Journal of Radioanalytical and Nuclear Chemistry

, Volume 177, Issue 2, pp 291–299 | Cite as

Final purification of uranium-233 oxide product from reprocessing treatment of irradiated thorium rods

  • A. Palamalai
  • S. V. Mohan
  • M. Sampath
  • R. Srinivasan
  • P. Govindan
  • A. Chinnusamy
  • V. R. Raman
  • G. R. Balasubramanian
Article

Abstract

Some batches of233U oxide product obtained from the reprocessing treatment of irradiated thorium rods, called J-rods in our plant, have been found to contain thorium as much as 85% and iron above 5% as impurities. This product has to be purified before sending for fabrication of the fuel. The present purification method consists of the following three steps: (1) preferential dissolution of U3O8 as compared to thoria, (2) a novel solvent extraction process, and (3) preferential precipitation of Th as oxalate leaving behind the entire U in the filtrate. Development and application of the present purification method to the above233U oxide proxduct are presented in this paper.

Keywords

Oxide Iron Precipitation Physical Chemistry Purification 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

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References

  1. 1.
    Unpublished information from our earlier purification work when iron alone was present as the impurity in233U oxide product.Google Scholar
  2. 2.
    R. T. KULKARNI, et al., Separation and purification of U-233 from boron and other impurities, Proc. Symp. on Radiochemistry and Radiation Chemistry, Bhabha Atomic Research Centre, Bombay, India, 26 Feb. 1988.Google Scholar
  3. 3.
    A. PALAMALAI, T. S. THANKACHAN, G. R. BALASUBRAMANIAN, Improvements in biamperometric method for remote analysis of urnaium. Report RRC-39, 1979.Google Scholar
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    USAEC Report, TID, 7015, Method-1218710.Google Scholar
  5. 5.
    J. BASSETT et al., Vogel's Textbook of Quantitative Inorganic Analysis, 4th ed., Longmans' Group Limited, London, 1978, p. 742.Google Scholar

Copyright information

© Akadémiai Kiadó 1994

Authors and Affiliations

  • A. Palamalai
    • 1
  • S. V. Mohan
    • 1
  • M. Sampath
    • 1
  • R. Srinivasan
    • 1
  • P. Govindan
    • 1
  • A. Chinnusamy
    • 1
  • V. R. Raman
    • 1
  • G. R. Balasubramanian
    • 1
  1. 1.Reprocessing ProgrammeIndira Gandhi Centre for Atomic ResearchKalpakkam(India)

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