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Environmental Geochemistry and Health

, Volume 40, Issue 5, pp 1867–1876 | Cite as

Combined ultrasound with Fenton treatment for the degradation of carcinogenic polycyclic aromatic hydrocarbons in textile dying sludge

  • Jian-Hao Zhang
  • Hai-Yuan Zou
  • Xun-An Ning
  • Mei-Qing Lin
  • Chang-Min Chen
  • Tai-Cheng An
  • Jian Sun
Original Paper

Abstract

To develop an effective method to remove the toxic and carcinogenic polycyclic aromatic hydrocarbons (CPAHs) from textile dyeing sludge, five CPAHs were selected to investigate the degradation efficiencies using ultrasound combined with Fenton process (US/Fenton). The results showed that the synergistic effect of the US/Fenton process on the degradation of CPAHs in textile dyeing sludge was significant with the synergy degree of 30.4. During the US/Fenton process, low ultrasonic density showed significant advantage in degrading the CPAHs in textile dyeing sludge. Key reaction parameters on CPAHs degradation were optimized by the central composite design as followed: H2O2 concentration of 152 mmol/L, ultrasonic density of 408 W/L, pH value of 3.7, the molar ratio of H2O2 to Fe2+ of 1.3 and reaction time of 43 min. Under the optimal conditions of the US/Fenton process, the degradation efficiencies of five CPAHs were obtained as 81.23% (benzo[a]pyrene) to 84.98% (benz[a]anthracene), and the benzo[a]pyrene equivalent (BaPeq) concentrations of five CPAHs declined by 81.22–85.19%, which indicated the high potency of US/Fenton process for removing toxic CPAHs from textile dyeing sludge.

Keywords

Carcinogenic polycyclic aromatic hydrocarbons Textile dyeing sludge Ultrasound Fenton Central composite design 

Notes

Acknowledgements

This research was supported by the Natural Science Foundation of China (No. 21577027); Science and Technology Project of Guangdong Province, China (No. 2015A020215032); Special Applied Technology Research and Development Key Project of Guangdong Province (No. 2015B020235013); and the Science and Technology Project of Guangzhou city (No. 201607010330).

Supplementary material

10653_2017_9946_MOESM1_ESM.docx (2.4 mb)
Supplementary material 1 (DOCX 2460 kb)

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Copyright information

© Springer Science+Business Media Dordrecht 2017

Authors and Affiliations

  • Jian-Hao Zhang
    • 1
  • Hai-Yuan Zou
    • 1
  • Xun-An Ning
    • 1
  • Mei-Qing Lin
    • 1
  • Chang-Min Chen
    • 1
  • Tai-Cheng An
    • 1
  • Jian Sun
    • 1
  1. 1.School of Environmental Science and Engineering, Institute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhouChina

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