Skip to main content
Log in

Concentration fluctuation measurements in tracer plumes using high and low frequency response detectors

  • Published:
Boundary-Layer Meteorology Aims and scope Submit manuscript

Abstract

A set of tracer experiments designed to compare two concentration fluctuation detectors and measure fluctuation statistics at high frequencies is described. A detector which has been used in several previous fluctuation experiments (the TIP photoionisation detector manufactured by Photovac of Canada) is compared with another with a much higher frequency response (the flame ionisation detector — FID — made by Cambustion of the UK). Good agreement is found and results show that the signal optimization system used in previous work with the TIP provides an accurate enhancement of the instrument output, thus improving confidence in the results of previous papers. They also confirm that the TIP detector is able to resolve most of the concentration variance in most situations of interest, but not at very short range. Measurements of the high frequency end of the fluctuation spectrum using the FID show inertial-convective subrange behaviour at frequencies not resolved by the TIP, supporting earlier work. Fluctuation spectra measured very close to the source are also shown to have a characteristic +2/3 power law behaviour (when nSc (n) is plotted against n) at lower frequencies, in agreement with theoretical predictions.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  • Benner, R. L. and Lamb, B. K.: 1985, ‘A Fast Response Continuous Analyzer for Halogenated Atmospheric Tracers’, J. Atmos. Ocean. Tech. 2, 582–589.

    Google Scholar 

  • Crooks, G. and Ramsay, S.: 1993, ‘A Wind Tunnel Study of Mean and Fluctuating Concentration in a Plume Dispersing over a Two-Dimensional Hill’, Boundary-Layer Meteorol. 66, 155–172.

    Google Scholar 

  • Davidson, M. J., Mylne, K. R., Jones, C. D., Phillips, J. C., Perkins, R. J., Fung, J. C. H., and Hunt, J. C. R.: 1995, ‘Plume Dispersion and Large Groups of Obstacles — A Field Investigation’, Atmos. Environ., in press.

  • Dinar, N., Kaplan, H., and Kleiman, M.: 1988, ‘Characterization of Concentration Fluctuations of a Surface Plume in a Neutral Boundary Layer’, Boundary-Layer Meteorol. 45, 157–175.

    Google Scholar 

  • Fackrell, J. E.: 1980, ‘A Flame Ionisation Detector for Measuring Fluctuating Concentration’, J. Phys. E: Sci. Instrum. 13, 888–893.

    Google Scholar 

  • Fackrell, J. E. and Robins, A. G.: 1982, ‘Concentration Fluctuations and Fluxes in Plumes from Point Sources in a Turbulent Boundary Layer’, J. Fluid Mech. 117, 1–26.

    Google Scholar 

  • Haana, S. R.: 1984, ‘The Exponential Probability Density Function and Concentration Fluctuations in Smoke Plumes’, Boundary-Layer Meteorol. 29, 361–375.

    Google Scholar 

  • Hall, D. J. and Emmott, M. A.: 1991, ‘Avoiding Aerosol Sampling Problems in Fast Response Flame Ionisation Detectors’, Experiments in Fluids 10, 237–240.

    Google Scholar 

  • Jones, C. D.: 1983, ‘On the Structure of Instantaneous Plumes in the Atmosphere’, J. Haz. Mat. 7, 87–112.

    Google Scholar 

  • Lewis, D. M. and Chatwin, P. C.: 1995, ‘The Treatment of Atmospheric Dispersion Data in the Presence of Noise and Baseline Drift’, Boundary-Layer Meteorol. 72, 53–85.

    Google Scholar 

  • Mylne, K. R.: 1992a, ‘Concentration Fluctuation Measurements in a Plume Dispersing in a Stable Surface Layer’, Boundary-Layer Meteorol. 60, 15–48.

    Google Scholar 

  • Mylne, K. R.: 1992b, ‘The PDF of Concentration Fluctuations — Comments on Yee (1990) and Yee (1991)’, Boundary-Layer Meteorol. 61, 189–193.

    Google Scholar 

  • Mylne, K. R.: 1993, ‘The Vertical Profile of Concentration Fluctuations in Near-Surface Plumes’, Boundary-Layer Meteorol. 65, 111–136.

    Google Scholar 

  • Mylne, K. R. and Davidson, M. J.: 1991, Concentration Fluctuation Experiments in Stable Conditions and in a Pseudo-Urban Environment, 19th International Technical Meeting on Air Pollution Modelling and its Application, Ierapetra, Crete, pp. 479–486, in Han van Dop (ed.), Air Pollution Modeling and Its Application, Vol. IX, Plenum Press, New York, 1992, pp. 631–640.

