Abstract
Most acid-deposition investigations have been concerned with the impact of nitrogen oxides (NOx) and sulfur dioxide (SO2) emissions on Europe and North America. This paper examines three issues beyond this central focus. Major conclusions are 1) ammonia (NH3) emissions and subsequent nitrogen (N) accumulation in terrestrial ecosystems have the potential to generate significant acidification in terrestrial and aquatic ecosystems; 2) sulfur (S) and N accumulation in environmental reservoirs will not only result in significant and extensive acidification but will also impact the earth's radiation balance, tropospheric oxidizing capacity, ecosystem nutrient balance and groundwater quality; and 3) future emissions will substantially increase in the developing world, especially in Asia. By 2020, Asian emissions of SO2, NOx and NH3 will be equal to or greater than the combined emissions from Europe and North America.
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Aber, J. D., Nadelhoffer, K., Steudler, P., and Melillo, J. M.: 1989, Nitrogen saturation in northern forest ecosystems, Bioscience 39, 378–386.
ApSimon, H. M., Couling, S., Cowell, D., and Warren, R. F.: 1995, Reducing the contribution of ammonia to nitrogen deposition across Europe, Water, Air, and Soil Pollut., this volume.
Brimblecombe, P., Hammer, C., Rodhe, H., Ryaboshapko, A., and Boutron, C. F.: 1989, Human influence on the sulphur cycle, in Evolution of the Global Biogeochemical Sulphur Cycle, Brimblecombe, P., and Lein, A. Y. (eds.), John Wiley and Sons, Ltd. New York, 77–121
Cerny, J.: 1995, Recovery of acidified catchments in the extremely polluted Krusne Hory Mts., Czech Republic, Water, Air, and Soil Pollut., this volume.
Charlson, R. J., Langner, J., Rodhe, H., Leovy, C. B., and Warren, S. G.: 1991, Perturbation of the northern hemisphere radiative balance by backscattering from anthropogenic sulfate aerosols, Tellus 43 AB, 152–163.
Cowling, E. B.: 1982, Acid precipitation in historical perspective, Environ. Sci. & Tech. 16, 110A-123A.
Cowling, E. B., and Nilsson, J.: 1995, Acidification research: lessons from history and visions of possible futures, Water, Air, and Soil Pollut., this volume.
Dentener, F. J., and Crutzen, P. J.: 1994, A three-dimensional model of the global ammonia cycle, J. Atmos. Chem. 19, 331–369.
Esser, G., and Kohlmaier, G. H.: 1991, Modeling terrestrial sources of nitrogen, phosphorus, sulphur and organic carbon to rivers, in Biogeochemistry of Major Rivers, Degens, E. T., Kempe, S., and Richey J. E. (eds.), John Wiley & Sons, Ltd., New York, 297–322.
Galloway, J. N., and Rodhe, H.: 1991, Regional atmospheric budgets of S and N fluxes: How well can they be quantified?, Proc. R. Soc. Edinburgh 97B, 61–80.
Galloway, J. N., Norton, S. A., and Church, M. R.: 1983, Freshwater acidification from atmospheric deposition of sulfuric acid: A conceptual model, Environ. Sci. & Tech. 17, 541 A.
Galloway, J. N., Levy II, H., and Kasibhatla, P.S.: 1994, Year 2020: Consequences of population growth and development on deposition of oxidized nitrogen, Ambio 23, 120–123.
Galloway, J. N., Schlesinger, W. H., Levy II, H., Michaels, A., and Schnoor, J. L: 1995a, Nitrogen fixation: Anthropogenic enhancement-environmental response, Global Biogeochem. Cycles 9, 235–252.
Galloway, J. N., Keene, W. C., and Likens, G. E.: 1995b, The composition of precipitation at a remote southern hemispheric location: Torres del Paine National Park, Chile, J. Geophys. Res., in press.
Gorham, E.: 1992, Atmospheric deposition to lakes and its ecological effects: A retrospective and prospective view of research, Japanese J. Limnol. 53, 231–248.
Granath, A., Thunholm, B., and Aastrup, M.: 1995, Evaluation of groundwater chemical data from the National Swedish groundwater monitoring programmes, Water, Air and Soil Pollut., this volume.
Havas, M., and Rosseland, B. O.: 1995, Response of Zooplankton, benthos, and fish to acidification: an overview, Water, Air, and Soil Pollut., this volume.
Henriksen, A., Skjelkvale, B. L., and Lydersen, E.: 1995, Acidification in Norway-status and trends II. Surface and groundwater, Water, Air, and Soil Pollut., this volume.
Houghton, J. T., Callander, B. A., and Varney, S. K.: 1992, Climate Change 1992, The Supplementary Report to the IPCC Scientific Assessment, Intergovernmental Panel on Climate Change, Press Syndicate of University of Cambridge.
Ivanov, M. V., Grinenko, V. A., and Rabinovich, A. P.: 1983, Sulphur flux from continents to oceans, in The Biogeochemical Sulphur Cycle, Ivanov, M. V., and Freney, J. R. (eds.), John Wiley & Sons, Chichester, 331–356.
