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Environmental Earth Sciences

, 78:646 | Cite as

Carbon sequestration at the Illinois Basin-Decatur Project: experimental results and geochemical simulations of storage

  • Peter M. BergerEmail author
  • Lois Yoksoulian
  • Jared T. Freiburg
  • Shane K. Butler
  • William R. Roy
Original Article
  • 67 Downloads

Abstract

The Midwest Geological Sequestration Consortium is conducting the Illinois Basin-Decatur Project (IBDP), a large-scale demonstration of carbon sequestration that injected the CO2 from an ethanol plant into the Mt. Simon Sandstone. Using site-specific data and samples, batch experiments were conducted at reservoir conditions and the reactive transport code TOUGHREACT was used to model the CO2 migration and interactions in the injection formation. In the model, most of the mineral alteration occurred after the injection was completed and brine displaced the CO2 at the base of the plume. K-feldspar dissolution led to a nearly 10% increase in porosity which is a maximum estimate of alteration because, the model omits mineral transformations and may underestimate clay precipitation and the effects of grain coatings. The batch experiments recreated these conditions and showed a little alteration. In both the model and experiments, the bulk of the mineralogy remained inert. Calcite precipitated within the modeled plume where the transformation of K-feldspar to clays buffered the pH, though this process only produced minor mineral sequestration. Less-permeable layers in the model baffled the ascent of the CO2 plume and caused it to spread laterally. The plume did not reach the upper third of the Mt. Simon Sandstone. Both the model and the batch experiments show that the bulk of the Mt. Simon Sandstone will undergo little change due to CO2 injection, and the batch experiments show the feldspar dissolution in the model is likely limited.

Keywords

Carbon sequestration Mt. Simon Reactive transport model Batch experiment Kinetics 

Notes

Acknowledgements

We thank Scott Frailey and James Damico of the ISGS for the information on permeability and porosity, and Ivan Krapac, Bracken Wimmer, Abbas Iranmanesh, Chris Patterson, and Randy Locke for the water chemistry data. This material is based upon work supported by the US Department of Energy National Energy Technology Laboratory under Award Number DE-FC26-05NT42588 with support, in part, by awards made possible by the Illinois Department of Commerce and Economic Opportunity through the Office of Coal Development and the Illinois Clean Coal Institute. Any opinions, findings, and conclusions or recommendations expressed in this publication are those of the authors and do not necessarily reflect the views of the Illinois Department of Commerce and Economic Opportunity, the Office of Coal Development, or the Illinois Clean Coal Institute. This publication was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof.

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Copyright information

© Springer-Verlag GmbH Germany, part of Springer Nature 2019

Authors and Affiliations

  1. 1.Illinois State Geological SurveyChampaignUSA
  2. 2.University of IllinoisChampaignUSA
  3. 3.Centre for Ore Deposit and Earth SciencesUniversity of TasmaniaHobartAustralia
  4. 4.Energy & Environmental Research Center (EERC)Grand ForksUSA

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