Advertisement

Korean Journal of Chemical Engineering

, Volume 36, Issue 12, pp 2008–2022 | Cite as

Evaluation of novel Mg/Al/Ni-BaFe ternary layered hydroxides uptake of methyl orange dye from water

  • Nuhu Dalhat Mu’azuEmail author
  • Nabeel Jarrah
  • Mukarram Zubair
  • Mohammad Saood Manzar
  • Taye Saheed Kazeem
  • Mamdouh Al-Harthi
Environmental Engineering
  • 6 Downloads

Abstract

MgAlNi-BaFe ternary layered hydroxide (UMLDH) and its calcined (CMLDH) form were synthesized and tested as adsorbents for methyl orange dye (MO) uptake from water. The adsorptive performances of the new magnetic nanocomposites were modeled, evaluated and optimized via response surface methodology (RSM). The UMLDH and CMLDH maximum removal efficiency and adsorption capacities data were fitted into RSM models with insignificant lack of fit (p-values<0.05) and high R2=0.991–0.997. The UMLDH and CMLDH MO adsorption capacities increased with decrease in both pH and initial MO concentration and decreased when the temperature was increased. Under optimal operating conditions, pseudo-second-order described kinetics of MO sorption on the nanocomposites, while the Freundlich isotherm gave the best fits for both the two adsorbents. The MO uptake simultaneously incorporated both mono and multi-layer surface adsorption involving strong electrostatic attraction and chemical interactions between MO and the adsorbents surface functional groups. Respectively, the obtained maximum Langmuir theoretical sorption capacity of 715.44 and 708 mg/g, indicated profoundly improved MO sorption capacities compared with many other magnetic-LDHs. These results demonstrate the potential of MgAlNi-BaFe as excellent adsorbents for effective remediation of dyes wastewater effluents.

Keywords

Barium Ferrite LDH MgAlNi Nanocomposites Methyl Orange Dye Uptake Response Surface Methodology 

Preview

Unable to display preview. Download preview PDF.

Unable to display preview. Download preview PDF.

Notes

Acknowledgements

Funding provided by King Abdul-Aziz City for Science and Technology (KACST) under NSTIP through Project No. 12-Env2229-46 at Imam Abdulrahman Bin Faisal University and the Center of Research Excellences in Nanotechnology King Fahd University of Petroleum & Minerals for synthesis and characterization of the adsorbents is acknowledged and appreciated.

Supplementary material

11814_2019_384_MOESM1_ESM.pdf (3.2 mb)
Evaluation of novel Mg/Al/Ni-BaFe ternary layered hydroxides uptake of methyl orange dye from water

