Applied Physics A

, Volume 83, Issue 2, pp 333–336

Ultra-short laser ablation of metals and semiconductors: evidence of ultra-fast Coulomb explosion



We have studied ultra-fast laser ablation of Si and a metal via the neutral and ion yield, the energy distribution of emitted neutrals and the charge distribution as a function of the laser pulse width. Two processes, one leading to the ejection of fast (3–7 eV), the other to slow thermal particles, can be identified. The origin of the first process can be correlated with laser pulse widths (or pump–probe delays) and processes on a time scale below 100 fs. Results for Si confirm recent findings for Coulomb explosion (CE) and we show for the first time that CE exists as a mechanism of material removal from metals for ultra-short laser pulses.


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  1. 1.
    R. Stoian, A. Rosenfeld, D. Ashkenasi, I.V. Hertel, N.M. Bulgakova, E.E. Campbell, Phys. Rev. Lett. 8809, 7603 (2002)Google Scholar
  2. 2.
    W.G. Roeterdink, L.B. Juurlink, O.P. Vaughan, J.D. Diez, M. Bonn, A.W. Kleyn, Appl. Phys. Lett. 82, 4190 (2003)CrossRefADSGoogle Scholar
  3. 3.
    R. Stoian, A. Rosenfeld, I.V. Hertel, N.M. Bulgakova, E.E. Campbell, Appl. Phys. Lett. 85, 694 (2004)CrossRefADSGoogle Scholar
  4. 4.
    W.G. Roeterdink, M. Bonn, A.W. Kleyn, Appl. Phys. Lett. 85, 696 (2004)CrossRefADSGoogle Scholar
  5. 5.
    J. Reif, F. Costache, S. Eckert, M. Henyk, Appl. Phys. A 79, 1229 (2004)CrossRefADSGoogle Scholar
  6. 6.
    N.M. Bulgakova, R. Stoian, A. Rosenfeld, E.E. Campbell, I.V. Hertel, Appl. Phys. A 79, 1153 (2004)ADSGoogle Scholar
  7. 7.
    H.P. Cheng, J.D. Gillaspy, Phys. Rev. B 55, 2628 (1997)CrossRefADSGoogle Scholar
  8. 8.
    A. Cavalleri, K. Sokolowski-Tinten, J. Bialkowski, M. Schreiner, D. v. d. Linde, J. Appl. Phys. 85, 3301 (1999)CrossRefADSGoogle Scholar
  9. 9.
    A. Rousse, C. Rischel, S. Fourmaux, I. Uschmann, S. Sebban, G. Grillon, P. Balcou, E. Forster, J.P. Geindre, P. Audebert, J.C. Gauthier, D. Hulin, Nature 410, 65 (2001)PubMedCrossRefADSGoogle Scholar
  10. 10.
    D. Perez, L.J. Lewis, Phys. Rev. Lett. 89, 4 (2002)CrossRefGoogle Scholar
  11. 11.
    D. Perez, L.J. Lewis, Phys. Rev. B 67, 184102 (2003)CrossRefADSGoogle Scholar
  12. 12.
    E. Leveugle, D.S. Ivanov, L.V. Zhigilei, Appl. Phys. A 79, 1643 (2004)ADSGoogle Scholar
  13. 13.
    C. Schafer, H.M. Urbassek, L.V. Zhigilei, Phys. Rev. B 66, 8 (2002)CrossRefGoogle Scholar
  14. 14.
    V. Schmidt, W. Husinsky, G. Betz, Phys. Rev. Lett. 85, 3516 (2000)CrossRefPubMedADSGoogle Scholar
  15. 15.
    D. Kaplan, P. Tournois, J. Phys. IV 12, 69 (2002)CrossRefGoogle Scholar
  16. 16.
    J. Kanasaki, K. Taniumra, Phys. Rev. B 66, 125320 (2002)CrossRefADSGoogle Scholar
  17. 17.
    P. Lorazo, L.J. Lewis, M. Meunier, Phys. Rev. Lett. 9122, 5502 (2003)Google Scholar
  18. 18.
    K.H. Bennemann, J. Phys.: Condens. Matter 16, 1056 (2004)CrossRefGoogle Scholar
  19. 19.
    B. Rethfeld, A. Kaiser, M. Vicanek, G. Simon, Appl. Phys. A 69, S109 (1999)CrossRefADSGoogle Scholar
  20. 20.
    W.S. Fann, R. Storz, H.W. Tom, J. Bokor, Phys. Rev. Lett. 68, 2834 (1992)CrossRefPubMedADSGoogle Scholar
  21. 21.
    W. Husinsky, H. Dachraoui, C. Matei, G. Betz, in High Power Laser Ablation V (Proc. SPIE 5448), ed. by C.R. Phipps (SPIE, Bellingham, UA, 2004), p 1165Google Scholar
  22. 22.
    S. Amoruso, X. Wang, C. Altucci, C. De Lisio, M. Armenante, R. Bruzzese, R. Velotta, S. Amoruso, Appl. Phys. Lett. 77, 3728 (2000)CrossRefADSGoogle Scholar
  23. 23.
    H. Dachraoui, W. Husinsky, submitted to APLGoogle Scholar
  24. 24.
    A. Assion, T. Baumert, T. Brixner, M. Bergt, B. Kiefer, V. Seyfried, M. Strehle, G. Gerber, Science 282, 919 (1998)CrossRefPubMedADSGoogle Scholar
  25. 25.
    R. Stoian, A. Mermillod-Blondin, S. Winkler, A. Rosenfeld, I.V. Hertel, M. Spyridaki, E. Koudoumas, C. Fotakis, I.M. Burakov, N.M. Bulgakova, Proc. SPIE 5662, 593 (2004)CrossRefADSGoogle Scholar

Copyright information

© Springer-Verlag 2006

Authors and Affiliations

  1. 1.Institut für Allgemeine PhysikVienna University of TechnologyWienAustria

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