Journal of Optics

, Volume 46, Issue 4, pp 486–491 | Cite as

One, two and three photon absorption of two level system in femto-second laser excitation

Research Article
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Abstract

Theoretically, we have studied the multi-photon absorption by rate equation approach in the presence of femto-second laser excitation. The time dependent and saturation effects in the nonlinear transmittance are incorporated as they will occur in the absorption process. At low intensity excitation, the transmitted pulse shape has the same shape as incident pulse, but at excitation intensities above the saturation intensity, the shape of the transmitted pulse has got change according to the absorption coefficient variation with intensity. Transmittance in the two and three photon absorption has discussed comparatively in both single beam transmittance and z-scan. In the nonlinear absorption study under femto-second laser excitation, the high peak power of femto-second laser can saturate the absorption in multi-photon absorption even though the process is through virtual levels. We have shown that, at excitation intensities above the saturation intensity, how the absorption coefficient deviates the logarithmic plot of transmittance from its straight line nature.

Keywords

Rate equations Femto second pulses Multi-photon absorption Z-scan Single beam transmittance 

References

  1. 1.
    A. Sharan, R.C. Sharma, S.N. Sandhya, A. Ayyer, K.K. Sharma, Modeling absorption in saturable absorbers. Opt. Commun. 199(1), 267–275 (2001)ADSCrossRefGoogle Scholar
  2. 2.
    S. Webster, S.A. Odom, L.A. Padilha, O.V. Przhonska, D. Peceli, H. Hu, G. Nootz, A.D. Kachkovski, J. Matichak, S. Barlow, H.L. Anderson, Linear and nonlinear spectroscopy of a porphyrin − squaraine − porphyrin conjugated system. J. Phys. Chem. B 113(45), 14854–14867 (2009)CrossRefGoogle Scholar
  3. 3.
    A. Srinivasa Rao, Theoretical study on nonlinear properties of four level systems under nano-second illumination. Laser Phys. 25(5), 055701 (2015)CrossRefGoogle Scholar
  4. 4.
    M. del Rayo, Y.O. Barmenkov, A.V. Kir yanov, A.N. Starodumov, J. Vanhanen, T. Jaaskelainen, Application of the Z-scan technique to a saturable medium with excited state absorption. Laser Phys. Lawrence 11(4), 502–506 (2001)Google Scholar
  5. 5.
    C. Li, L. Zhang, M. Yang, H. Wang, Y. Wang, Dynamic and steady-state behaviors of reverse saturable absorption in metallophthalocyanine. Phys. Rev. A 49, 1149–1157 (1994)ADSCrossRefGoogle Scholar
  6. 6.
    A. Kobyakov, D.J. Hagan, E.W. Van Stryland, Analytical approach to dynamics of reverse saturable absorbers. Josa B 17(11), 1884–1893 (2000)ADSCrossRefGoogle Scholar
  7. 7.
    R.L. Swofford, W.M. McClain, The effect of spatial and temporal laser beam characteristics on two-photon absorption. Chem. Phys. Lett. 34(3), 455–460 (1975)ADSCrossRefGoogle Scholar
  8. 8.
    J. He, Y. Qu, H. Li, J. Mi, W. Ji, Three-photon absorption in ZnO and ZnS crystals. Opt. Exp. 13(23), 9235–9247 (2005)ADSCrossRefGoogle Scholar
  9. 9.
    G.S. He, Q. Zheng, A. Baev, P.N. Prasad, Saturation of multiphoton absorption upon strong and ultrafast infrared laser excitation. J. Appl. Phys. 101(8), 083108 (2007)ADSCrossRefGoogle Scholar
  10. 10.
    K.V. Adarsh, K.S. Sangunni, S. Sandeep, R. Philip, S. Kokenyesi, V. Takats, Observation of three-photon absorption and saturation of two-photon absorption in amorphous nanolayered Se/As2S3 thin film structures. J. Appl. Phys. 102, 026102 (2007)ADSCrossRefGoogle Scholar
  11. 11.
    D.S. Corrêa, L. De Boni, L. Misoguti, I. Cohanoschi, F.E. Hernandez, C.R. Mendonça, Z-scan theoretical analysis for three-, four-and five-photon absorption. Opt. Commun. 277(2), 440–445 (2007)ADSCrossRefGoogle Scholar
  12. 12.
    M. Rumi, J.W. Perry, Two-photon absorption: an overview of measurements and principles. Adv. Opt. Photon. 2(4), 451–518 (2010)CrossRefGoogle Scholar
  13. 13.
    F. Boitier, A. Godard, E. Rosencher, C. Fabre, Measuring photon bunching at ultrashort timescale by two-photon absorption in semiconductors. Nat. Phys. 5(4), 267–270 (2009)CrossRefGoogle Scholar
  14. 14.
    B. Gu, Y. Sun, W. Ji, Two-photon-induced excited-state nonlinearities. Opt. Exp. 16(22), 17745–17751 (2008)ADSCrossRefGoogle Scholar
  15. 15.
    P. Sperber, A. Penzkofer, S0-Sn two-photon absorption dynamics of rhodamine dyes. Opt. Quant. Electron. 18(5), 381–401 (1986)CrossRefGoogle Scholar
  16. 16.
    J. Wang, G. Bing, X.-W. Ni, H.-T. Wang, Z-scan theory with simultaneous two-and three-photon absorption saturation. Opt. Laser Technol. 44(2), 390–393 (2012)ADSCrossRefGoogle Scholar
  17. 17.
    G. Boudebs, S. Cherukulappurath, M. Guignard, J. Troles, F. Smektala, F. Sanchez, Experimental observation of higher order nonlinear absorption in tellurium based chalcogenide glasses. Opt. Commun. 232(1), 417–423 (2004)ADSCrossRefGoogle Scholar
  18. 18.
    B. Gu, W. Ji, Two-step four-photon absorption. Opt. Exp. 16(14), 10208–10213 (2008)ADSCrossRefGoogle Scholar
  19. 19.
    J.N.B. Reddy, V.B. Naik, S. Elizabeth, H.L. Bhat, N. Venkatram, D. Narayanarao, Multiphoton absorption in CsLiB6O10 with femtosecond infrared laser pulses. J. Appl. Phys. 104(5), 053108 (2008)ADSCrossRefGoogle Scholar
  20. 20.
    R.A. Ganeev, A.I. Ryasnyansky, N. Ishizawa, M. Baba, M. Suzuki, M. Turu, S. Sakakibara, H. Kuroda, Two-and three-photon absorption in CS2. Opt. Commun. 231(1), 431–436 (2004)ADSCrossRefGoogle Scholar

Copyright information

© The Optical Society of India 2017

Authors and Affiliations

  1. 1.Department of PhysicsPondicherry UniversityKalapetIndia

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