Analysis for naturally occuring radionuclides at environmental concentrations by gamma spectrometry
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Abstract
The analytical potential of low level, high resolution gamma-ray spectrometry for naturally occurring radionuclides at environmental levels is described, with particular emphasis on detector background levels and sensitivity. Comparisons are drawn between the performance of a specially designed low background detector system, and that of standard “off the shelf” devices. Sample characteristics, calibration procedures and checks, are described, and empirical minimum detection limits of between 0.4 Bq·kg−1 (226Ra,228Th) and 10 Bq·kg−1 (210Pb) are derived for soil or sediment samples of about 250 g. Representative analyses of a variety of environmental samples, including water, plant material, animal tissue and sediment, are given to illustrate the routine use of the spectrometer.
Keywords
Radionuclide Detector System Sediment Sample 210Pb Environmental SamplePreview
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References
- 1.O. G. BARTELS, Health Phys., 38 (1980) 89.Google Scholar
- 2.D. C. CAMP, C. GATROUSIS, L. A. MAYNARD, Nucl. Instr. Methods, 117 (1974) 189.Google Scholar
- 3.J. A. COOPER, R. W. PERKINS, Nucl. Instr. Methods, 99 (1972) 125.Google Scholar
- 4.H. H. CUTSHALL, I. L. LARSEN, C. R. OLSEN, Nucl. Instr. Methods, 206 (1983) 309.Google Scholar
- 5.K. DEBERTIN, U. SCHÖTZIG, Nucl. Instr. Methods, 158 (1978) 471.Google Scholar
- 6.R. J. ELSINGER, P. T. KING, W. S. MOORE, Anal. Chim. Acta, 144 (1982) 277.Google Scholar
- 7.H. L. MALM, M. M. WATT, I. BOSTOCK, J. L. CAMPBELL, P. JAGAM, J. J. SIMPSON, Nucl. Instr. Methods, 223 (1984) 420.Google Scholar
- 8.J. MICHEL, W. S. MOORE, P. T. KING, Anal. Chem., 53 (1981) 1885.Google Scholar
- 9.M. H. MOMENI, Nucl. Instr. Methods, 193 (1982) 185.Google Scholar
- 10.A. S. MURRAY Environmental radioactivity studies relevant to thermoluminescence dating. D. Phil, Thesis, University of Oxford, 1981.Google Scholar
- 11.A. S. MURRAY, M. J. AITKEN, The measurement and importance of radioactive disequilibria in TL samples, in: A Specialist Seminar on Thermoluminescence Dating, PACT, 6 1980, p. 155.Google Scholar
- 12.A. R. SMITH, H. A. WOLLENBERG, High resolution gamma-ray spectrometry for the laboratory analysis of the uranium and thorium decay series, in: The Natural Radiation Environment II, J. A. S. ADAMS, W. M. LOWDER, T. F. GESSELL, (Eds), CONF-720805, Washington, D. C., 1972.Google Scholar
- 13.N. A. WOGMAN, Natural contamination in radionuclides detection system IEEE Trans. Nucl. Sci., (1981) 275.Google Scholar
- 14.W. H. ZIMMER, S. E. WAGNER, Nucl. Instr. Methods, 223 (1984) 412.Google Scholar