Journal of Materials Science

, Volume 45, Issue 11, pp 2843–2851 | Cite as

The anisotropy of ac conductivity and dielectric constant of anisotropic conductor–insulator composites

Article

Abstract

We study the complex ac admittance tensor (ac conductivity and dielectric constant) of anisotropic conductor–insulator composite materials, based on anisotropic two-dimensional RC-networks consisting of randomly placed conductors and capacitors with different conductor existence (bond occupation) probabilities in two directions. We calculate numerically each component of the complex ac admittance tensor by applying a transfer matrix method and reveal the effect of the anisotropy of the bond occupation probability on the frequency characteristics of the ac admittance tensor. It is found that the dual relation holds for each diagonal component of the complex admittance tensor of the anisotropic two-dimensional RC-network. For the effective conductance in the metallic region, the anisotropy depends not only on the anisotropy of the bond occupation probability, but also on the frequency ω. We derive the analytical relation between the anisotropy of the conductance and the anisotropy of the bond occupation probability, at both the dc limit and ω RC = 1. The calculated results on the ac admittance are compared with the effective medium theory and how the accuracy of the theory is related with the microscopic current path is clarified.

Keywords

Vertical Component Percolation Threshold Transfer Matrix Method Effective Conductance Dual Relation 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

Notes

Acknowledgements

We acknowledge Dr. Shigeru Kohinata in Sumitomo Metal Mining Co. for stimulating discussion on high frequency conductance on conductive epoxy adhesive.

References

  1. 1.
    Nakai T, Shimoji T, Tanaka M, Nakajima K, Kohinata S (1994) Proceedings of the eighth international microelectronics conference, p 167Google Scholar
  2. 2.
    Song Y, Noh TW, Lee S-I, Gaines JR (1986) Phys Rev B 33:904CrossRefADSGoogle Scholar
  3. 3.
    Wu J, McLachlan DS (1998) Phys Rev B 58:14880CrossRefADSGoogle Scholar
  4. 4.
    Chiteme C, McLachlan DS (2003) Phys Rev B 67:024206CrossRefADSGoogle Scholar
  5. 5.
    Jhans H, Kim D, Rasmussen RJ, Honig JM (1996) Phys Rev B 54:11224CrossRefADSGoogle Scholar
  6. 6.
    Chiteme C, McLachlan DS, Sauti G (2007) Phys Rev B 75:094202CrossRefADSGoogle Scholar
  7. 7.
    Bergman DJ (1992) Solid State Phys 46:147CrossRefADSGoogle Scholar
  8. 8.
    Landauer R (1952) J Appl Phys 23:779CrossRefADSGoogle Scholar
  9. 9.
    Kirkpatrick S (1973) Rev Mod Phys 45:574CrossRefADSGoogle Scholar
  10. 10.
    Efros AL, Shklovskii BI (1976) Phys Stat Sol b 76:475CrossRefADSGoogle Scholar
  11. 11.
    Bergman DJ, Imry Y (1977) Phys Rev Lett 39:1222CrossRefADSGoogle Scholar
  12. 12.
    Bergman DJ, Imry Y (1981) Phys Rev Lett 14:855Google Scholar
  13. 13.
    Derrida B, Vannimenus J (1982) J Phys A 15:L557CrossRefMathSciNetADSGoogle Scholar
  14. 14.
    Wilkinson D, Langer JS, Sen PN (1983) Phys Rev B 28:1081CrossRefADSGoogle Scholar
  15. 15.
    Newman MEJ, Ziff RM (2000) Phys Rev Lett 85:4104CrossRefPubMedADSGoogle Scholar
  16. 16.
    Yoshida K, Tomi Y, Ueda S (1988) Jpn J Appl Phys 27:2224CrossRefADSGoogle Scholar
  17. 17.
    Dianoux R, Smilde HJH, Marchi F, Buffet N, Mur P, Comin F, Chevrier J (2005) Phys Rev B 71:125303CrossRefADSGoogle Scholar
  18. 18.
    Stankovich S, Dikin DA, Dommett GHB, Kohlaas KM, Zimney EJ, Stach EA, Piner RD, Nguyen ST, Ruoff RS (2006) Nature 442:282CrossRefPubMedADSGoogle Scholar
  19. 19.
    Grujicic M, Cao G, Roy WN (2004) J Mater Sci 39:4441. doi: 10.1023/B:JMSC.0000034136.11779.96 CrossRefADSGoogle Scholar
  20. 20.
    Du F, Fisher JE, Winey KI (2005) Phys Rev B 72:121404(R)ADSGoogle Scholar
  21. 21.
    Lobb CJ, Frank DJ, Tinkham M (1981) Phys Rev B 23:2262CrossRefMathSciNetADSGoogle Scholar
  22. 22.
    Shklovskii BI (1978) Phys Stat Sol b 85:K111CrossRefADSGoogle Scholar
  23. 23.
    Smith LN, Lobb CJ (1979) Phys Rev B 20:3653CrossRefADSGoogle Scholar
  24. 24.
    Nakanishi H, Reynols PJ, Render S (1981) J Phys A 14:855CrossRefADSGoogle Scholar
  25. 25.
    Murtanto TB, Natori S, Nakamura J, Natori A (2006) Phys Rev B 74:115206CrossRefADSGoogle Scholar
  26. 26.
    Dykhne AM (1971) Sov Phys JETP 32:63ADSGoogle Scholar
  27. 27.
    Bernasconi J (1974) Phys Rev B 9:4575CrossRefADSGoogle Scholar
  28. 28.
    Bergman DJ, Duering E, Murat M (1990) J Stat Phys 58:1CrossRefADSGoogle Scholar

Copyright information

© Springer Science+Business Media, LLC 2010

Authors and Affiliations

  1. 1.Department of Electronic-EngineeringThe University of Electro-CommunicationsTokyoJapan

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