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Environmental Monitoring and Assessment

, Volume 169, Issue 1–4, pp 335–345 | Cite as

Analysis of spatial–temporal distributions of nitrate-N concentration in Shitoukoumen catchment in northeast China

  • Jun Li
  • Wenxi LuEmail author
  • Xiankui Zeng
  • Jiehui Yuan
  • Furong Yu
Article

Abstract

This article discusses the generation and migration process of nitrate-N pollution in shallow groundwater caused by agricultural nonpoint source pollution in the catchment area of Shitoukoumen Reservoir in northeast China. By monitoring the shallow groundwater nitrate-N in the low-water period, the normal season, and high-flow period in the study area for a year, it was found that the nitrate-N concentration in the shallow groundwater of this area had a seasonal variation in both spatial and time distribution. In the time distribution, the peak value appeared in July, the high-flow period, and the valley value appeared in April, the low-water period, and showed a significant correlation with the time distribution of fertilization rate and rainfall. In the spatial distribution of nitrate-N pollution, when the distribution in shallow groundwater was analyzed separately in the three different periods (low-water period, the normal season, and high-flow period) and the discipline transference and enrichment of nitrate-N pollution in shallow groundwater was determined, this indicated that the region in the southeast study area where runoff conditions were better was less contaminated, and the region where runoff conditions were poor, as well as the region along the river were seriously polluted. The nitrate-N concentration in shallow groundwater was distributed mainly along the path of groundwater flow and was excreted in the drainage region. This showed that the spatial distribution of nitrate-N concentration in the shallow groundwater of the entire region was mainly controlled by the groundwater flow system. At the same time, in the middle and lower reaches of the study area, the seasonal changes in the recharged–excreted relationship between groundwater and river caused seasonal differences in the spatial distribution of nitrate-N pollution in groundwater. The combined effects of the groundwater mobility and the surface river resulted in a poor correlation between the groundwater nitrate-N concentration and land-use types. Only in the plain area where there was little influence from groundwater runoff and the surface river did the groundwater nitrate-N concentration correlate with land-use types. The spatial and time distribution of nitrate-N concentration in the shallow groundwater of the study area was impacted by agricultural nonpoint source pollution, the groundwater flow system, and the surface river and formed a concentration response system which uses basins as a unit.

