Applied Physics B

, Volume 79, Issue 1, pp 71–75

Investigation of the spatial profile of stimulated Raman scattering beams in D2 and H2 gases using a pulsed Nd:YAG laser at 266 nm

  • S. Tzortzakis
  • G. Tsaknakis
  • A. Papayannis
  • A.A. Serafetinides
Article

Abstract

The stimulated Raman scattering (SRS) beam spatial mode structure is studied in H2 and D2 gases, in a 60 cm-long high-pressure Raman cell, using a pulsed Nd:YAG laser at 266 nm. The conversion efficiencies of the first and second Stokes in H2, D2 and H2/D2 mixtures have been measured precisely in the 1–14 atm range. The SRS beam profiles were recorded for different gas pressures in the high-pressure Raman cell and interesting behaviour is revealed. Homogeneous SRS spatial profiles were obtained only for pressures higher than 7 atm. For lower pressures the profiles are either in the form of a ring or of a more complicated shape. The results are explained in terms of nonlinear self-focusing processes during the pump beam propagation in the Raman cell. Also, from our measurements, a more precise value of the nonlinear index of refraction for the H2 and D2 at 266 nm is proposed.

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References

  1. 1.
    R. Byer: IEEE J. Quantum Elect. QE-12, 732 (1976) Google Scholar
  2. 2.
    T. Loree, D. Barker, P. Scott: IEEE J. Quantum Elect. QE-15, 337 (1979) Google Scholar
  3. 3.
    D. Cotter, K. White: Opt. Commun. 49, 205 (1984) ADSCrossRefGoogle Scholar
  4. 4.
    X. Cheng, Q. Lou, R. Wang, Z. Wang: Appl. Phys. Lett. 51, 75 (1987) ADSGoogle Scholar
  5. 5.
    G. Stoffels, P. Schmidt, N. Dam, J.J. ter Meulen: Appl. Opt. 36, 6797 (1997) ADSCrossRefGoogle Scholar
  6. 6.
    I. Fischer, T. Schultz: Appl. Phys. B. 64, 15 (1997) ADSCrossRefGoogle Scholar
  7. 7.
    A. Papayannis, G.N. Tsikrikas, A.A. Serafetinides: Appl. Phys. B 67, 563 (1998) ADSCrossRefGoogle Scholar
  8. 8.
    C. Lynga, F. Ossler, T. Metz, J. Larsson: Appl. Phys. B. 72, 913 (2001) ADSCrossRefGoogle Scholar
  9. 9.
    G. Ancellet, A. Papayannis, G. Mégie, J. Pelon: J. Ocean. Atmos. Tech. 6, 832 (1989) CrossRefGoogle Scholar
  10. 10.
    A. Papayannis, G. Ancellet, J. Pelon, G. Mégie: Appl. Opt. 29, 467 (1990) ADSCrossRefGoogle Scholar
  11. 11.
    B. Calpini, V. Simeonov, F. Jeanneret, J. Kuebler, V. Sathya, H. Van Den Bergh: Chimia 51, 700 (1997) Google Scholar
  12. 12.
    E. Durieux, L. Fiorani, B. Calpini, M. Flamm, L. Jaquet, H. Van Den Bergh: Atmos. Environ. 32, 2141 (1998) ADSCrossRefGoogle Scholar
  13. 13.
    Z. Chu, U. Singh, T. Wilkerson: Appl. Opt. 30, 4350 (1991) ADSCrossRefGoogle Scholar
  14. 14.
    W. Carnuth, T. Trickl: Rev. Sci. Instrum. 65, 3324 (1994) ADSCrossRefGoogle Scholar
  15. 15.
    D. Lancaster, J. Dawes: Opt. Commun. 120, 307 (1995) ADSCrossRefGoogle Scholar
  16. 16.
    N.G. Jerlon: Optical Oceanography (Elsevier, New York 1968) Google Scholar
  17. 17.
