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Joining of Cf/SiBCN Composite with a Ni-Cr-Pd(Si,B) Filler Alloy

  • Wen-Wen Li
  • Bo Chen
  • Hua-Ping XiongEmail author
  • Yao-Yong Cheng
  • Wen-Jiang Zou
Article
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Abstract

Joining of Cf/SiBCN composite was conducted by a newly designed Ni-Cr-Pd(Si,B) system filler alloy. The dynamic wettability on the Cf/SiBCN composite was measured by the sessile drop method. The joint microstructure and the fracture surface were analyzed by scanning electron microscope and x-ray diffraction spectrometer. The results showed that the Ni-Cr-Pd(Si,B) filler alloy exhibited a low contact angle of 11.6° on the composite after holding at 1170 °C for 30 min. Element Cr played an active role in the interfacial reaction, and a Cr7C3 reaction layer with a thickness of 8 µm was formed at the surface of the Cf/SiBCN composite. Under the brazing condition of 1170 °C for 10 min, the joint strength at the room temperature reached 66.8 MPa. When the test temperature increased to 600 and 800 °C, the joint strength was even elevated to 90.3 and 81.2 MPa, respectively. The joint strength at high temperature was higher than that at room temperature, and this should be attributed to the improvement of the joint plasticity and the release of the residual thermal stresses within the brazed joint.

Keywords

Cf/SiBCN composite joining joint strength microstructure wettability 

Notes

Acknowledgments

This research work was sponsored by the National Natural Science Foundation of China (Grant Nos. 59905022, 50475160, 51275497 and 51775525). We also thank Aeronautical Science Foundation of China (Grant 2008 ZE21005).