Keywords

Nitrate-N Nonpoint source pollution Shallow groundwater China 

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References

  1. Canadela, L. (1991). Diffused pollution of groundwater by agriculture: A study in the Maresme area of Barcelona[M]. Spain. Proc. Int. Conf. Environ. Pollute.Google Scholar
  2. Dong, W. H., & Lin, X. Y. (2004). Analysis on the influence factors of the nitrogen pollution in shallow groundwater—A case in the north high plain of Songhua River in Songnen Basin [J]. Journal of Jilin University (Earth Science Edition), 34(2), 231–235 (in Chinese).Google Scholar
  3. Editorial Board of China Agriculture Almanac (2003). Almanac of China Agriculture[M]. Beijing: China Agriculture Press (in Chinese).Google Scholar
  4. Foreman, J. K., & Gcodhead, K. (1975). The formation and analysis of N-nitrosamine[J]. Journal of the Science of Food and Agriculture, (26), 1771.Google Scholar
  5. Goss, M. J., Barry, D. A. J., & Rudolph, D. L. (1998). Contamination in Ontario farmstead domestic wells and its association with agriculture: 1. Results from drinking water wells[J]. Journal of Contaminant Hydrology, 32(3–4), 267–293.CrossRefGoogle Scholar
  6. Lin, X. Y., & Chen, M. X. (2000). Study on groundwater resources and sustainable development in Songnen Basin[M]. Beijing: Seismological Publishing House (in Chinese).Google Scholar
  7. Liu, Y., & Zhao, Y. X. (2004). Chinese and foreign experts call on: Agricultural nonpoint source pollution has been to control[EB/OL]. Demos net, http://finance.sina.com.cn/chanjing/b/20041102/15031126447.shtml, 2004–11–02 (in Chinese).
  8. Liu, H. B., Lei, B. K., & Zhang, Y. G. (2001). Investigation and evaluation on nitrate pollution in groundwater of Shunyi District[J]. Plant Nutrition and Ferti1izer Science, 7(4), 385–390 (in Chinese).Google Scholar
  9. Liu, G. D., Wu, W. L., & Zhang, J. (2005). Regional differentiation of nonpoint source pollution of agriculture-derived nitrate-N in groundwater in northern China[J]. Agriculture, Ecosystems and Environment, 107, 211–220.CrossRefGoogle Scholar
  10. Liu, H. B., Li, Z. H., & Zhang, Y. G. (2006). Nitrate contamination of groundwater and its affecting factors in rural areas of Beijing plain[J]. Acta Pedologica Sinica, 43(3), 405–413 (in Chinese).Google Scholar
  11. Liu, X. C., Wang, R., & Sun, Z. X. (2008). Nitrate contamination of drinking-water in three types of crop-producing areas in Liaoning Province[J]. Journal of Irrigation and Drainage, 27(5), 9–13 (in Chinese).Google Scholar
  12. Lu, D. Q., Dong, Y. A., & Sun, B. H. (1998). Study on effect of nitrogen fertilizer use on environment pollution[J]. Plant Nutrition and Fertilizer Science, 4(1), 8–15 (in Chinese).Google Scholar
  13. Lu, S. H., Zen, X. Z., Zhang, F. S., et al. (2002). Investigation on nitrate pollution of groundwater in countryside of Chengdu city[J]. Acta Pedologica Sinica, 39, 286–193 (in Chinese).Google Scholar
  14. Ma, L. S., Wang, Z. Q., Zhang, S. M., et al. (1997). Pollution from agricultural nonpoint sources and its control in river system of Taihu lake, Jiangsu. Acta Scientiae Circumstantiae, 17(1), 39–47 (in Chinese).Google Scholar
  15. Qiao, G. J., Zhang, J. L., & Tang, J. Z. (2004). Mechanism analysis and management measures of nitrogen pollution of groundwanter[J]. Water Resources Protection, (3), 9–12 (in Chinese).Google Scholar
  16. Spiegelhalder, B., Eisenbrand, G., & Preussmann, R. (1976). Influence of dietary nitrate on nitrite content of human saliva: Possible relevance to in vivo formation of N-nitroso compounds[J]. Food and Cosmetics Toxicology, 14(6), 545–548.CrossRefGoogle Scholar
  17. Thorbum, P. J., Biggs, J. S., Weier, K. L., et al. (2003). Nitratein groundwater of intensive agricultural areas in coastal Northeastern Australia[J]. Agriculture, Ecosystems and Environment, 94, 49–58.CrossRefGoogle Scholar
  18. Ye, S. G., & Wang, S. (2008). Studies on prevention of agricultural nonpoint pollution in water source areas [J]. China Water Resources, (5), 18–20 (in Chinese).Google Scholar
  19. Zhang, M. Q., Gao, H. X., & Wu, K. J. (1990). Analysis of environmental conditions of Matan nitrate polluted water resource region in Lanzhou City. Environmental Science, 11(5), 79–82 (in Chinese).Google Scholar
  20. Zhang, W. L., Wu, S. X., Ji, H. J., et al. (2004). Estimation of agricultural nonpoint source pollution in China and the alleviating strategies[J]. Scientia Agriculture Sinica, 37(7), 1008–1017 (in Chinese).Google Scholar

Copyright information

© Springer Science+Business Media B.V. 2009

Authors and Affiliations

  • Jun Li
    • 1
    • 2
  • Wenxi Lu
    • 2
    Email author
  • Xiankui Zeng
    • 2
  • Jiehui Yuan
    • 2
  • Furong Yu
    • 2
  1. 1.State Key Laboratory of Hydraulics and, Mountain River EngineeringChengduPeople’s Republic of China
  2. 2.College of Environment and ResourcesJilin UniversityChangchunPeople’s Republic of China

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