    B.J. McCall, A.J. Huneycutt, R.J. Saykally, C.M. Lindsay, T. Oka, M. Fushitani, Y. Miyamoto, T. Momose: Appl. Phys. Lett. 82, 1350 (2003) ADSCrossRefGoogle Scholar
  18. 18.
    D. Hanna, D.J. Pointer, D. Pratt: Opt. Commun. 60, 187 (1986) ADSCrossRefGoogle Scholar
  19. 19.
    L. de Schoulepnikoff, V. Mitev, V. Simeonov, B. Calpini, H. Van Der Bergh: Appl. Opt. 36, 5026 (1997) ADSCrossRefGoogle Scholar
  20. 20.
    G. Venkin, L. Kulyuk, D. Maleev: Sov. J. Quantum. Elect. 5, 1348 (1976) ADSCrossRefGoogle Scholar
  21. 21.
    D.A. Haner, S. McDermid: IEEE J. Quantum Elect. QE-26, 1292 (1990) Google Scholar
  22. 22.
    M. Milton, G. Ancellet, A. Apituley, J. Bosenberg, W. Carnuth, F. Castagnoli, T. Trickl, H. Edner, L. Stefanutti, T. Schaberl, A. Sunesson, C. Weitkamp: Appl. Phys. B. 66, 105 (1998) ADSCrossRefGoogle Scholar
  23. 23.
    V. Simeonov, V. Mitev, H. Van Der Bergh, B. Calpini: Appl. Opt. 37, 7112 (1998) ADSCrossRefGoogle Scholar
  24. 24.
    D. Diebel, M. Bristow, R. Zimmermann: Appl. Opt. 30, 626 (1991) ADSCrossRefGoogle Scholar
  25. 25.
    J.L. Carlsten, J. Rifkin, D.C. MacPherson: J. Opt. Soc. Am. B 3, 1476 (1986) ADSCrossRefGoogle Scholar
  26. 26.
    X. Jiangfan, W. Naiyan: IEEE J. Quantum Elect. QE-36, 533 (2000) Google Scholar
  27. 27.
    N. Bloembergen: Am. J. Phys. 35, 989 (1967) ADSCrossRefGoogle Scholar
  28. 28.
    A. Papayannis: Etude Expérimentale de la Distribution Verticale de l’Ozone dans la Troposphère et la Basse Stratosphère par Télédétection Laser: Application aux Echanges Stratosphère-Troposphère et a la Physicochimie de la Couche Limite Atmosphérique. Ph.D. Thesis, Université Paris VII, Paris, France (1989) Google Scholar
  29. 29.
    A. Couairon, S. Tzortzakis, L. Berge, M. Franco, B. Prade, A. Mysyrowicz: J. Opt. Soc. Am. B 19, 1117 (2002) ADSCrossRefGoogle Scholar
  30. 30.
    M.J. Weber: Handbook of Optical Materials (CRC, Boca Raton, FL, 2003) Google Scholar
  31. 31.
    W.E. Martin, R.J. Winfield: Appl. Opt. 27, 567 (1988) ADSCrossRefGoogle Scholar
  32. 32.
    W.G. Rado: Appl. Phys. Lett. 11, 123 (1967) ADSCrossRefGoogle Scholar
  33. 33.
    H. Komine, W.H. Long, E.A. Stappaerts, S.J. Brosnan: J. Opt. Soc. Am. B 3, 1428 (1986) ADSCrossRefGoogle Scholar
  34. 34.
    M. Duncan, R. Mahon, L. Tankersley, J. Reintjes: J. Opt. Soc. Am. B 7, 1336 (1990) ADSCrossRefGoogle Scholar
  35. 35.
    L.Y. Zhu, J. Kim, R.A. Mathies: J. Raman Spectrosc. 30, 777 (1999) ADSCrossRefGoogle Scholar
  36. 36.
    V. Simeonov, G. Larcherveque, P. Quaglia, H. Van Der Bergh, B. Calpini: Appl. Opt. 38, 5186 (1999)ADSCrossRefGoogle Scholar

Copyright information

© Springer-Verlag 2004

Authors and Affiliations

  • S. Tzortzakis
    • 1
  • G. Tsaknakis
    • 1
  • A. Papayannis
    • 1
  • A.A. Serafetinides
    • 1
  1. 1.Lasers and their Applications Group Physics DepartmentNational Technical University of AthensAthensGreece

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