Meteorology and Atmospheric Physics

, Volume 119, Issue 1–2, pp 59–70 | Cite as

Impact of chemical and meteorological boundary and initial conditions on air quality modeling: WRF-Chem sensitivity evaluation for a European domain

  • Mathias Ritter
  • Mathias D. Müller
  • Oriol Jorba
  • Eberhard Parlow
  • L.-J. Sally Liu
Original Paper

Abstract

This study evaluates the impact of different chemical and meteorological boundary and initial conditions on the state-of-the-art Weather Research and Forecasting (WRF) model with its chemistry extension (WRF-Chem). The evaluation is done for July 2005 with 50 km horizontal resolution. The effect of monthly mean chemical boundary conditions derived from the chemical transport model LMDZ-INCA on WRF-Chem is evaluated against the effect of the preset idealized profiles. Likewise, the impact of different meteorological initial and boundary conditions (GFS and Reanalysis II) on the model is evaluated. Pearson correlation coefficient between these different runs range from 0.96 to 1.00. Exceptions exists for chemical boundary conditions on ozone and for meteorological boundary conditions on PM10, where coefficients of 0.90 were obtained. Best results were achieved with boundary and initial conditions from LMDZ-INCA and GFS. Overall, the European simulations show encouraging results for observed air pollutant, with ozone being the most and PM10 being the least satisfying.

Notes

Acknowledgments

This study was supported by the Swiss National Science Foundation and is part of the SAPALDIA study. Further supporters are the Federal Office for Forest, Environment and Landscape; the Federal Office of Public Health; the Federal Office of Roads and Transport; the cantons government of Aargau, Basel-Stadt, Basel-Land, Geneva, Luzern, Ticino, and Zurich; the Swiss Lung League; the Lung Leagues of Basel-Stadt/Basel-Landschaft, Geneva, Ticino, and Zurich. The work has been performed under the HPC-EUROPA2 project (project number: 228398) with the support of the European Commission—Capacities Area—Research Infrastructures. Data from the GENEMIS project coordinated by the Institute of Energy Economics and the Rational Use of Energy (IER) at the University of Stuttgart have been used.

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Copyright information

© Springer-Verlag Wien 2012

Authors and Affiliations

  • Mathias Ritter
    • 1
    • 2
    • 3
  • Mathias D. Müller
    • 1
  • Oriol Jorba
    • 4
  • Eberhard Parlow
    • 1
  • L.-J. Sally Liu
    • 2
    • 5
    • 6
  1. 1.Meteorology, Climatology and Remote SensingUniversity of BaselBaselSwitzerland
  2. 2.Environmental Exposure Sciences, Department of Epidemiology and Public HealthSwiss Tropical and Public Health InstituteBaselSwitzerland
  3. 3.BaselSwitzerland
  4. 4.Earth Sciences DepartmentBarcelona Supercomputing CenterBarcelonaSpain
  5. 5.University of BaselBaselSwitzerland
  6. 6.Department of Environmental and Occupational Health SciencesUniversity of WashingtonSeattleUSA

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