References

  1. 1.
    Z. P. Xu, J. Zhang, M. O. Adebajo, H. Zhang and C. Zhou, Appl. Clay Sci., 53, 139 (2011).CrossRefGoogle Scholar
  2. 2.
    Y. Kuthati, R.K. Kankala and C.-H. Lee, Appl. Clay Sci., 112-113, 100 (2015).CrossRefGoogle Scholar
  3. 3.
    M. Daud, M. S. Kamal, F. Shehzad and M. A. Al-Harthi, Carbon, 104, 241 (2016).CrossRefGoogle Scholar
  4. 4.
    N. N. Das, J. Konar, M. K. Mohanta and S. C. Srivastava, J. Colloid Interface Sci., 270, 1 (2004).CrossRefPubMedPubMedCentralGoogle Scholar
  5. 5.
    M. Zubair, M. Daud, G. McKay, F. Shehzad and M. A. Al-Harthi, Appl. Clay Sci., 143, 279 (2017).CrossRefGoogle Scholar
  6. 6.
    L. Lu, J. Li, D.H.L. Ng, P. Yang, P. Song and M. Zuo, J. Ind. Eng. Chem., 46, 315 (2017).CrossRefGoogle Scholar
  7. 7.
    R.-r. Shan, L.-g. Yan, K. Yang, S.-j. Yu, Y.-f. Hao, H.-q. Yu and B. Du, Chem. Eng. J., 252, 38 (2014).CrossRefGoogle Scholar
  8. 8.
    Y. Wang, T. Du, L. Zhou, Y. Song, S. Che and X. Fang, Korean J. Chem. Eng., 35, 709 (2018).CrossRefGoogle Scholar
  9. 9.
    M. Daud, M.S. Kamal, F. Shehzad and M.A. Al-Harthi, Carbon, 104, 241 (2016).CrossRefGoogle Scholar
  10. 10.
    R. Ma, Z. Liu, L. Li, N. Iyi and T. Sasaki, J. Mater. Chem., 16, 3809 (2006).CrossRefGoogle Scholar
  11. 11.
    W. Peng, H. Li, Y. Liu and S. Song, J. Mol. Liq., 230, 496 (2017).CrossRefGoogle Scholar
  12. 12.
    G. Huang, L. Jiang, D. Wang, J. Chen, Z. Li and S. Ma, J. Mol. Liq., 220, 346 (2016).CrossRefGoogle Scholar
  13. 13.
    Y.-X. Wang, K. Gupta, J.-R. Li, B. Yuan, J.-C. E. Yang and M.-L. Fu, Colloids Surf., A: Physicochem. Eng. Aspects, 538, 378 (2018).CrossRefGoogle Scholar
  14. 14.
    Q. Yang, S. Ren, Q. Zhao, R. Lu, C. Hang, Z. Chen and H. Zheng, Chem. Eng. J., 333, 49 (2018).CrossRefGoogle Scholar
  15. 15.
    L. Huang, M. He, B. Chen and B. Hu, Chemosphere, 199, 435 (2018).CrossRefPubMedGoogle Scholar
  16. 16.
    R.-G. Ciocarlan, E. M. Seftel, M. Mertens, A. Pui, M. Mazaj, N. N. Tusar and P. Cool, Mater. Sci. Eng.: B, 230, 1 (2018).CrossRefGoogle Scholar
  17. 17.
    B. Tanhaei, A. Ayati, M. Lahtinen and M. Sillanpää, Chem. Eng. J., 259, 1 (2015).CrossRefGoogle Scholar
  18. 18.
    M. R. Abukhadra M. Rabia M. Shaban and F. Verpoort, Adv. Powder Technol., 29, 2501 (2018).CrossRefGoogle Scholar
  19. 19.
    M. R. Abukhadra, A. Adlii and B. M. Bakry, Int. J. Biol. Macromol., 126, 402 (2019).CrossRefGoogle Scholar
  20. 20.
    R.-S. Juang, Y.-C. Yei, C.-S. Liao, K.-S. Lin, H.-C. Lu, S.-F. Wang and A.-C. Sun, J. Taiwan Inst. Chem. Engineers, 90, 51 (2018).CrossRefGoogle Scholar
  21. 21.
    S. Bao, K. Li, P. Ning, J. Peng, X. Jin and L. Tang, J. Taiwan Inst. Chem. Engineers, 87, 64 (2018).CrossRefGoogle Scholar
  22. 22.
    V. Ganesan, C. Louis and S. P. Damodaran, J. Environ. Chem. Eng., 6, 2176 (2018).CrossRefGoogle Scholar
  23. 23.
    Z. Zhang and J. Kong, J. Hazard. Mater., 193, 325 (2011).CrossRefPubMedGoogle Scholar
  24. 24.
    R. Jiang, Y.-Q. Fu, H.-Y. Zhu, J. Yao and L. Xiao, J. Appl. Polym. Sci., 125, E540 (2012).CrossRefGoogle Scholar
  25. 25.
    Z. Yang, S. Ji, W. Gao, C. Zhang, L. Ren, W. W. Tjiu, Z. Zhang, J. Pan and T. Liu, J. Colloid Interface Sci., 408, 25 (2013).CrossRefPubMedGoogle Scholar
  26. 26.
    L. Adlnasab, M. Ezoddin, M.A. Karimi and N. Hatamikia, Res. Chem. Intermediates, 44, 3249 (2018).CrossRefGoogle Scholar
  27. 27.
    X. Wu, B. Li and X. Wen, J. Nanopart. Res., 19, 131 (2017).CrossRefGoogle Scholar
  28. 28.
