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Stability improvement under high efficiency—next stage development of perovskite solar cells

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Abstract

With efficiency of perovskite solar cells (PSCs) overpassing 23%, to realize their commercialization, the biggest challenge now is to boost the stability to the same level as conventional solar cells. Thus, tremendous effort has been directed over the past few years toward improving the stability of these cells. Various methods were used to improve the stability of bulk perovskites, including compositional engineering, interface adjustment, dimensional manipulation, crystal engineering, and grain boundary decoration. Diverse device configurations, carrier transporting layers, and counter electrodes are investigated. To compare the stability of PSCs and clarify the degradation mechanism, diverse characterization methods were developed. Overall stability of PSCs has become one central topic for the development of PSCs. In this review, we summarize the state-of-the-art progress on the improvement of device stability and discuss the directions for future research, hoping it provides an overview of the current status of the research on the stability of PSCs and guidelines for future research.

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Acknowledgements

This work was supported by the the National Key Research and Development Program of China (2015AA034601, 2016YFA0204000), the National Natural Sciences Foundation of China (21571129, 21702069, 91733301, 91433203, 61474049, 51502141, 51761145042, 51627803, 91433205, 51421002, 11874402), ShanghaiTech Start-up Funding, the Fundamental Research Funds for the Central Universities, the Program for HUST Academic Frontier Youth Team, the Science and Technology Department of Hubei Province (2017AAA190) and the Double first-class research funding of China-EU Institute for Clean and Renewable Energy (RP-2018-SOLAR-001, RP-2018-SOLAR-002), and the International Partnership Program of Chinese Academy of Sciences (112111KYSB20170089). J. Shi and Q. Meng appreciate the valuable help from Mr. Jionghua Wu and Ms. Yiming Li of Institute of Physics, Chinese Academy of Sciences.

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  1. These authors contributed equally to this work.

Authors and Affiliations

  1. School of Physical Science and Technology, Shanghai Tech University, Shanghai, 201210, China

    Danni Yu, Haoying Tang & Zhijun Ning

  2. Michael Grätzel Center for Mesoscopic Solar Cells, Wuhan National Laboratory for Optoelectronics, Huazhong University of Science and Technology, Wuhan, 430074, China

    Yue Hu, Wenhao Zhang & Hongwei Han

  3. Key Laboratory for Renewable Energy, Beijing Key Laboratory for New Energy Materials and Devices, Institute of Physics, Chinese Academy of Sciences, Beijing, 100190, China

    Jiangjian Shi & Qingbo Meng

  4. Key Laboratory for Advanced Materials and Institute of Fine Chemicals, East China University of Science and Technology, Shanghai, 200237, China

    He Tian

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  1. Danni Yu
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  2. Yue Hu
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  3. Jiangjian Shi
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  4. Haoying Tang
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  6. Qingbo Meng
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  7. Hongwei Han
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  8. Zhijun Ning
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  9. He Tian
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Corresponding authors

Correspondence to Qingbo Meng, Hongwei Han or Zhijun Ning.

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Yu, D., Hu, Y., Shi, J. et al. Stability improvement under high efficiency—next stage development of perovskite solar cells. Sci. China Chem. 62, 684–707 (2019). https://doi.org/10.1007/s11426-019-9448-3

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  • DOI: https://doi.org/10.1007/s11426-019-9448-3

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