Journal of Structural Chemistry

, Volume 50, Supplement 1, pp 14–21 | Cite as

Topology features of chemically homogeneous sublattices in crystal structures

  • V. N. Serezhkin
  • D. V. Pushkin
  • L. B. Serezhkina
Article

Abstract

Using Voronoi-Dirichlet polyhedra, the principle of maximum space filling in sublattices containing atoms of a particular element (from H to Cf) is tested in the structures of all crystalline compounds studied so far. It is found that atoms of the overwhelming majority of elements are most often surrounded by 14 neighboring atoms in these sublattices. Anomalous features of H- and C-sublattices, in which hydrogen and carbon atoms most commonly have 15 and 16 neighboring atoms respectively, and sublattices consisting of Ar, Ac, Pa, Am, Cm, Bk, or Cf atoms, in which the number of nearest neighboring atoms is usually 12, are discovered. The main reasons for the revealed differences are discussed.

Keywords

principle of maximum space filling crystal structures atomic sublattices Voronoi-Dirichlet polyhedra 

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References

  1. 1.
    B. K. Vainshtein, V. M. Fridkin, and V. L. Indenbom, Modern Crystallography in four Volumes [in Russian], Vol. 2, Nauka, Moscow (1979).Google Scholar
  2. 2.
    T. C. Hales, Annals Mathem., 162, No. 3, 1065 (2005).CrossRefGoogle Scholar
  3. 3.
    G. B. Bokii, Crystal Chemistry [in Russian], Nauka, Moscow (1971).Google Scholar
  4. 4.
    W. P. Pearson, Crystal Chemistry and Physics of Metals and Alloys, Wiley, New York (1972).Google Scholar
  5. 5.
    V. S. Urusov, Theoretical Crystal Chemistry [in Russian], Izd. Mosk. Gos. Univ., Moscow (1987).Google Scholar
  6. 6.
    A. F. Wells, Structural Inorganic Chemistry, Oxford University Press, Oxford (1984).Google Scholar
  7. 7.
    S. V. Borisov and N. V. Podberezskaya, Stable Cationic Frameworks in the Structures of Fluorides and Oxides [in Russian], Nauka, Novosibirsk (1984).Google Scholar
  8. 8.
    S. V. Borisov, Kristallografiya, 45, No. 5, 779 (2000).Google Scholar
  9. 9.
    A. Vegas, Cryst. Rev., 7, No. 1, 189 (2000).CrossRefGoogle Scholar
  10. 10.
    A. Vegas and M. Jansen, Acta Crystallogr. B58, No. 1, 38 (2002).Google Scholar
  11. 11.
    N. V. Belov, Structure of Ionic Crystals and Metallic Phases [in Russian], Izd. Akad. Nauk SSSR, Moscow (1947).Google Scholar
  12. 12.
    N. V. Belov, Essays on Structural Mineralogy [in Russian], Nedra, Moscow (1976).Google Scholar
  13. 13.
    V. N. Serezhkin, D. V. Pushkin, and L. B. Serezhkina, Koordinats. Khim., 32, No. 11, 832 (2006).Google Scholar
  14. 14.
    V. N. Serezhkin, A. G. Verevkin, D. V. Pushkin, and L. B. Serezhkina, ibid., 34, No. 3, 230 (2008).Google Scholar
  15. 15.
    V. N. Serezhkin, D. V. Pushkin, L. B. Serezhkina, and A. N. Stepanov, ibid., No. 12, 937.Google Scholar
  16. 16.
    J. Conway and N. Sloane, Sphere Packings, Lattices and Groups, Springer-Verlag, New York (1999).Google Scholar
  17. 17.
    V. A. Blatov and V. N. Serezhkin, Russ. J. Inorg. Chem., Suppl, S105 (2000).Google Scholar
  18. 18.
    V. A. Blatov, A. P. Shevchenko, and V. N. Serezhkin, Koordinats. Khim., 25, No. 7, 483 (1999).Google Scholar
  19. 19.
    Inorganic Crystal Structure Database. Gmelin-institut für Anorganische Chemie & FIC Karlsruhe (2007).Google Scholar
  20. 20.
    Cambridge Structural Database System., Version 5.27, Univ. Cambridge, UK.Google Scholar
  21. 21.
    A. I. Gusev, Nonstoichiometry, Disorder, Short-Range and Long-Range Order in a Solid Body [in Russian], Fizmatlit, Moscow (2007).Google Scholar
  22. 22.
    V. A. Blatov and V. N. Serezhkin, Kristallografiya, 40, No. 2, 197 (1995).Google Scholar
  23. 23.
    V. A. Blatov and V. N. Serezhkin, Acta Crystallogr., A53, No. 2, 144 (1997).Google Scholar
  24. 24.
    V. A. Blatov and V. N. Serezhkin, Kristallografiya, 40, No. 6, 965 (1995).Google Scholar

Copyright information

© Pleiades Publishing, Ltd. 2009

Authors and Affiliations

  • V. N. Serezhkin
    • 1
  • D. V. Pushkin
    • 1
  • L. B. Serezhkina
    • 1
  1. 1.Samara State UniversitySamaraRussia

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