Hultberg, H.: 1995, Acid rain in a historical perspective, Water, Air, and Soil Pollut., this volume. Hutchinson, T. C.: 1995, Influence of acidification on the biodiversity of temperate forest ecosystems, Water, Air, and Soil Pollut., this volume.
Johnson, D. W., Hornbeck, J. W., Kelly, J. M., Swank, W. T., and Todd, D. E.: 1980, Regional patterns of soil sulfate accumulation: Relevance to ecosystem budgets, in Atmospheric Sulfur Deposition: Environmental Impacts and Health Effects, Shriner, D. S., Richmond, C. R., and Lindberg, W. E. (eds.), Ann Arbor Science, Ann Arbor, Michigan, 507–519.
Keller, M., Kaplan, W. A., and Wofsy, S. C.: 1986, Emissions of N2O, CH4, CO2 from tropical forest soils, J. Geophys. Res. 91, 11,791–11,802.
Krzyzanowski, M., and Lubkert-Alcamo, B.: 1995, Estimate of health effects of acidifying air pollutants and tropospheric ozone in Europe, Water, Air, and Soil Pollut. submitted
Kucera, V., and Fitz, S.: 1995, Direct and indirect air pollution effects on materials including cultural monuments, Water, Air, and Soil Pollut., this volume.
Likens, G. E., Keene, W. C., Miller, J. M., and Galloway, J. N.: 1987, Chemistry of precipitation from a remote, terrestrial site in Australia, J. Geophys. Res. 92, 13,299–13,314.
Mackenzie, F. T.: 1994, Global climatic change: Climatically important biogenic gases and feedbacks, in Biotic Feedbacks in the Global Climatic System: Will the Warming Feed the Warming?, Woodwell, G. M., and Mackenzie, F. T. (eds.), Oxford University Press, England, 22–46.
Matzner, E.: 1995, Regional air pollution effects on forests and forest soils, Water, Air, and Soil Pollut., this volume.
Michaels, A. F., Siegel, D. A., Johnson, R. J., Knap, A. H., and Galloway, J. N.: 1993, Episodic inputs of atmospheric nitrogen to the Sargasso Sea: Contributions to new production and phytoplankton blooms, Global Biogeochem. Cycles 7, 339–351.
Moody, J. L., Pszenny, A. A. P., Gaudry, A., Keene, W. C., Galloway, J. N., and Polian, G.: 1991, Precipitation composition and its variability in the southern Indian Ocean: Amsterdam Island, 1980–1987, J. Geophys. Res. 96, 20769–20786.
Nixon, S. W.: 1995, Coastal marine eutrophication: A definition, social causes, and future concerns, Ophelia 41, 199–219.
Owens, N. J. P., Galloway, J. N., and Duce, R. A.: 1992, Episodic atmospheric nitrogen deposition to oligotrophic oceans, Nature 357, 397–399.
Paerl, H. W., and Fogel, M. L.: 1994, Isotopic characterization of atmospheric nitrogen inputs as sources of enhanced primary production in coastal Atlantic Ocean waters, Marine Biology 119, 635–645.
Rodhe, H., and Herrera, R. (eds): 1988, Acidification in Tropical Countries, J. Wiley and Sons, Chichester.
Rodhe, H., Galloway, J., and Zhao, D.: 1992, Acidification in southeast Asia-Prospects for coming decades, Ambio 21, 148–149.
Rodhe, H., Gallardo, L., Kjellstrom, E., and Langner, J.: 1995, Global scale transport of acidifying pollutants, Water, Air, and Soil Pollut., this volume.
Sellden, G., and Pleijel, H.: 1995, Photochemical oxidant effects on vegetation, Water, Air, and Soil Pollut., this volume.
Summers, P. W. and Whelpdale, D. M.: 1995, The global distribution of acidic deposition, Water, Air, and Soil Pollut., this volume.
Verta, M. and Mannio, J.: 1995, How will acidification influence the effect of heavy metals?, Water, Air, and Soil Pollut., this volume.
von Bromssen, U.: 1989, National Swedish Environmental Protection Board Report 3547, NSEPB, Research Secretariat, Box 1302, S-171 25 Solna, Sweden.
Weiss, R. F.: 1981, The temporal and spatial distribution of tropospheric nitrous oxide, J. Geophys. Res. 86, 7185–7195.
Whelpdale, D. M., and Galloway, J. N.: 1994, Sulfur and reactive nitrogen oxide fluxes in the North Atlantic atmospheric, Global Biogeochem. Cycles 8, 481–493.
Wright, R. F., and Schindler, D. W.: 1995, Interaction of acid rain and global changes: effects on terrestrial and aquatic ecosystems, Water, Air, and Soil Pollut., this volume.
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Galloway, J.N. Acid deposition: Perspectives in time and space. Water Air Soil Pollut 85, 15–24 (1995). https://doi.org/10.1007/BF00483685
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DOI: https://doi.org/10.1007/BF00483685