    Z. Jia, S. Li, J. Liu, Q. Qin and R. Zhu, Bull. Mater. Sci., 38, 1757 (2015).CrossRefGoogle Scholar
  29. 29.
    R.-G. Ciocarlan, E.M. Seftel, M. Mertens, A. Pui, M. Mazaj, N. Novak Tusar and P. Cool, Mater. Sci. Eng.: B, 230, 1 (2018).CrossRefGoogle Scholar
  30. 30.
    H. Sun, L. Cao and L. Lu, Nano Res., 4, 550 (2011).CrossRefGoogle Scholar
  31. 31.
    K. Cui, B. Yan, Y. Xie, H. Qian, X. Wang, Q. Huang, Y. He, S. Jin and H. Zeng, J. Hazard. Mater., 350, 66 (2018).CrossRefPubMedPubMedCentralGoogle Scholar
  32. 32.
    S. N. Basahel, T. T. Ali, M. Mokhtar and K. Narasimharao, Nanoscale Res. Lett., 10, 73 (2015).CrossRefPubMedPubMedCentralGoogle Scholar
  33. 33.
    N. D. Mu’azu, N. Jarrah, T. S. Kazeem, M. Zubair and M. Al-Harthi, Appl. Clay Sci., 161, 23 (2018).CrossRefGoogle Scholar
  34. 34.
    M. Zubair, N. Jarrah, M. S. Manzar, M. Al-Harthi, M. Daud, N. D. Mu’azu and S. A. Haladu, J. Mol. Liq., 230, 344 (2017).CrossRefGoogle Scholar
  35. 35.
    N. D. Mu’azu, M. H. Al-Malack and N. Jarrah, Desalination Water Treat, 52, 7293 (2014).CrossRefGoogle Scholar
  36. 36.
    M. H. Essa, N. D. Mu’azu, S. Lukman and A. Bukhari, Soil and Sediment Contamination: An International J., 24, 30 (2015).CrossRefGoogle Scholar
  37. 37.
    N. D. Mu’azu, S. A. Haladu, N. Jarrah, M. Zubair, M. H. Essa and S. A. Ali, J. Hazard. Mater., 342, 58 (2018).CrossRefPubMedPubMedCentralGoogle Scholar
  38. 38.
    R.H. Myers and D.C. Montgomery, Response Surface Methodology: Process and Product Optimization Using Designed Experiments, Wiley, New York (1995).Google Scholar
  39. 39.
    Y. Vlamidis, E. Scavetta, M. Giorgetti, N. Sangiorgi and D. Tonelli, Appl. Clay Sci., 143, 151 (2017).CrossRefGoogle Scholar
  40. 40.
    M. Hussein, A. Jaafar, A. Yahaya, M. Masarudin and Z. Zainal, Int. J. Mol. Sci., 15, 20254 (2014).CrossRefPubMedPubMedCentralGoogle Scholar
  41. 41.
    A. A. Oladipo and M. Gazi, J. Water Process Eng., 2, 43 (2014).CrossRefGoogle Scholar
  42. 42.
    F. B. D. Saiah, B.-L. Su and N. Bettahar, J. Hazard. Mater., 165, 206 (2009).CrossRefGoogle Scholar
  43. 43.
    S. Yang, L. Wang, X. Zhang, W. Yang and G. Song, Chem. Eng. J., 275, 315 (2015).CrossRefGoogle Scholar
  44. 44.
    T. S. Kazeem, M. Zubair, M. Daud, N. D. Mu’azu and M. A. Al-Harthi, Korean J. Chem. Eng., 36, 1057 (2019).CrossRefGoogle Scholar
  45. 45.
    S. Tang and H. K. Lee, Anal. Chem., 85, 7426 (2013).CrossRefGoogle Scholar
  46. 46.
    H. Zaghouane-Boudiaf, M. Boutahala and L. Arab, Chem. Eng. J., 187, 142 (2012).CrossRefGoogle Scholar
  47. 47.
    Z. Wang and X. Li, High Perform. Polym., 0954008317716976 (2017).Google Scholar
  48. 48.
    P. Scherrer, Nachr. Ges. Wiss. Göttingen, 2, 96 (1918).Google Scholar
  49. 49.
    R. Elmoubarki, F. Z. Mahjoubi, A. Elhalil, H. Tounsadi, M. Abdennouri, M. H. Sadiq, S. Qourzal, A. Zouhri and N. Barka, J. Mater. Res. Technol., 6, 271 (2017).CrossRefGoogle Scholar
  50. 50.
    D. Chebli, A. Bouguettoucha, A. Reffas, C. Tiar, M. Boutahala, H. Gulyas and A. Amrane, Desalination Water Treatment, 57, 22061 (2016).CrossRefGoogle Scholar
  51. 51.
    M. Zubair, N. Jarrah, A. Khalid, M.S. Manzar, T.S. Kazeem and M. A. Al-Harthi, J. Mol. Liq.., 249, 254 (2018).CrossRefGoogle Scholar
  52. 52.
    M.N. Pahalagedara, M. Samaraweera, S. Dharmarathna, C.-H. Kuo, L. R. Pahalagedara, J. A. Gascón and S. L. Suib, J. Phys. Chem. C, 118, 17801 (2014).CrossRefGoogle Scholar
  53. 53.
