Skip to main content
Log in

An intensive 1-month investigation of trace metal deposition and throughfall at a mountain spruce forest

  • Published:
Water, Air, and Soil Pollution Aims and scope Submit manuscript

Abstract

During July 1986, atmospheric concentrations and deposition rates of Ph, Cd, Zn, and Mn were measured at a spruce forest in the Great Smoky Mountains National Park, and meteorological data were recorded. Precipitation, cloud water impaction, and dry deposition were quantified. Average total fluxes of 12, 1.0, 53, and 40 µg m−2 d−1 for Pb, Cd, Zn, and Mn, respectively, were measured; dry deposition constituted 46, 32, 62 and 66% of each of the totals. Cloud impaction (unusually low for this particular month) was measurable but not quantitatively important. Dry deposited Pb and Zn were washed from the canopy by subsequent rainfall — revealing greater throughfall fluxes associated with increasing antecedent dry period durations. Cadmium and Mn did not, however, show this relationship. Measurements revealed little interaction of Cd with the forest canopy, while considerable net leaching of Mn was evident (as had been expected). The canopy behaviors of both Pb (i.e., leaching) and Zn (i.e., uptake) were contrary to expectations.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  • Bondietti, E. A., Hoffman, P. O., and Larsen, I. L.: 1984, J. Envir. Radioact. 1, 5.

    Google Scholar 

  • Coe, J. M. and Lindberg, S. E.: 1987, J. Air Pollut. Control Assoc., 37, 237.

    Google Scholar 

  • Davidson, C. I., Goold, W. D., Mathlson, T. P., Wiersma, G. B., Brown, K. W., and Michael, T.: 1985, Environ. Sci. and Technol. 19, 27.

    Google Scholar 

  • Elias, R. W.: 1986, ‘Effects of Lead on Ecosystems, in Air Quality Criteria for Lead, EPA-600/8–83/028aF, U.S. Environ. Protection Agency, Research Triangle Park, N.C.

    Google Scholar 

  • Falconer, R. and Falconer, R.: 1980, J. Geophys. Res. 85, 7465.

    Google Scholar 

  • Hicks, B. B., Wesley, M. L., Lindberg, S. E., and Bromberg, S. M. (eds.): 1986, Proceedings of the Dry Deposition Workshop of the National Acid Precipitation Assessment Program, March 25–37, 1986, NOAA/ATDD, P.O. Box 2456, Oak Ridge, TN 37831.

  • Johnson, D. W., Lindberg, S. E., Bondietti, E. A., Cole, D. W., Lovett, G. M., Mitchell, M., Ragsdale, L. H., and Pitelka, L. F.: 1987, Paper 87-34.4 in Proc. Air Pollut. Control. Assoc. Annual Meeting, New York, June 21–26, 1987.

  • Johnson, A. H . and Siccama, T. G.: 1983, Envir. Sci. Technol. 17, 294A.

    Google Scholar 

  • Lindberg, S. E. and Harriss, R. C.: 1983, Jour. Geophys. Res. 88, 5091–5100.

    Google Scholar 

  • Lindberg, S. E.: 1989, ‘Behavior of Cd, Mn, and Pb in Forest Canopy Throughfall’, in Control and Fate of Atmospheric Trace Metals, J. Pacyna and B. Ottar (eds.), NATO ASI Series 268, Kluwer Publ.

  • Lindberg, S. E., Lovett, G. M., Richter, D. R., and Johnson, D. W.: 1986, Science 231, 141.

    Google Scholar 

  • Lindberg, S. E. and Turner, R. R.: 1988, Water, Air, and Soil Pollut. 39, 123.

    Google Scholar 

  • Lindberg, S. E., Silsbee, D., Schaefer, D. A., O0wens, J. G., and Petty, W.: 1988a, pp. 321–344 in Processes of Acidic Deposition in Mountainous Terrain, M. Unsworth and D. E. Fowler (eds.), Kluwer Academic Publishers, London.

    Google Scholar 

  • Lindberg, S. E., Lovett, G. M., Schaefer, D. A., and Bredemeier, M.: 1988b, J. Aerosol Sci. 19, 1187.

