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Phase measurements in surface nonlinear optics: The effect of laser beam quality

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Abstract

When the relative phase of a surface nonlinear polarizability is measured by interference techniques, the resultant interferogram may be of lower contrast than that expected for ideal waves. It is shown, both theoretically and experimentally that this degradation arises from the multimode character of the pulsed lasers used. Differences between longitudinal and transverse mode effects are demonstrated. The laser coherence time may be deduced from the fringe degradation caused by longitudinal modes.

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References

  1. Y.R. Shen: Nature 337, 519 (1989); Annu. Rev. Phys. Chem. 40, 327 (1989)

    Google Scholar 

  2. G.L. Richmond, J.M. Robinson, V.L. Shannon: Prog. Surf. Sci. 28, 1 (1988)

    Google Scholar 

  3. T.F. Heinz, M.M.T. Loy: Am. Inst. Phys. Conf. Proc. (Advances in Laser Science III) 172, 452 (1988)

    Google Scholar 

  4. J.H. Hunt, P. Guyot-Sionnest, Y.R. Shen: Chem. Phys. Lett. 133, 189 (1987)

    Google Scholar 

  5. A.L. Harris, C.E.D. Chidsey, N.J. Levinos, D.N. Loiacono: Chem. Phys. Lett. 141, 350 (1987)

    Google Scholar 

  6. J. Miragliotta, R.S. Polizzotti, P. Rabinowitz, S.D. Cameron, R.B. Hall: Chem. Phys. 143, 123 (1990)

    Google Scholar 

  7. C.V. Shank, R. Yen, C. Hirlimann: Phys. Rev. Lett. 51, 900 (1983)

    Google Scholar 

  8. H.M. Rojhantalab, G.L. Richmond: J. Phys. Chem. 93, 3269 (1989)

    Google Scholar 

  9. E.V. Sitzmann, K.B. Eisenthal: J. Phys. Chem. 92, 4579 (1988)

    Google Scholar 

  10. S.G. Grubb, M.W. Kim, Th. Rasing, Y.R. Shen: Langmuir 4, 452 (1988)

    Google Scholar 

  11. H.W.K. Tom, T.F. Heinz, Y.R. Shen: Phys. Rev. Lett. 51, 1983 (1983)

    Google Scholar 

  12. K. Kemnitz, K. Bhattacharyya, J.M. Hicks, G.R. Pinto, K.B. Eisenthal, T.F. Heinz: Chem. Phys. Lett. 131, 285 (1986)

    Google Scholar 

  13. G. Berkovic, Y.R. Shen, G. Marowsky, R. Steinhoff: J. Opt. Soc. Am. B 6, 205 (1989)

    Google Scholar 

  14. R.J.W. Hollering: J. Opt. Soc. Am. B 8, 374 (1991)

    Google Scholar 

  15. R. Superfine, J.Y. Huang, Y.R. Shen: Chem. Phys. Lett. 172, 303 (1990); Opt. Lett. 15, 1276 (1990)

    Google Scholar 

  16. J.Y. Huang, A. Lewis: Biophys. J. 55, 835 (1989)

    Google Scholar 

  17. G.A. Reider, M. Huemer, A.J. Schmidt: Opt. Commun. 68, 149 (1988)

    Google Scholar 

  18. D.A. Koos, G.L. Richmond: J. Chem. Phys. 93, 869 (1990)

    Google Scholar 

  19. G. Lupke, G. Marowsky, R. Steinhoff: Appl. Phys. B 49, 283 (1989)

    Google Scholar 

  20. R.K. Chang, J. Ducuing, N. Bloembergen: Phys. Rev. Lett. 15, 6 (1965)

    Google Scholar 

  21. A. Yariv: Quantum Electronics, 2nd edn. (Wiley, New York 1975) Chap. 6

    Google Scholar 

  22. A. Yariv: Optical Electronics, 3rd edn. (Holt, Rinehart and Wilson, New York 1985) Chap. 10

    Google Scholar 

  23. R.J. Collier, C.B. Burckhardt, L.H. Lin: Optical Holography (Academic, New York 1971) Chap. 7

    Google Scholar 

  24. N. Bloembergen, R.K. Chang, S.S. Jha, C.H. Lee: Phys. Rev. 174, 813 (1968)

    Google Scholar 

  25. G. Berkovic: Physica A 168, 140 (1990)

    Google Scholar 

  26. S. Yitzchaik, G. Berkovic, V. Krongauz: Chem. Mater. 2, 162 (1990)

    Google Scholar 

  27. This procedure was used in Ref. [19] (G. Marowsky: private communication)

    Google Scholar 

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Berkovic, G., Shvartsberg, E. Phase measurements in surface nonlinear optics: The effect of laser beam quality. Appl. Phys. B 53, 333–338 (1991). https://doi.org/10.1007/BF00331823

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