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Catalysis Letters

, Volume 144, Issue 10, pp 1661–1666 | Cite as

Ceria Prepared by Flame Spray Pyrolysis as an Efficient Catalyst for Oxidation of Diesel Soot

  • Jakob M. Christensen
  • Davide Deiana
  • Jan-Dierk Grunwaldt
  • Anker D. JensenEmail author
Article

Abstract

Ceria has been prepared by flame spray pyrolysis and tested for activity in catalytic soot oxidation. In tight contact with soot the oxidation activity (measured in terms of the temperature of maximal oxidation rate, Tmax) of the flame made ceria is among the highest reported for CeO2. This can to a significant degree be ascribed to the large surface area achieved with the flame spray pyrolysis method. The importance of the inherent soot reactivity for the catalytic oxidation was studied using various soot samples, and the reactivity of the soot was found to have a significant impact, as the Tmax-value for oxidation in tight contact with a catalyst scaled linearly with the Tmax-value in non-catalytic soot oxidation. The Tmax-value in non-catalytic soot oxidation was in turn observed to scale linearly with the H/C ratio of the carbonaceous materials.

Graphical Abstract

Keywords

Ceria Soot oxidation Flame spray pyrolysis Nanoparticles 

Notes

Acknowledgments

Financial support from The Danish Council for Strategic Research (DSF) is gratefully acknowledged (Grant no. 2106-08-0039). Martin Høj and Brian Brun Hansen are gratefully acknowledged for aid in connection with the experimental work.

Supplementary material

10562_2014_1319_MOESM1_ESM.docx (3.8 mb)
Supplementary material 1 (DOCX 3924 kb)

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Copyright information

© Springer Science+Business Media New York 2014

Authors and Affiliations

  • Jakob M. Christensen
    • 1
  • Davide Deiana
    • 2
  • Jan-Dierk Grunwaldt
    • 1
    • 3
  • Anker D. Jensen
    • 1
    Email author
  1. 1.Department of Chemical and Biochemical EngineeringTechnical University of DenmarkKgs LyngbyDenmark
  2. 2.Center for Electron NanoscopyTechnical University of DenmarkKgs. LyngbyDenmark
  3. 3.Institute for Technical and Polymer ChemistryKarlsruhe Institute of TechnologyKarlsruheGermany

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