    W. Yao, S. Yu, J. Wang, Y. Zou, S. Lu, Y. Ai, N. S. Alharbi, A. Alsaedi, T. Hayat and X. Wang, Chem. Eng. J., 307, 476 (2017).CrossRefGoogle Scholar
  54. 54.
    N. D. Mu’azu, A. Usman, N. Jarrah and O. Alagha, Soil and Sediment Contamination: An International J., 25, 757 (2016).CrossRefGoogle Scholar
  55. 55.
    G. Wang, S. Zhang, T. Li, X. Xu, Q. Zhong, Y. Chen, O. Deng and Y. Li, RSC Adv., 5, 58010 (2015).CrossRefGoogle Scholar
  56. 56.
    G. Wang, S. Zhang, X. Xu, Q. Zhong, C. Zhang, Y. Jia, T. Li, O. Deng and Y. Li, Sci. Total Environ., 569-570, 557 (2016).CrossRefPubMedGoogle Scholar
  57. 57.
    M. Shaban, M. R. Abukhadra, A. S. Mohamed, M. G. Shahien and S. S. Ibrahim, J. Inorg. Organomet. Polym. Mater., 28, 279 (2018).CrossRefGoogle Scholar
  58. 58.
    Y. Lu, B. Jiang, L. Fang, F. Ling, J. Gao, F. Wu and X. Zhang, Chemosphere, 152, 415 (2016).CrossRefPubMedPubMedCentralGoogle Scholar
  59. 59.
    L. Lu, J. Li, D. H. Ng, P. Yang, P. Song and M. Zuo, J. Ind. Eng. Chem., 46, 315 (2017).CrossRefGoogle Scholar
  60. 60.
    N. Belhouchat, H. Zaghouane-Boudiaf and C. Viseras, Appl. Clay Sci., 135, 9 (2017).CrossRefGoogle Scholar
  61. 61.
    A. Khalid and M. Zubair, Arabian J. for Sci. Eng., 43, 2167 (2018).CrossRefGoogle Scholar
  62. 62.
    S. Karaca, A. Gürses, M. Ejder and M. Açikyıldiz, J. Hazard. Mater., 128, 273 (2006).CrossRefPubMedGoogle Scholar
  63. 63.
    D. Bharali and R. C. Deka, Colloids Surf., A: Physicochem. Eng. Aspects, 525, 64 (2017).CrossRefGoogle Scholar
  64. 64.
    S. L. Wang, R. J. Hseu, R. R. Chang, P. N. Chiang, J. H. Chen and Y.M. Tzou, Colloids Surf., A: Physicochem. Eng. Aspects, 277, 8 (2006).CrossRefGoogle Scholar
  65. 65.
    C. Nguyen and D. D. Do, Carbon, 39, 1327 (2001).CrossRefGoogle Scholar
  66. 66.
    P. Monash and G. Pugazhenthi, Environ. Prog. Sustainable Energy, 33, 154 (2014).CrossRefGoogle Scholar
  67. 67.
    Y. X. Zhang, X. D. Hao, M. Kuang, H. Zhao and Z. Q. Wen, Appl. Surf. Sci., 283, 505 (2013).CrossRefGoogle Scholar
  68. 68.
    K. Y. Foo and B. H. Hameed, Chem. Eng. J., 156, 2 (2010).CrossRefGoogle Scholar
  69. 69.
    W. J. Weber and J. C. Morris, J. Sanitary Eng;. Division, 89, 31 (1963).Google Scholar
  70. 70.
    L. Nirumand, S. Farhadi, A. Zabardasti and A. Khataee, Ultrason. Sonochem., 42, 647 (2018).CrossRefPubMedPubMedCentralGoogle Scholar
  71. 71.
    S. Bao, K. Li, P. Ning, J. Peng, X. Jin and L. Tang, J. Taiwan Inst. Chem. Engineers, 87, 64 (2018).CrossRefGoogle Scholar
  72. 72.
    Y. Lu, B. Jiang, L. Fang, F. Ling, J. Gao, F. Wu and X. Zhang, Chemosphere, 152, 415 (2016).CrossRefPubMedPubMedCentralGoogle Scholar

Copyright information

© The Korean Institute of Chemical Engineers 2019

Authors and Affiliations

  • Nuhu Dalhat Mu’azu
    • 1
    Email author
  • Nabeel Jarrah
    • 2
  • Mukarram Zubair
    • 1
  • Mohammad Saood Manzar
    • 1
  • Taye Saheed Kazeem
    • 3
  • Mamdouh Al-Harthi
    • 4
    • 5
  1. 1.Department of Environmental EngineeringImam Abdulrahman Bin Faisal UniversityDammamSaudi Arabia
  2. 2.Department of Chemical EngineeringMutah UniversityKarakJordan
  3. 3.Department of Civil Environmental EngineeringKing Fahd University of Petroleum & MineralsDhahranSaudi Arabia
  4. 4.Department of Chemical EngineeringKing Fahd University of Petroleum & MineralsDhahranSaudi Arabia
  5. 5.Center of Research Excellences in NanotechnologyKing Fahd University of Petroleum & MineralsDhahranSaudi Arabia

Personalised recommendations