).

    Google Scholar 

  38. P. V. Zinov'ev, Yu. V. Naboikin, L. A. Ogurtsova, et al., “Suppression of light generation on phonon wing in naphthalene crystal containing ββ-dinaphthylethylene by a resonant-frequency field, ” Kvantovaya Élektron.,4, No. 4, 899–901 (1974).

    Google Scholar 

  39. V. K. Dobrokhotova, Yu. V. Naboikin, L. A. Ogurtsova, et al., “Stimulated emission on forbidden triplet-singlet transitions of mixed molecular crystals,” Pis'ma Zh. Tekh. Fiz.,6, No. 9, 538–540 (1980).

    Google Scholar 

  40. S. G. Rautian and I. I. Sobel'man, “Questions of negative absorption,” Opt. Spektrosk.,10, No. 1, 134–135 (1961).

    Google Scholar 

  41. E. Q. Brock, P. Csavinsky, E. Hormats, et al., “Coherent stimulated emission from organic molecular crystals,” J. Chem. Phys.,35, No. 2, 759–760 (1961).

    Google Scholar 

  42. Yu. V. Naboikin, L. A. Ogurtsova, and I. D. Fil', “Emission spectra and luminescence kinetics of organic molecules in conditions of reabsorption on triplet-triplet transitions,” Opt. Spektrosk.,20, No. 1, 53–57 (1966).

    Google Scholar 

  43. Yu. V. Naboikin, L. A. Ogurtsova, and I. D. Fil', “Reabsorption of emission on excited levels and possibility of light generation,” in: Quantum Electronics [in Russian], Naukova Dumka, Kiev (1966), pp. 183–187.

    Google Scholar 

  44. Yu. V. Naboikin, L. A. Ogurtsova, and I. D. Fil', “Possibility of obtaining induced emission in conditions of reabsorption on triplet-triplet transitions,” Zh. Prikl. Spektrosk.,6, No. 4, 538–540 (1967).

    Google Scholar 

  45. S. N. Singh, M. G. Jayswall, R. S. Sing, et al., “Triplet-singlet emission spectrum of acenaphthenequinone vapours,” Bull. Chem. Soc. Jpn.,42, No. 7, 2048–2050 (1969).

    Google Scholar 

  46. Electromagnetic Superradiance [in Russian], Kazanskii Fiziko-Tekhnicheskoi Institut, Kazan (1975).

  47. P. V. Zinov'ev, Yu. V. Naboikin, and N. B. Silaeva, “Observation of self-induced transparency in a pyrene-containing diphenyl crystal under nonresonant excitation,” Pis'ma Zh. Tekh. Fiz.,5, No. 2, 77–79 (1979).

    Google Scholar 

  48. P. V. Zinov'ev, G. G. Zaitseva, Yu. V. Naboikin, et al., “Self-induced transparency in pyrene-containing diphenyl crystal excited by its own stimulated emission,” Zh. Éksp. Teor. Fiz.,77, No. 4 (10), 1519–1527 (1979).

    Google Scholar 

  49. P. V. Zinov'ev, Yu. V. Naboikin, and N. B. Silaeva, “Effect of coherent processes on spectrum and kinetics of emission of a pyrene-containing diphenyl crystal at 4.2-1.2°K,” Izv. Akad. Nauk SSSR, Ser. Fiz.,44, No. 4, 780–782 (1980).

    Google Scholar 

  50. V. S. Gorobchenko, Yu. V. Naboikin, and L. A. Ogurtsova, “Possible observation of superradiance on vibrational transitions of complex organic molecules,” Ukr. Fiz. Zh.,25, No. 10, 1736–1738 (1980).

    Google Scholar 

  51. V. A. Goloyadov, S. V. Lopina, and I. A. Rom-Krichevskaya, “Stimulated emission of subnanosecond duration from impure naphthalene crystals excited by ultrashort laser pulses,” Ukr. Fiz. Zh.,21, No. 2, 215–217 (1976).

    Google Scholar 

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Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 34, No. 6, pp. 1036–1051, June, 1981.

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Naboikin, Y.V., Ogurtsova, L.A. Stimulated emission of mixed molecular crystals and its use for investigation of relaxation processes. J Appl Spectrosc 34, 637–650 (1981). https://doi.org/10.1007/BF00618279

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