Abstract
Air pollution and atmospheric deposition by PCBs and organochlorine pesticides (isomers of HCH and p,p′-DDE) were studied at Paris from January 1986 to June 1987. The deposition measured as total (wet plus dry) was also followed during 1986 on two suburban and two rural sites. The distribution of the pollutants between the vapor phase and aerosols was evaluated by sampling air through a glass microfiber filter connected to a Tenax resin cartridge. The study shows that in the atmosphere as in waters of the catchment area of the Seine river, PCBs are the main organochlorine pollutants. Pollution by OCL is of the same order as the one described in literature (mean γ-HCH concentration 1.4 ng m−3) while PCB concentrations in the atmosphere are equal to or higher than those observed in USA and Europe (range 5 to 44 ng m−3). On the average, 93% of the PCBs are in the vapor phase with a composition approximating Aroclor 1242. In aerosols and precipitations the composition is closely related to Aroclor 1254. The total fallout for 1986 was 40 μg m−2 for PCBs and 20 μg m−2 for γ-HCH, rainfall being 611 mm.
Similar content being viewed by others
References
AFNOR: 1984, Prélèvement sur filtre des matières particulières en suspension dans l'air ambiant, Norme X 43-021, 6 pp.
Alencastro, L. F. and Tarradellas, J.: 1983, ‘Etude de la concentration en PCB des eaux usées dans les stations d'épuration’, Gaz-Eaux-Faux usées, 63° année, 3, 113.
Bidleman, T. F. and Olney, C. E.: 1974, Bull. Envir. Contam. Toxicol. 11, 442.
Bidleman, T. F.: 1981, Atmosph. Environment 15, 619.
Bidleman, T. F., Christensen, E., Billings, N., and Leonard, R.: 1981, J. Marine Res. 39, 443.
Billings, N. and Bidleman, T. F.: 1980, Environ. Sci. Technol. 14, 679.
Billings, N. and Bidleman, T. F.: 1983, Atmosph. Environment 17, 383.
Chevreuil, M., Chesterikoff, A., and Létolle, R.: 1987a, ‘Evaluation de la répartition particulaire/aqueuse des PCB (polychlorobiphényles) en Seine’, C.R. Acad. Sci. Paris, 304, Série II, n° 9.
Chevreuil, M., Chesterikoff, A., and Létolle, R.: 1987b, Water Res. 21, 427.
Doskey, P. and Andren, A.: 1981a, J. Great Lakes Res. 7, 15.
Doskey, P. and Andren, A.: 1981b, Environ. Sci. Technol. 15, 705.
Duce, R. and Duursma, E.: 1977, Marine Chemistry 5, 319.
Duce, R., Mohnen, V., Zimmerman, P., Grosjean, D., Cautreels, W., Chatfield, R., Jaenicke, R., Ogren, J., Pellizzari, E., and Wallace, G.: 1983, Rev. Geophys. Space Physics 21, 921.
Eisenreich, S., Looney, B., and Thornton, J.: 1980, Assessment of Airbone Organic Contaminants in the Great Lakes Ecosystem, Science Advisory Board, IJC, Windsor, Ontario.
Eisenrcich, S., Looney, B., and Thornton, J.: 1981, Environ. Sci. Technol. 15, 30.
Giam, C., Atlas, E., Chan, H., and Neff, G.: 1980, Atmosph. Environment 14, 65.
Handa, N.: 1977, Marine Chemistry 5, 341.
Harvey, G. and Steinhauer, W.: 1974, Atmosph. Environment 8, 777.
Horzempa, L. and Di Toro, D.: 1983, Water Res. 17, 851.
Larsson, P.: 1985, Nature 317, 347.
Marchand, M.: 1985, ‘Processus géochimiques d'apports et de distribution des polluants organiques dans l'environnement marin. Etude appliquée aux hydrocarbures et aux hydrocarbures halogénés’, Thèse Doct. ès Sciences, Univ. Paris VI, 22 november 1985, 309 pp.
Mazzone, S. and Nicaud, S.: 1987, Importance de l'échantillonnage dans l'étude de la pollution des sols par les micro polluants organiques, Rapport de recherche 3ème cycle, Ecole Polytechnique Fédérale de Lausanne, 76 pp.
Murphy, T. and Rzeszutko, C.: 1977, J. Great Lakes Res. 3, 305.
Olier, J. P.: 1987, Quatre conférences sur les PCB, Rapport du Ministère de l'Environnement, Service de l'Environnement Industriel.
OMS: 1978, Polychlorobiphényles et polychloroterphényles. Critères d'Hygiène de l'Environnement, 2, Genève, 93 pp.
Simon, S.: 1984, Note sur la contamination par les PCB dans l'estuaire de la Seine et son bassin versant, Extrait du rapport annuel de la Cellule Antipollution de Rouen, Service de la Navigation de la Seine, 4ème section.
Södergren, A.: 1972, Nature (Lond.) 236, 395.
Strachan, W.: 1979, J. Great Lakes Res. 5, 61.
Thomas, W.: 1984, Water, Air, and Soil Pollut. 22, 351.
Thomas, W.: 1986, Atmosph. Environment 20, 995.
Wescot, J. and Bidleman, T.: 1981, J. Chromat. 210, 331.
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Chevreuil, M., Chesterikoff, A., Létolle, R. et al. Atmospheric pollution and fallout by PCBS and organochlorine pesticides (Ile-De-France). Water Air Soil Pollut 43, 73–83 (1989). https://doi.org/10.1007/BF00175584
Received:
Revised:
Issue Date:
DOI: https://doi.org/10.1007/BF00175584