    Google Scholar 

  • Mylne, K. R. and Mason, P. J.: 1991, ‘Concentration Fluctuation Measurements in a Dispersing Plume at a Range of up to 1000 m’, Quart. J. Roy. Meteorol. Soc. 117, 177–206.

    Google Scholar 

  • Panofsky, H. A. and Dutton, J. A.: 1984, Atmospheric Turbulence, John Wiley, New York.

    Google Scholar 

  • Peterson, H. G., Lamb, B. K., and Stock, D. E.: 1988, ‘Plume Concentration and Velocity Fluctuations during Convective and Stable Conditions’, 8th Symp. on Turb. and Diff., AMS 341–344.

  • Sawford, B. L.: 1987, ‘Conditional Concentration Statistics for Surface Plumes in the Atmospheric Boundary Layer’, Boundary-Layer Meteorol. 38, 209–223.

    Google Scholar 

  • Sawford, B. L., Frost, C. C., and Allan, T. C.: 1985, ‘Atmospheric Boundary-Layer Measurements of Concentration Statistics from Isolated and Multiple Sources’, Boundary-Layer Meteorol. 31, 249–268.

    Google Scholar 

  • Thomson, D. J.: 1990, ‘A Stochastic Model for the Motion of Particle Pairs in Isotropic High Reynolds Number Turbulence, and its Application to the Problem of Concentration Variance’, J. Fluid Mech. 210, 113–153.

    Google Scholar 

  • Thomson, D. J.: 1996, ‘The Second-Order Moment Structure of Dispersing Plumes and Puffs, submitted to J. Fluid Mech.

  • Yee, E.: 1990, ‘The Shape of the Probability Density Function of Short-Term Concentration Fluctuations of Plumes in the Atmospheric Boundary Layer’, Boundary-Layer Meteorol. 51, 269–298.

    Google Scholar 

  • Yee, E.: 1991, ‘Application of Nonlinear Dynamical Systems Analysis to Conditionally Sampled Concentration Fluctuations of a Passive Scalar in the Atmospheric Boundary Layer’, Boundary-Layer Meteorol. 57, 49–78.

    Google Scholar 

  • Yee, E.: 1992, Reply to the Comments on: The PDF of Concentration Fluctuations by K. R. Mylne’, Boundary-Layer Meteorol. 61, 195–204.

    Google Scholar 

  • Yee, E., Kosteniuk, P. R., Chandler, G. M., Biltoft, C. A., and Bowers, J. F.: 1993a, ‘Statistical Characteristics of Concentration Fluctuations in Dispersing Plumes in the Atmospheric Surface Layer’, Boundary-Layer Meteorol. 65, 69–109.

    Google Scholar 

  • Yee, E., Kosteniuk, P. R., Chandler, G. M., Biltoft, C. A., and Bowers, J. F.: 1993b, ‘Recurrence Statistics of Concentration Fluctuations in Plumes within a Near-Neutral Atmospheric Surface Layer’, Boundary-Layer Meteorol. 66, 127–153.

    Google Scholar 

  • Yee, E., Chan, R., Kosteniuk, P. R., Chandler, G. M., Biltoft, C. A., and Bowers, J. F.: 1994a, ‘Concentration Fluctuation Measurements in Clouds Released from a Quasi-Instantaneous Point Source in the Atmospheric Surface Layer’, Boundary-Layer Meteorol. 71, 341–373.

    Google Scholar 

  • Yee, E., Chan, R., Kosteniuk, P. R., Chandler, G. M., Biltoft, C. A., and Bowers, J. F.: 1994b, ‘Experimental Measurements of Concentration Fluctuations and Scales in a Dispersing Plume in the Atmospheric Surface Layer Obtained Using a Very Fast Response Concentration Detector’, J. Appl. Meteorol. 33, 996–1016.

    Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Rights and permissions

Reprints and permissions

About this article

Cite this article

Mylne, K.R., Davidson, M.J. & Thomson, D.J. Concentration fluctuation measurements in tracer plumes using high and low frequency response detectors. Boundary-Layer Meteorol 79, 225–242 (1996). https://doi.org/10.1007/BF00119439

Download citation

  • Accepted:

  • Issue Date:

  • DOI: https://doi.org/10.1007/BF00119439

Keywords

Navigation