    Google Scholar 

  • Lindberg, S. E. and Johnson, D. W. (eds.): 1989, 1988 Annual Report of the Integrated Forest Study, ORNL/TM 11121, Oak Ridge National Lab. (in press).

  • Lindberg, S. E., Johnson, D. W., Lovett, G. M., Taylor, G. E., Van Miegroet, H., and Owens, J. G.: 1989, Sampling and analysis protocols for the Integrated Forest Study, ORNL/TM-I 1214, Oak Ridge National Lab.

  • Lovett, G. M., Reiners, W. A., and Olson, R. K.: 1982, Science 218, 1303.

    Google Scholar 

  • Lovett, G. M.: 1984, Atmos Envir. 18, 361.

    Google Scholar 

  • Lovett, G. M. and Lindberg, S. E.: 1984, J. Appl. Ecol. 21, 1013.

    Google Scholar 

  • Mayer, R.: 1983, in B. Ulrich and J. Pankrath (eds.), Effects of Accumulation of Air Pollutants in Forest Ecosystems, Reidel, London, pp. 47–56.

    Google Scholar 

  • National Research Council ; 1989, Controlling Airborne Particles, Nat. Academy of Sciences Press, Washington, DC.

    Google Scholar 

  • Nriagu, J. O., ed.: 1984, Changing Metal Cycles and Human Health, Springer-Verlag, Berlin.

    Google Scholar 

  • Nriagu, J. O.: 1989, ‘Natural versus Anthropogenic Emissions of Trace Metals to the Atmosphere’, in Control and Fate of Atmospheric Trace Metals, J. M. Pacyna and B. Ottar (eds.), Kluwer Academic Publishers, Dordrecht, Holland.

    Google Scholar 

  • Petty, W. H. and Lindberg, S. E.: 1987, ‘An Intensive Short-Term Study of Atmospheric Lead Deposition to a High-Elevation Spruce Forest’, in Proceedings: Heavy Metals in the Environment, S. E. Lindberg and T. C. Hutchinson (eds.), CEP Consultants, Publishers, Edinburgh.

    Google Scholar 

  • Salomons, W. and Förstner, U.: 1984, Metal in the Hydrocycle, Springer-Verlag, New York.

    Google Scholar 

  • Schaefer, D. A., Lindberg, S. E., and Hoffman, W. A.: 1989, Tellus 41B, 207.

    Google Scholar 

  • Stevens, R. K., Dzubay, T. G., Shaw, K. W., Jr., McGlenny, W. A., Lewis, C. W., and Wilson, W. E.: 1980, Environ. Sci. Technol. 14, 1491.

    Google Scholar 

  • Ulrich, B. and Klockow, D. (eds.), Proceedings: International Congress on Forest Decline Research: State of Knowledge Perspectives, Friedrichshafen, F.R.G., October 2–6, 1989, Kluwer Acad. Publ. Co., Dordrecht, Holland.

    Google Scholar 

  • Tukey, H. B.: 1970, Annu. Rev. Plant Physiology, 21, 305.

    Google Scholar 

  • Unsworth, M. and Fowler, D. E. (eds.): 1988, Processes of Acidic Deposition in Mountainous Terrain, Kluwer Academic Publishers, London, pp. 321–344.

    Google Scholar 

  • Wiersma, G. B.: 1980, Lead Particles in the Great Smoky Mountains Biosphere Reserve, Report No. 600/4–80–002, U.S. Environ. Protection Agency, Washington, D.C.

    Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Additional information

Author for all correspondence.

Operated by Martin Marietta Energy Systems, Inc., under contract DE-AC05-84OR21400 with the U.S. Department of Energy.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Petty, W.H., Lindberg, S.E. An intensive 1-month investigation of trace metal deposition and throughfall at a mountain spruce forest. Water Air Soil Pollut 53, 213–226 (1990). https://doi.org/10.1007/BF00170738

Download citation

  • Received:

  • Revised:

  • Issue Date:

  • DOI: https://doi.org/10.1007/BF00170738

Keywords

Navigation