References

  1. 1.
    S.H. Dong, T. Zhao, and C.H. Xu, Synthesis and Thermal Behavior of Polymeric Precursors for Si-B-C-N Ceramic, J. Appl. Polym. Sci., 2010, 118, p 3400–3406CrossRefGoogle Scholar
  2. 2.
    B. Liang, Z.H. Yang, Y.T. Li, J.K. Yuan, D.C. Jia, and Y. Zhou, Ablation Behavior and Mechanism of SiCf/Cf/SiBCN Ceramic Composites with Improved Thermal Shock Resistance Under Oxyacetylene Combustion Flow, Ceram. Int., 2015, 41, p 8868–8877CrossRefGoogle Scholar
  3. 3.
    J. Houska, Ageing Resistance of SiBCN Ceramics, Ceram. Int., 2015, 41, p 7921–7928CrossRefGoogle Scholar
  4. 4.
    J. Houska and S. Kos, SiBCN Materials for High-Temperature Applications: Atomistic Origin of Electrical Conductivity, J. Appl. Phys., 2010, 108, p 782–792CrossRefGoogle Scholar
  5. 5.
    D.X. Li, Z.H. Yang, D.C. Jia, D.X. Wu, Q.S. Zhu, B. Liang, S.J. Wang, and Y. Zhou, Microstructure, Oxidation and Thermal Shock Resistance of Grapheme Reinforced SiBCN Ceramics, Ceram. Int., 2016, 42, p 4429–4444CrossRefGoogle Scholar
  6. 6.
    J.Y. Wang, X.M. Duan, Z.H. Yang, D.C. Jia, and Y. Zhou, Ablation Mechanism and Properties of SiCf/SiBCN Ceramic Composites Under an Oxyacetylene Torch Environment, Corros. Sci., 2014, 82, p 101–107CrossRefGoogle Scholar
  7. 7.
    X. Sun, H.T. Liu, J.S. Li, and H.F. Cheng, Effects of CVD SiBCN Interphases on Mechanical and Dielectric Properties of SiCf/SiC Composites Fabricated via a PIP Process, Ceram. Int., 2016, 42, p 82–89CrossRefGoogle Scholar
  8. 8.
    M. Sun, R.Y. Fu, J. Chen, X.F. Mao, J. Zhang, Z.H. Yang, and B. Liang, Fabrication and Microstructures of Functional Gradient SiBCN-Nb Composite by Hot Pressing, Mater. Charact., 2016, 114, p 115–121CrossRefGoogle Scholar
  9. 9.
    J.M. Fernandez, R. Asthana, M. Singh, and F.M. Valera, Active Metal Brazing of Silicon Nitride Ceramics Using a Cu-Based Alloy and Refractory Metal Interlayers, Ceram. Int., 2016, 42, p 5447–5454CrossRefGoogle Scholar
  10. 10.
    R. Pan, S. Kovacevic, T. Lin, P. He, D.P. Sekulic, and S.D. Mesarovic, Control of Residual Stresses in 2Si-B-3C-N and Nb Joints by the Ag-Cu-Ti + Mo Composite Interlayer, Mater. Des., 2016, 99, p 193–200CrossRefGoogle Scholar
  11. 11.
    Y.Q. Qin and J.C. Feng, Active Brazing Carbon/Carbon Composite to TC4 with Cu and Mo Composite Interlayer, Mater. Sci. Eng., A, 2009, 525, p 181–185CrossRefGoogle Scholar
  12. 12.
    W.W. Li, B. Chen, Y. Xiong, H.P. Xiong, Y.Y. Cheng, and W.J. Zou, Joining of Cf/SiBCN Composite with Two Ni-Based Brazing Fillers and Interfacial Reactions, J. Mater. Sci. Technol., 2017, 33, p 487–491CrossRefGoogle Scholar
  13. 13.
    J.Q. Peng, H.J. Seifert, and F. Aldinger, Thermal Expansion Behavior of Precursor-Derived Amorphous Si-C-N and Si-B-C-N Ceramics, J. Mater. Sci. Technol., 2002, 18, p 139–142CrossRefGoogle Scholar
  14. 14.
    C.G. Pan, H.C. Wang, H.F. Wang, and J.L. Zhou, Thermal Parameters Research of Laser Cladding Ni60-Cr3C2 Cermets on Surface of Hot Forging Dies (热锻模表面激光熔覆Ni60-Cr3C2金属陶瓷的热物性参数研究), China Surf. Eng., 2010, 23, p 35–38 ((in Chinese))Google Scholar
  15. 15.
    N. Yoshikuni, K. Nishimoto, and K. Saida, Improvement in Bonding Strength of Si3N4 to Metals Joints by Controlling Reaction Layer Thickness, J. Jpn. Weld. Soc., 1993, 11, p 294–300CrossRefGoogle Scholar
  16. 16.
    W.-W. Li, B. Chen, H.-P. Xiong, and W.-J. Zou, Brazing SiC Matrix Composites Using Co-Ni-Nb-V Alloy, Weld. World, 2017, 33, p 487–491Google Scholar
  17. 17.
    X.Q. Li, L. Li, K. Hu, and S.G. Qu, Vacuum Brazing of TiAl-Based Intermetallics with Ti-Zr-Cu-Ni-Co Amorphous Alloy as Filler Metal, Intermetallics, 2015, 57, p 7–16CrossRefGoogle Scholar
  18. 18.
    H.P. Xiong, W. Dong, B. Chen, Y.S. Kang, A. Kawasaki, H. Okamura, and R. Watanabe, Wettability of Ni-V, Co-V, and Ni-Cr-V System Brazing Alloys on Si3N4 Ceramic and Interfacial Reactions, Mater. Sci. Eng., A, 2008, 474, p 376–381CrossRefGoogle Scholar
  19. 19.
    C. Jian, H. Chen, Q.Y. Wang, and Y.X. Li, Effect of Brazing Temperature and Holding Time on Joint Properties of Induction Brazed WC-Co/Carbon Steel Using Ag-Based Alloy, J. Mater. Process. Technol., 2016, 229, p 562–569CrossRefGoogle Scholar
  20. 20.
    H.P. Xiong, B. Chen, Y.S. Kang, W. Mao, A. Kawasaki, H. Okamura, and R. Watanabe, Wettability of Co-V, and Pd-Ni-Cr-V System Alloys on SiC Ceramic and Interfacial Reactions, Scr. Mater., 2007, 56, p 173–176CrossRefGoogle Scholar
  21. 21.
    J.S. Park, K. Landry, and J.H. Perepezko, Kinetic Control of Silicon Carbide/Metal Reactions, Mater. Sci. Eng., A, 1999, 259, p 279–286CrossRefGoogle Scholar
