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Hydrothermal-photoreduction synthesis of novel Ag@AgBr/BiVO4 plasmonic heterojunction photocatalysts with enhanced activity under white light emitting diode (wLED) irradiation

  • Yongfeng Cai
  • Shiyan Chang
  • Yunfeng Liu
  • Yi ShenEmail author
  • Fengfeng LiEmail author
  • Liangyu Li
  • Shuangshuang Zhu
  • Xiaoyi Zheng
Article

Abstract

Plasmonic heterojunction photocatalysts consisting of silver covered AgBr/BiVO4 structures (Ag@AgBr/BiVO4) were prepared by hydrothermal-photoreduction method. Their phase composition and microstructure were characterized by X-ray diffraction, X-ray photoelectron spectroscopy, scanning electron and transmission electron microscopies. The photo-generated electron–hole pair recombination rate was characterized by I–t curves and photoluminescence measurements. Visible light absorption range of Ag@AgBr/BiVO4 plasmonic heterojunction was significantly enhanced. Ag@AgBr/BiVO4 showed high efficiency for degradation of rhodamine B (RhB) under wLED light. RhB degraded by ~ 82% during 150 min reaction time. Ag@AgBr/BiVO4 photocatalyst remained constant after 8 cycles indicating its extreme stability. Enhancement mechanism of Ag@AgBr/BiVO4 plasmonic heterojunction photocatalyst is discussed.

Notes

Acknowledgements

This work is supported by the National Science Foundation Project of China (Grant Nos. 51772099, 51572069); North China University of Science and Technology Graduate Innovation Project (No. 2018S06); The authors would like to thank shiyanjia lab for the support of HRTEM test.

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Copyright information

© Springer Science+Business Media, LLC, part of Springer Nature 2018

Authors and Affiliations

  • Yongfeng Cai
    • 1
  • Shiyan Chang
    • 1
  • Yunfeng Liu
    • 1
  • Yi Shen
    • 1
    Email author
  • Fengfeng Li
    • 1
    Email author
  • Liangyu Li
    • 1
  • Shuangshuang Zhu
    • 1
  • Xiaoyi Zheng
    • 1
  1. 1.Key Laboratory of Environment Functional Materials of Tangshan City, Hebei Provincial Key Laboratory of Inorganic Nonmetallic Materials, College of Materials Science and EngineeringNorth China University of Science and TechnologyTangshanChina

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