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Journal of Materials Science: Materials in Electronics

, Volume 29, Issue 22, pp 19147–19154 | Cite as

Effect of Na-substitution on magnetoresistance and flux pinning energy of Bi-2212 ceramics prepared via hot-forging process

  • B. Özçelik
  • M. Gürsul
  • F. Karaçora Nane
  • M. A. Madre
  • A. Sotelo
Article
  • 76 Downloads

Abstract

In this study, polymerization method with polyethyleneimine, followed by hot-forging process was used to synthesize bulk textured Bi2Sr2Ca1−xNaxCu2Oy (x = 0.0, 0.05, 0.075 0.1, and 0.15) ceramics. Magnetoresistance performance of samples was studied by change of flux pinning mechanism. The effect of Na-substitution on the magnetoresistance, flux pinning energy, irreversibility field, upper critical magnetic field and coherence length was evaluated in the framework of thermally activated flux flow model. A resistivity transition broadening under various magnetic fields (0–5 T) was analyzed. By using the resistivity data, the upper critical field and the coherence length at T = 0 K were deduced. For \({\text{H}} \bot c~,\) HC2(0) and ξ(0) values were calculated as 31, 31.3, 36.7, 38.3, 35.1 T and 33.1, 32.4, 30.0, 29.3, 30.6 Å, for 0.0, 0.05, 0.075, 0.10, and 0.15 Na-doped samples, respectively. For \({\text{H}}~||c,\) HC2(0) and ξ(0) values were 95 and 112.3 T and 18.6 and 17.1 Å, for the samples of Na0 and Na2, respectively. In particular, the flux pinning or activation energies of Bi2Sr2Ca1−xNaxCu2O8+y where x = 0.10 were determined to be 0.19 eV for 0 T and 0.06 eV for 5 T.

Notes

Acknowledgements

This work is supported by the Research Fund of Çukurova University, Adana, Turkey, under Grant Contracts No. FBA-2014-3500. M.A. Madre, and A. Sotelo wish to thank the Gobierno de Aragón-FEDER (Research Group T 54-17 R), and the Spanish MINECO-FEDER (MAT2017-82183-C3-1-R) for financial support. Authors would like to acknowledge the use of Servicio General de Apoyo a la Investigación-SAI, Universidad de Zaragoza.

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Copyright information

© Springer Science+Business Media, LLC, part of Springer Nature 2018

Authors and Affiliations

  • B. Özçelik
    • 1
  • M. Gürsul
    • 1
  • F. Karaçora Nane
    • 2
  • M. A. Madre
    • 3
  • A. Sotelo
    • 3
  1. 1.Department of Physics, Faculty of Sciences and LettersÇukurova UniversityAdanaTurkey
  2. 2.Department of Electrical and Electronic Engineering, Engineering FacultyHakkari UniversityHakkariTurkey
  3. 3.ICMA (CSIC-Universidad de Zaragoza)ZaragozaSpain

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