  22. 22.
    A.R. Miedema, F.R. de Boer, R. Boom, and J.W.F. Dorleijn, Tables for the Heat of Solution of Liquid Metals in Liquid Metal Solvents, Calphad, 1977, 1, p 353–359CrossRefGoogle Scholar
  23. 23.
    Y. Sun, J. Zhang, Y.P. Geng, K. Ikeuchi, and T. Shibayanagi, Microstructure and mecanical proprties of an Si3N4/Si3N4 joit braed with Au-Ni-Pd-V filer ally, Scr. Mater., 2011, 64, p 414–417CrossRefGoogle Scholar
  24. 24.
    K. Bhanumurthy and J.C. Schuster, Interface Reactions Between Silicon Carbide and Metals (Ni, Cr, Pd, Zr), Compos. Part A Appl. Sci., 2001, 32, p 569–574CrossRefGoogle Scholar
  25. 25.
    H.P. Xiong, B. Chen, Y. Pan, and L. Ye, Joining of Cf/SiC Composite with a Cu-Au-Pd-V Brazing Filler and Interfacial Reactions, J. Eur. Ceram. Soc., 2014, 34, p 1481–1486CrossRefGoogle Scholar
  26. 26.
    C.L. Ou, D.W. Liaw, Y.C. Du, and R.K. Shiue, Brazing of 422 Stainless Steel Using the AWS Classification BNi-2 Braze Alloy, J. Mater. Sci., 2006, 41, p 6353–6361CrossRefGoogle Scholar
  27. 27.
    F. Gao, H.Y. Xu, and Y. Ma, Study on the Properties of Cr7C3-NiCr and Cr23C6-Ni Coatings Deposited by HVOF Processes (超音速火焰喷涂Cr7C3-NiCr, Cr23C6-Ni涂层性能研究), Powder. Metall. Technol., 2014, 32, p 335–337 ((in Chinese))Google Scholar
  28. 28.
    H.P. Xiong, W. Mao, Y.H. Xie, B. Chen, W.L. Guo, X.H. Li, and Y.Y. Cheng, Control of the Interfacial Reactions and Strength of SiC/SiC Joints Brazed with Newly-Developed Co-Based Brazing Alloy, J. Mater. Res., 2007, 22, p 2727–2736CrossRefGoogle Scholar
  29. 29.
    A.M. Hadian and R.A.L. Drew, Strength and Microstructure of Silicon Nitride Ceramics Brazed with Nickel-Chromium-Silicon Alloys, J. Am. Ceram. Soc., 1996, 79, p 659–665CrossRefGoogle Scholar
  30. 30.
    M. Cekada, P. Panjan, M. Macek, and P. Smid, Comparison of Structural and Chemical Properties of Cr-Based Hard Coatings, Surf. Coat. Technol., 2002, 151–152, p 31–35CrossRefGoogle Scholar
  31. 31.
    J. Zhang, M. Naka, and Y. Zhou, Brazing Si3N4 Ceramic Using a Cu-Pd-Ti Filler Alloy for High-Temperature Applications, J. Mater. Sci., 2004, 39, p 3159–3161CrossRefGoogle Scholar
  32. 32.
    J.R. Mcdermid, M.D. Pugh, and R.A.L. Drew, The Interaction of Reaction-Bonded Silicon Carbide and Inconel 600 with a Nickel-Based Brazing Alloy, Metall. Mater. Trans. A, 1989, 20, p 1803–1810CrossRefGoogle Scholar
  33. 33.
    W. Qi, J. Lu, S. Xu, S. Zhong, B. Wang, and X. Qiu, Vacuum Brazing Diamond Grits with Cu-Based or Ni-Based Filler Metal, J. Mater. Eng. Perform., 2017, 26, p 4112–4120CrossRefGoogle Scholar
  34. 34.
    Q. Tong and L. Cheng, Liquid Infiltration Joining of 2D C/SiC Composite, Sci. Eng. Compos. Mater., 2006, 13, p 31–36CrossRefGoogle Scholar
  35. 35.
    J.H. Xiong, J.H. Huang, H. Zhang, and X.K. Zhao, Joining of Cf/SiC Composite and TC4 Using Ag-Al-Ti Active Brazing Alloy, J. Mater. Eng. Perform., 2011, 20, p 1084–1089CrossRefGoogle Scholar
  36. 36.
    J. Zhang and L.Y. Jin, Numerical Simulation of Residual Stress in Brazing Joint Between Cemented Carbide and Steel, Mater. Sci. Technol., 2005, 21, p 1455–1459CrossRefGoogle Scholar
  37. 37.
    J.X. Zhang, R.S. Chandel, Y.Z. Chen, and H.P. Seow, Effect of Residual Stress on the Strength of an Alumina-Steel Joint by Partial Transient Liquid Phase (PTLP) Brazing, J. Mater. Process. Technol., 2002, 122, p 220–225CrossRefGoogle Scholar
  38. 38.
    N. Li, S. Huang, G. Zhang, R. Qin, W. Liu, H. Xiong, G. Shi, and J. Blackbum, Progress in Additive Manufacturing on New Materials: A Review, J. Mater. Sci. Technol., 2019, 35, p 242–269CrossRefGoogle Scholar
  39. 39.
    W. Li, B. Chen, H. Xiong, W. Zou, and H. Ren, Joining of Cf/SiC Composite to GH783 Superalloy with NiPdPtAu-Cr Filler Alloy and A Mo Interlayer, J. Mater. Sci. Technol., 2019, 35, p 2099–2106CrossRefGoogle Scholar
  40. 40.
    H. Xiong, W. Mao, Y. Xie, W. Guo, X. Li, and Y. Cheng, Brazing of SiC to a Wrought Nickel-based Superalloy Using CoFeNi(Si,B)CrTi Filler Metal, Mater. Lett., 2007, 61, p 4662–4665CrossRefGoogle Scholar
  41. 41.
    J. Fernie, R. Drew, and K. Knowles, Joining of Engineering Ceramics, Int. Mater. Reviews., 2009, 54, p 283–331CrossRefGoogle Scholar

Copyright information

© ASM International 2019

Authors and Affiliations

  • Wen-Wen Li
    • 1
  • Bo Chen
    • 1
  • Hua-Ping Xiong
    • 1
    Email author
  • Yao-Yong Cheng
    • 1
  • Wen-Jiang Zou
    • 1
  1. 1.Welding and Plastic Forming DivisionBeijing Institute of Aeronautical MaterialsBeijingChina

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