Abstract
Ambient particulate sulfate measurements have been intermittently performed at a rural site in Israel over a period of more than two years. Concurrent measurements of ambient pollutants (SO2, NO−NOx, and O3), as well as meteorological data, were also carried out. The daily data included four particulate sulfate samples representing four successive 6 h accumulating periods. The measured concentrations of sulfate ions ranged from a low 2 μg m-3 observed during the winter season to a high of >50 μg m-3 obtained during the summer. Little correlation was obtained between the sulfate concentration and either O3 or SO2, although sulfate and O3 showed a similar diurnal and annual trend. Based on the data distribution and on a photochemical model, it was concluded that a large part of the particulate sulfate observed at the eastern coast of the Mediterranean Sea must be related to long-range transport from distant sources.
Similar content being viewed by others
References
Altshuller A. P., 1979, Model prediction of the rate of homogeneous oxidation of sulfur dioxide in the atmosphere, Atmos. Environ. 13, 1653–1661.
Charlson R. J. and Rohde H., 1982, Factors controlling the acidity of rain water, Nature (London) 295, 683–695.
Dayan U., 1986, Climatology of back trajectories from Israel based on synoptic analysis, J. Climate Appl. Meteorol. 25, 591–595.
Forest J., Garber R., and Newman L., 1979, Formation of sulfate, ammonium and nitrate in an oilfired power plant plume, Atmos. Environ. 13, 1287–1297.
Husar R. B., Patterson D. E., Husar J. D., Gillani N. V., and Wilson W. E., 1978, Sulfur budget of a power plant plume, Atmos. Environ. 12, 549–568.
Lifshitz B., Peleg M., and Luria M., 1988, The influence of medium range transport on O3 levels at a rural site in Israel, J. Atmos. Chem. 7, 19–33.
Luria M., Almog A., and Peleg M., 1984, Transport and transformation of air pollutants from Israel's coastal area, Atmos. Environ. 18, 2095–2104.
Luria M., Van Valin C. C., Wellman D. L., and Pueschel R. F., 1986, The contribution of Gulf Area natural sulfur to the North American Sulfur budget, Environ. Sci. Technol. 20, 91–95.
Luria M. and Meagher J. F., 1988, Computer simulation of the boundary layer oxidation and removal of atmospheric pollutants over the western Atlantic Ocean, Atmos. Environ. 22, 307–319.
Luria M., Van Valin C. C., Wellman D. L., Keene W. C., Galloway J. N., and Boatman J. F., 1988, Eastward sulfur flux from the Northeastern United States, Atmos. Environ. 22, 1847–1855.
Luria, M., Lifschitz, B., Gawi, Z., and Peleg, M., 1989, Sulfate levels at rural and urban sites in Israel, Proc. 8th Clean Air Congress, The Hague, Holland, September 11–15 (in press).
Mahrer Y. and Pielke R. A., 1977, Numerical study of the air flow over irregular terrain, Beitrage zur Physik der Atmosphäre, 50, 98–113.
Meagher J. F., Bailey M., and Luria M., 1983, The seasonal variation of atmospheric SO2 to SO4 2- conversion rate, J. Geophys. Res. 88, 1525–1427.
Prospero J. M., Savoy D., Ness R. T., Duce R. A., and Merrill J., 1985, Particulate sulfate and nitrate in the boundary layer over the North Pacific Ocean, J. Geophys. Res. 90, 10586–10589.
Stockwell W. R. and Calvert J. G., 1983, The mechanism of HO−SO2 reaction, Atmos. Environ. 17, 2231–2235.
Van Valin C. C., Wellman D. L., and Stearns L. P., 1987, Aerosol and cloudwater properties at Whiteface Mountain, New York, Water, Air and Soil Pollut. 34, 369–383.
Wolff G. T., Ruthokoski M. S., Stroup D. P., Korsog P. E., Ferman M. A., Wendel G. J., and Stedman D. H., 1986, Measurements of SOx, NOxand aerosol species at Bermuda, Atmos. Environ. 20, 1229–1239.
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Luria, M., Lifschitz, B. & Peleg, M. Particulate sulfate levels at a rural site in Israel. J Atmos Chem 8, 241–250 (1989). https://doi.org/10.1007/BF00051496
Received:
Revised:
Issue Date:
DOI: https://doi.org/10.1007/BF00051496